Article
Chemistry, Multidisciplinary
Jiang Cui, Hongkui Zheng, Kai He
Summary: Conversion-type materials are being explored as potential high-energy-density alternatives for rechargeable ion batteries, with in situ TEM being extensively employed to provide mechanistic insights into the behavior of battery materials. This review comprehensively summarizes recent developments in in situ TEM techniques for investigating dynamic phase transformation and associated structural, morphological, and chemical evolutions during conversion reactions with alkali ions in secondary batteries, with a special emphasis on spinel metal oxides and 2D metal chalcogenides. Unique scientific findings obtained through in situ TEM are highlighted, addressing fundamental questions and practical issues related to phase transformation, structural evolution, electrochemical redox, reaction mechanism, kinetics, and degradation.
ADVANCED MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Fei Qi, Qiuran Li, Wenxia Zhang, Qiang Huang, Bingyan Song, Yuanfu Chen, Jiarui He
Summary: In this study, a three-dimensional and freestanding ReS2/graphene heterostructure (3DRG) was synthesized for the first time via a one-pot hydrothermal method, which can be directly used as a freestanding and binder-free anode for lithium-ion batteries (LIBs). The 3DRG anode exhibits hierarchically sandwich-like, nanoporous, and conductive three-dimensional network constructed by two-dimensional ReS2/graphene heterostructural nanosheets. With a current density of 100 mA g-1, the 3DRG anode delivers a high reversible specific capacity of 653 mAh g-1. It also shows higher rate capability and cycling stability compared to the bare ReS2 anode.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Engineering, Environmental
Wei Li, Zhujun Yao, Shengzhao Zhang, Xiuli Wang, Xinhui Xia, Changdong Gu, Jiangping Tu
Summary: Sodium-vanadium fluorophosphates coated with polypyrrole show excellent rate capability and cycling stability in solid-state sodium ion batteries. The solid-state full sodium ion batteries based on this composite exhibit an attractive high energy density.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Chemistry, Physical
Fiaz Hussain, Hamza Maqbool, Songbai Han, Liping Wang, Jinlong Zhu, Yusheng Zhao, Wei Xia
Summary: This study utilized density functional theory (DFT) and DFT + U calculations to investigate the structural stability and performance of Na2FeS2 in sodium-ion batteries. The results revealed the instability of Na2FeS2, but it exhibited a low diffusion barrier and high theoretical capacity. Additionally, the substitution of transition metals at the Fe sites resulted in the promising Na2MnS2 with excellent structural stability and high theoretical capacity.
ACS APPLIED ENERGY MATERIALS
(2023)
Article
Energy & Fuels
El abadila Iffer, Mohammed Belaiche, Chouaib Ahmani Ferdi, Moustapha Elansary, Abdul Khader Sunar, Yanxia Wang, Yuliang Cao
Summary: The monoclinic alpha-NaVOPO(4) was synthesized using sol-gel method, and its poor electrochemical activity was attributed to its low intrinsic electronic conductivity. The material exhibits high voltage, good ionic conductivity and stability, but shows poor performance due to the large charge transfer resistance. Experimental and theoretical results explain the origin of this behavior, with detailed magnetic study also reported in this paper.
INTERNATIONAL JOURNAL OF ENERGY RESEARCH
(2021)
Article
Chemistry, Physical
Guisheng Liang, Xuhui Xiong, Liting Yang, Xianhu Liu, Renchao Che
Summary: Sodium-ion batteries (SIBs) have gained attention for grid-scale energy storage due to the abundance and cost-effectiveness of sodium. The development of electrode materials with stable long-term capacity remains a challenge. The use of Ca-CeVO4 compound as an electrode material shows exceptional cycling stability and high reversible capacity, contributing to the future design of stable electrode materials for long-life SIBs.
JOURNAL OF MATERIALS CHEMISTRY A
(2021)
Article
Multidisciplinary Sciences
Don H. McTaggart, Jack D. Sundberg, Lauren M. McRae, Scott C. Warren
Summary: This study systematically evaluates cathode materials for fluoride-ion batteries (FIBs) using the Materials Project crystal structure database. Promising ternary fluorides are identified based on structural stability and fluorination/defluorination reactions. Properties such as energy density, cost, and bandgaps are presented to facilitate the discovery of next-generation battery materials.
Article
Energy & Fuels
Gaushiya A. Shaikh, David Cornil, Sanjeev K. Gupta, Rajeev Ahuja, P. N. Gajjar
Summary: The applicability of a two-dimensional beta-antimonene monolayer as a negative electrode material for Na-, K-, and Mg-ion batteries has been studied, and it has been found to have low diffusion barriers and high storage capacity, offering excellent performance.
