期刊
JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY
卷 19, 期 8, 页码 5287-5294出版社
AMER SCIENTIFIC PUBLISHERS
DOI: 10.1166/jnn.2019.16826
关键词
Biomass; 3D Hierarchical Structure; BiOX(X = Cl, Br)-(CMC)
类别
资金
- Fuzhou science and technology project [2017-G-90]
- project of Fujian Provincial Department of Education [JAT170390]
3D hierarchical structure BiOX(X = Cl, Br)-(CMC) assembled from 2D nanosheets with {010) facets exposed have been successfully synthesized by the assistance of biomass solvent CMC-Na. All the nitrogen adsorption isotherms and photoelectrochemical results reflected that BiOX(X = Cl, Br)-(CMC) exhibit higher specific surface area, superior optical absorption efficiency and separation efficiency of photoinduced electron-hole than BiOX(X=Cl, Br) 2D nanosheets exposed with {001} facets. Besides, 96.5% and 60.3% of tetracycline hydrochloride (TC) were photodegradated in 60 minutes under the visible light irradiation catalyzed by BiOBr-(CMC) and BiOCl-(CMC), which is much better than BiOBr and BiOCl. The formation and enhanced photocatalytic activity of 3D hierarchical structure BiOX-(CMC) may be ascribe to the bi-functional groups of CMC, which can affect the crystallization process and morphology of BiOX. According to the merit of environmental friendly and improved photocatalytic activity of the 3D hierarchitecture, we believe that this work broadens the possibility of designing efficient BiOX photocatalyst with {010} facets exposed.
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