期刊
ATMOSPHERIC ENVIRONMENT
卷 213, 期 -, 页码 470-484出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.atmosenv.2019.06.046
关键词
Black carbon; Optical properties; Radiative effects; Urban valley; OPAC; SBDART
资金
- Natural Science Foundation of China [41605103]
- Youth Innovation Promotion Association, CAS, China [2017462]
- Natural Science Foundation of Gansu, China [1606RJZA022]
- CAS Light of West China Program, China
- Opening Project of Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAPS), China [FDLAP16005]
- Excellent Post Doctoral Program, China [2016LH0020]
The concentrations, optical and radiative effects of carbonaceous aerosols were essential to studies of the climatic, environmental and health effects. The previous studies less combined numerical simulation with in-situ observations, especially for the aerosol vertical profiles. In this study, we off-line measured vertical profiles of submicron black carbon (BC) aerosols and on-line obtained aerosol optical properties over urban Lanzhou during 26 December 2017 to 11 January 2018. The BC optical properties and radiative effects were evaluated using Optical Properties of Aerosols and Clouds (OPAC) and Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) models. The absorption and scattering coefficients and optical depth of BC aerosols ranged from 9 to 83 M m(-1) , 3-24 M m(-1) and 0.02 to 0.2 respectively, which in average accounted for 50%, 3% and 11% of the optical properties of total aerosols during the study period. BC aerosol radiative forcing (ARF) within ATMOS (top-surface) varying from 16.6 to 108.8 W m(-2) accounted for 17.3%-97.4% of total aerosols ARF with an average of 66.6%, and the percentages increased significantly as BC concentrations increased during the period. The mean atmospheric heating rate (AHR) induced by BC aerosols was 1.94 K day(-1) ranging from 0.46 to 3.03 K day(-1) during the study period. This study contributes to understanding the impacts of light-absorbing aerosols on climate and haze pollution in an urban valley.
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