Article
Chemistry, Physical
Xian Yuan, Zhenhua Chen, Bin Huang, Yuping He, Naigen Zhou
Summary: The MoS2/M2CS2 heterostructures were found to be stable and exhibit metallic properties, with low diffusion barriers indicating excellent rate performances for various metal-ion batteries. The theoretical capacities for NIBs/LIBs were significantly higher than for KIBs/MIBs, demonstrating their suitability as anode materials. Additionally, the heterostructures showed promising potential for NIBs with lower open-circuit voltages and higher capacities compared to LIBs.
JOURNAL OF PHYSICAL CHEMISTRY C
(2021)
Article
Chemistry, Physical
Xiaoling Cui, Shimin Wang, Xiushen Ye, Xiaoqi Fan, Cankun Gao, Yin Quan, Shuxiang Wen, Xingpeng Cai, Jin Huang, Shiyou Li
Summary: In this study, the performance of the P2 phase layered manganese-based transition metal (TM) oxides in sodium-ion batteries (SIBs) is improved by doping with F and Mg. F-doping reduces capacity fading caused by irreversible phase transition and Jahn-Teller effect, while Mg-doping completely inhibits phase transition and mitigates the slide of TM layers. The double-doping of F and Mg synergistically improves the performance of SIBs.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Applied
Lulu Li, Ming Zhu, Guanyao Wang, Fangfang Yu, Liaoyong Wen, Hua-Kun Liu, Shi-Xue Dou, Chao Wu
Summary: In this study, a highly stable Bi-based sodiophilic substrate is reported to stabilize the sodium metal anode, effectively addressing challenges associated with side reactions and dendrite growth. The experimental results demonstrate that the asymmetric cells based on this substrate exhibit excellent electrochemical performance.
JOURNAL OF ENERGY CHEMISTRY
(2022)
Review
Chemistry, Multidisciplinary
Shuangyan Qiao, Qianwen Zhou, Meng Ma, Hua Kun Liu, Shi Xue Dou, Shaokun Chong
Summary: Rechargeable sodium-ion batteries (SIBs) face challenges in electrode materials due to the large ionic radius of Na-ion. However, progress has been made in intercalation, conversion, alloying, conversion-alloying, and organic anode materials for SIBs. Various optimization strategies have been summarized to improve the electrochemical properties of anodes. The merits, drawbacks, challenges, and future directions for high-performance anode materials are discussed.
Article
Nanoscience & Nanotechnology
By Noah B. Schorr, Igor Kolesnichenko, Laura C. Merrill, Bryan R. Wygant, Katharine L. Harrison, Timothy N. Lambert
Summary: This study demonstrates the application of synthesized FeS2 nanoparticles as a cathode material for stable cycling lithium batteries, when coupled with an optimized electrolyte. The research emphasizes the importance of nanoparticle design and appropriate voltage conditions in achieving high performance and avoiding detrimental substances in lithium batteries.
ACS APPLIED NANO MATERIALS
(2021)
Article
Chemistry, Physical
Neha Yadav, Brahmananda Chakraborty, T. J. Dhilip Kumar
Summary: The study demonstrates the potential of C-silicyne as the anode material for Na/K ion batteries. C-silicyne exhibits excellent electrochemical properties, high storage capacity, and low diffusion barriers, making it a promising electrode material for efficient and stable ion batteries.
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
(2021)
Article
Green & Sustainable Science & Technology
Yifei Yuan, Ryan Sharpe, Kun He, Chenghang Li, Mahmoud Tamadoni Saray, Tongchao Liu, Wentao Yao, Meng Cheng, Huile Jin, Shun Wang, Khalil Amine, Reza Shahbazian-Yassar, M. Saiful Islam, Jun Lu
Summary: Rechargeable aqueous Zn-MnO2 technology combines favorable sustainability characteristics, including safety, cost, and environmental compatibility. Advanced characterizations and theoretical calculations provide fresh insight into the charge storage mechanism, closing an ongoing debate and suggesting ways forward.
