期刊
ORGANIC LETTERS
卷 21, 期 10, 页码 3813-3816出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b01258
关键词
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资金
- NIH-NIGMS [GM 124030]
- University of Michigan Rackham dissertation fellowship
The Pd-catalyzed coupling of malonate nucleophiles with alkenes bearing tethered aryl or alkenyl triflates is described. These alkene difunctionalization reactions afford malonate-substituted cyclopentanes that contain fused aryl or cycloalkenyl rings. The transformations generate a five-membered ring, two C-C bonds, and provide products bearing up to three stereocenters with good chemical yield and generally high diastereoselectivity.
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