Spatio-Temporal Variations of Multiple Primary Air Pollutants Emissions in Beijing of China, 2006-2015

Air pollution in Beijing, China has attracted continuous worldwide public attention along with the rapid urbanization of the city. By implementing a set of air pollution mitigation measures, the air quality of Beijing has been gradually improved in recent years. In this study, the intrinsic factors leading to air quality improvement in Beijing are studied via a quantitative evaluation of the temporal and spatial changes in emissions of primary air pollutants over the past ten years. Based on detailed activity levels of each economic sector and a localized database containing source and pollutant specific emission factors, an integrated emissions inventory of primary air pollutants discharged from various sources between 2006 and 2015 is established. With the implementation of phased air pollution mitigation measures, and the Clean Air Action Plan, the original coal-dominated energy structure in Beijing has undergone tremendous changes, resulting in the substantial reduction of multiple air pollutants. The total of emissions of six major atmospheric pollutants (PM10, PM2.5, SO2, NOX, VOCs and NH3) in Beijing decreased by 35% in 2015 compared to 2006-this noticeable decrease was well consistent with the declining trend of ambient concentration of criterion air pollutants (SO2, PM10, PM2.5 and NO2) and air quality improvement, thus showing a good correlation between the emission of air pollutants and the outcome of air quality. SO2 emission declined the most, at about 71.7%, which was related to the vigorous promotion of combustion source control, such as the shutdown of coal-fired facilities and domestic stoves and transition to clean energy, like natural gas or electricity. Emissions of PM decreased considerably (by 48%) due to energy structure optimization, industrial structure adjustments, and end-of-pipe PM source control. In general, NOX, NH3, and VOCs decreased relatively slightly, by 25%, 14%, and 2%, respectively, and accordingly, they represented the limiting factors for improving air quality and the key points of air pollution mitigation in Beijing for the future.