NATURE SUSTAINABILITY
(2022)
Article
Engineering, Environmental
Jintao Zhang, Dong-Sheng Li, Zhi Yi Leong, Jianbei Qiu, Xuhui Xu, Hui Ying Yang
Summary: Se substituted NiS2 nanoparticles decorated multichannel carbon fibers (MCF/NiSexS2-x) were fabricated as anode materials for lithium and sodium-ion batteries, showing enhanced reaction kinetics, improved electric conductivity, and superior structural stability. The MCF/NiSexS2-x anode delivered high capacity and stable cycle life for both Li and Na storage.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Materials Science, Multidisciplinary
Jingheng Nie, Bo Zhou, Shaofan Fang, Ye Wang, Yu Wang, Bingbing Tian, Hanlin Hu, Haizhe Zhong, Henan Li, Yumeng Shi
Summary: Metal halide perovskites (MHPs) are emerging semiconducting materials with exceptional opto-electronic properties. The exciton emission mechanism in MHPs is still not well understood due to their diverse chemical composition and versatile lattice structure. This review provides a critical overview of the experimental and theoretical approaches used to determine the exciton emission mechanism and summarizes the strategies for achieving efficient light emission in MHPs.
MATERIALS TODAY PHYSICS
(2023)
Article
Nanoscience & Nanotechnology
Shunqiong Jiang, Xue Liang Li, Daliang Fang, Wei Ying Lieu, Chen Chen, M. Shahnawaz Khan, Dong-Sheng Li, Bingbing Tian, Yumeng Shi, Hui Ying Yang
Summary: Lithium-sulfur (Li-S) batteries with hierarchical matrixes derived from metal-organic frameworks (MOFs) were developed to address the challenges of Li dendrite growth, electrochemical kinetics, and the shuttling effect of lithium polysulfides (LiPSs). The anode host CC-ZnO@Li demonstrated enhanced cycling stability, while the cathode host CC-NC-Co@S exhibited excellent electrochemical performance. The pouch cell based on these hosts showed good stability in different bending states, indicating the potential of high-performance Li-S batteries.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Nanoscience & Nanotechnology
Daliang Fang, Shaozhuan Huang, Tingting Xu, Pan Sun, Xue Liang Li, Yew Von Lim, Dong Yan, Yang Shang, Bing-Jian Su, Jenh-Yih Juang, Qi Ge, Hui Ying Yang
Summary: An efficient sulfur host, Zn-N-2@NG, consisting of atomic low-coordinated Zn-N-2 sites dispersed on N-rich microporous graphene, is proposed for sodium-sulfur batteries. It exhibits high sulfur content, high-rate capability, and long cycling stability. The Zn-N-2 sites demonstrate superior bidirectional catalysis on sulfur conversion, and in situ transmission electron microscopy reveals the difficulty of decomposing Na2S without liquid electrolytes, emphasizing the critical role of liquid electrolytes in the catalytic oxidation of Na2S.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Chemistry, Multidisciplinary
Liping Yang, Lu Guo, Dong Yan, Ye Wang, Ting Shen, Dong-Sheng Li, Mei Er Pam, Yumeng Shi, Hui Ying Yang
Summary: In this study, a hollow structure design and phase structure engineering were used to enhance the electrochemical performance of (Bi-Sb)2S3@N-C anode in potassium ion batteries (PIBs). The (Bi-Sb)2S3@N-C anode exhibited superior (de)-potassiation kinetics, excellent rate performance, and long cycling life due to the unique reaction mechanism and advantages of the hollow nanostructure with carbon shell. Additionally, the (Bi-Sb)2S3@N-C//PTCDA full cell showed a high reversible capacity after 300 cycles.
Article
Chemistry, Applied
Bolun Yu, Jingjing Yao, Haipu Li, Hui Ying Yang
Summary: The Fe2+-activated persulfate and H2O2 system showed efficient removal of mixed sulfonamides under a wide pH and temperature range. The coexistence of sulfate radicals and hydroxyl radicals in the system played a crucial role in the elimination of sulfonamides. The reaction rate constants of the radicals at different reactive sites explained the varying removal ratios of different sulfonamides.
