期刊
ACS PHOTONICS
卷 6, 期 6, 页码 1365-1371出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.9b00290
关键词
Berreman mode; epsilon-near-zero; infrared; nanophotonics; second harmonic generation; field enhancement
类别
资金
- Office of Naval Research [N00014-18-2107]
- Vanderbilt School of Engineering
Immense optical field enhancement was predicted to occur for the Berreman mode in ultrathin films at frequencies in the vicinity of epsilon-near-zero (ENZ). Here, we report the first experimental proof of this prediction in the mid-infrared by probing the resonantly enhanced second harmonic generation (SHG) at the longitudinal optic phonon frequency from a deeply subwavelength-thin aluminum nitride (AlN) film. Employing a transfer matrix formalism, we show that the field enhancement is completely localized inside the AlN layer, revealing that the observed SHG signal of the Berreman mode is solely generated in the AlN film. Our results demonstrate that ENZ Berreman modes in intrinsically low-loss polar dielectric crystals constitute a promising platform for nonlinear nanophotonic applications.
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