APPLIED ORGANOMETALLIC CHEMISTRY
(2023)
Article
Engineering, Environmental
Xiao Liang, Kang Zhou, Dawei Duan, Fei Wang, Chuangye Ge, Xianfang Zhou, Mingjian Yuan, Yumeng Shi, Haoran Lin, Quanyao Zhu, Gang Li, Hanlin Hu
Summary: In this work, UiO-66, a classical Zr-MOFs material, was added to the PbI2 layer to improve the conversion process and durability of perovskite solar cells. The addition of UiO-66 changed the morphology of the PbI2 film, resulting in better contact with organic salt and enhanced perovskite conversion. It also suppressed halide vacancies formation and improved charge transport and optoelectronic properties. The UiO-66-assisted devices achieved a champion power conversion efficiency of 23.05% and improved stability compared to the pristine devices.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Nanoscience & Nanotechnology
Tingting Xu, Lijuan Hou, Congcong Yan, Jingrui Hou, Bofang Tian, Huiyu Yuan, Dezhi Kong, Hui Wang, Xinjian Li, Ye Wang, Guopeng Zhang
Summary: A heterogeneous seed layer of Au nanoparticles (NPs) is deposited on 3D porous vertical graphene nanosheets on carbon cloth (Au-VG/CC) to create a lithiophilic surface, resulting in a smooth and dendrite-free morphology. The Au-VG/CC electrode shows a small voltage hysteresis (67.2 mV) and long cycling life (more than 500 h) at a high current density of 5 mA cm-2 with 5 mAh cm-2. XRD and in-situ transmission electron microscopy reveal a lithiophilic layer of Li3Au, which guides lithium deposition. Furthermore, a full battery assembled with Li@Au-VG/CC anode and LiFePO4 cathode exhibits a capacity of 77.3 mAh g-1 at 100 mA g-1 after 200 cycles.
SCRIPTA MATERIALIA
(2023)
Article
Chemistry, Multidisciplinary
Daliang Fang, Tanmay Ghosh, Shaozhuan Huang, Ye Wang, Jianbei Qiu, Xuhui Xu, Hui Ying Yang
Summary: Designing effective catalysts is crucial for improving the performance of room-temperature sodium-sulfur batteries. This study successfully integrated two different catalysts (ZnS-NC@Ni-N-4) on nitrogen-doped carbon nanospheres to enhance the redox kinetics and inhibit the shuttle effect, resulting in high-performance RT Na-S batteries.
Article
Engineering, Chemical
Jingjing Yao, Jiayi Wen, Haipu Li, Ying Yang, Hui Ying Yang
Summary: The complexation of tetracyclines with Fe species plays a significant role in the removal of tetracyclines by ferrate. Experimental results show that the complexation of tetracyclines with Fe3+ contributes to 79% of the overall removal, followed by oxidation (11%) and adsorption/flocculation (10%). Thermodynamic and kinetic calculations suggest that complexation reactions between Fe3+ and tetracyclines are more likely to occur than oxidation reactions between ferrate and hydroxyl radicals. The complexation rates of tetracyclines with Fe3+ determine the removal of multiple tetracyclines by ferrate, highlighting the importance of considering complexation in the removal of pollutants.
SEPARATION AND PURIFICATION TECHNOLOGY
(2023)
Article
Materials Science, Multidisciplinary
Feier Fang, Wenlong He, Zexiang Liu, Ke Jiang, Ye Wang, Fuming Chen, Henan Li, Yumeng Shi
Summary: A lead-free double perovskite (Cs2AgBiBr6) has attracted attention for optoelectronic applications due to its non-toxicity, high stability, and high detection sensitivity. By reducing grain boundaries, non-radiative recombination can be suppressed, leading to the potential for good performance in photodetector applications. This study synthesized high-quality, large-area Cs2AgBiBr6 thin films using a blade-coating method under ambient conditions, providing a promising approach for the development of environmentally friendly and high-performance optoelectronic devices.
JOURNAL OF MATERIALS CHEMISTRY C
(2023)
Article
Engineering, Chemical
Liping Yang, Yixiang Li, Lu Guo, Pin Ma, Zhi Yi Leong, Jing Wang, Hui Ying Yang
Summary: This study aims to extract high-quality water for potable and industrial use from unconventional water sources using innovative methods. An innovative adsorbent was used to reduce boron and chloride levels in brackish water, and a capacitive deionization system was employed for chloride ion removal. The results demonstrate that this approach can meet water quality standards while significantly reducing chemical costs.
Article
Engineering, Electrical & Electronic
Ela Sachyani Keneth, Rama Lieberman, Avishag Pahima, V. B. Varma, Vinay Sharma, Chao Yuan, Qi Ge, R. V. Ramanujan, Shlomo Magdassi
Summary: Soft robots with flexible magnetic actuators are capable of delicate and sensitive movements. This study introduces a new method of fabricating 2D and 3D magneto-thermal actuators using a printing process. These actuators can be remotely and wirelessly activated by an alternating magnetic field, and demonstrate excellent performance in shape morphing. The findings suggest the potential of these magneto-thermal actuators in soft robotics, addressing the need for wireless and remote activation.
SENSORS AND ACTUATORS A-PHYSICAL
(2023)
Article
Chemistry, Physical
Sirinya Ukasi, Paritta Jutapukti, Chiranicha Ninthub, Nattapong Pinpru, Phakkhananan Pakawanit, Wanwilai Vittayakorn, Satana Pongampai, Naratip Vittayakorn, Thitirat Charoonsuk
Summary: This study explores the enhancement of electrical output of flexible hybrid piezoelectric-triboelectric nanogenerators by incorporating gamma-glycine into fully organic composites. The research demonstrates the importance of optimized concentrations of gamma-glycine and chitosan in achieving superior performance. The study identifies the critical content of gamma-glycine that leads to the highest output signal, and provides theoretical explanations for this observation.
Article
Chemistry, Physical
Yoonsang Ra, Yu-seop Kim, Seonmo Yang, Namgyu Kang, Gyuwon Oh, Chungyeon Cho, Sangmin Lee, Dongwhi Choi
Summary: In this study, a portable energy harvester (STEP) was proposed to drive various functional LEDs using biomechanical energy. The roles and functionalities of a triboelectric nanogenerator (TENG) and electromagnetic generator (EMG) in the hybrid energy harvester were experimentally demonstrated, and the necessity of hybridization for LED-involved devices was described. The STEP showed promising potential as an effective energy supply strategy for various functional LEDs in related industries.
Article
Chemistry, Physical
Dae Sol Kong, Kyung Hoon Kim, Ying Chieh Hu, Jong Hun Kim, Inseo Kim, Jeongwan Lee, Joonhyuk Lee, Won Hyuk Shon, Hanjin Yoo, Chul-Un Ro, Seungsu Lee, Hyoungjeen Jeen, Minbaek Lee, Minseok Choi, Jong Hoon Jung
Summary: With the rapid development of the Internet of Things and artificial intelligence, smart home has emerged to fulfill the security, convenience, and energy-saving issues of modern life. A flexoelectric mica crystal is used to augment the finger touch-driven triboelectric output for operating a wireless and multichannel smart home controller. This work provides important ingredients for enhancing triboelectric output and realizing a convenient, multifunctional, cost-effective, and adaptable smart home control system without batteries.
Article
Chemistry, Physical
Yi Han, Fang Wu, Xiaozhen Du, Zihao Li, Haixiang Chen, Dongxing Guo, Junlei Wang, Hong Yu
Summary: This paper presents a novel type of triboelectric nanogenerator that utilizes wind energy, with a Y-type bluff body to enhance vibration and output power. The application of this generator successfully provides power for a wireless temperature and humidity sensor.
Article
Chemistry, Physical
Wen Zhang, Fangyuan Cheng, Miao Chang, Yue Xu, Yuyu Li, Shixiong Sun, Liang Wang, Leimin Xu, Qing Li, Chun Fang, Meng Wang, Yuhao Lu, Jiantao Han, Yunhui Huang
Summary: This study successfully induced the formation of a uniform and robust CEI by constructing ZrO2 nano-rivets on the surface of LCO, stabilizing the surface of high-voltage LCO and facilitating lithium-ion diffusion.
Article
Chemistry, Physical
Karl P. Olson, Laurence D. Marks
Summary: This paper investigates the role of contacting shapes in triboelectricity and provides scaling rules for designing energy harvesting devices.
Article
Chemistry, Physical
Jong-An Choi, Jingu Jeong, Mingyu Kang, Hee-Jin Ko, Taehoon Kim, Keun Park, Jongbaeg Kim, Soonjae Pyo
Summary: Wind-driven triboelectric nanogenerators (WTENGs) are a promising emerging technology for sustainable wind energy harvesting, offering high output performance, lightweight design, and compact dimensions. This study introduces an innovative WTENG design that leverages a rolling-based mechanism to achieve efficient omnidirectional wind energy harvesting.
Article
Chemistry, Physical
Liwei Dong, Qian Tang, Chaoyang Zhao, Guobiao Hu, Shuai Qu, Zicheng Liu, Yaowen Yang
Summary: This paper proposes a novel hybrid scheme for flag-type nanogenerators (FNGs) that enhances their performance and broadens their operational wind speed ranges by harnessing the synergistic potential of two aerodynamic behaviors. The proposed flag-type triboelectric-piezoelectric hybrid nanogenerator (FTPNG) integrates flapping piezoelectric flags (PEFs) and a fluttering triboelectric flag (TEF). The FTPNG achieves significant power generation and a broad wind speed range, surpassing other FNGs, making it suitable for various self-powered systems and Internet of Things applications.
Review
Chemistry, Physical
Yunmeng Li, Xin Liu, Zewei Ren, Jianjun Luo, Chi Zhang, Changyong (Chase) Cao, Hua Yuan, Yaokun Pang
Summary: The demand for green and eco-friendly materials is growing due to increasing environmental concerns related to traditional petroleum-based products. Marine biomaterials have emerged as a promising alternative, thanks to their abundant availability, biocompatibility, biodegradability, and low toxicity. In this review, we discuss the development and applications of triboelectric nanogenerators (TENGs) based on marine biomaterials. The operational modes, foundational principles, intrinsic qualities, and advantages of marine biomaterials commonly used in TENG designs are highlighted. Approaches to enhance the efficacy of TENGs derived from marine biomaterials are also discussed, along with documented applications from existing literature. Furthermore, the existing challenges and future directions in marine biomaterial-inspired TENGs are explored.
Article
Chemistry, Physical
Matthew P. Wells, Adam J. Lovett, Yizhi Zhang, Zhongxia Shang, Kosova Kreka, Babak Bakhit, Haiyan Wang, Albert Tarancon, Judith L. MacManus-Driscoll
Summary: Reversible solid oxide cells (rSOCs) offer a promising solution to efficient energy conversion, but have been limited in portable power and electrolysis applications due to excessive polarisation resistance of the oxygen electrode at low temperatures. This study demonstrates the growth of symmetric and complete rSOC structures with reduced polarisation resistance by tuning oxygen vacancy through annealing, providing a promising route towards high-performance rSOC devices for portable power applications.
Article
Chemistry, Physical
Kangkang Bao, Minghui Wang, Yue Zheng, Panpan Wang, Liwen Yang, Yang Jin, Hui Wu, Bin Sun
Summary: This study utilizes ethanol as an electrolyte additive to modulate the migration of zinc ions and the surface structure of zinc anodes, resulting in improved capacity retention and cycle life of zinc-based aqueous batteries.
Article
Chemistry, Physical
Haichao Yang, Wensi Cai, Ming Wang, Saif M. H. Qaid, Zhiyuan Xu, Huaxin Wang
Summary: The introduction of sodium alginate (SA) into perovskite solar cells improves the carrier dynamics, stability, and performance by inhibiting nonradiative recombination and retarded charge dynamics.
Article
Chemistry, Physical
Cuirong Zhang, Mingyuan Wei, Zihan Chen, Wansheng Lin, Shifan Yu, Yijing Xu, Chao Wei, Jinwei Zhang, Ziquan Guo, Yuanjin Zheng, Qingliang Liao, Xinqin Liao, Zhong Chen
Summary: Artificial Intelligence of Things (AIoT) aims to establish smart and informative interactions between humans and devices. However, common pixelated sensing arrays in AIoT applications present problems such as hard and brittle devices, complex structures, and low precision. This article introduces an innovative solution called the all-in-one intelligent semitransparent interactive nerve patch (AISI nerve patch), which integrates sensing, recognition, and transmission functionalities into a thin and flexible patch. The AISI nerve patch is semitransparent, allowing for accurate identification without affecting aesthetics, and it can be attached to any curved surface for intelligent and interactive applications. With rapid response time and high precision recognition, it enables the integration of artificial intelligence and achieves high recognition accuracy for further development of AIoT.
Article
Chemistry, Physical
Youcun Bai, Heng Zhang, Huijun Song, Chong Zhu, Lijin Yan, Qin Hu, Chang Ming Li
Summary: A novel stainless-steel supported lattice-mismatched V-S-Se layered compound with high selenium vacancy was synthesized by adjusting the molar ratio of sulfur to selenium. The introduction of selenium vacancies created additional redox peaks of sulfur, providing more mass transport channels and active sites for zinc ions. The specific capacity and cycle stability of the electrode were significantly improved, demonstrating great potential for practical applications and providing insights into the effects of defects on battery performance.
Article
Chemistry, Physical
Yao Xiao, Puxian Xiong, Yakun Le, Zhenjie Lun, Kang Chen, Zhiduo Wang, Peishan Shao, Zhicong Chen, Dongdan Chen, Zhongmin Yang
Summary: This study successfully synthesized a material with multi-stimulus-responsive luminescence and confirmed the internal relationship between luminescence and defects by regulating the distribution and depth of defects. The dynamic process of multi-stimulus-responsive luminescence was validated by experimental and calculation results.