4.6 Article

Chiral selection rules for multi-photon processes in two-dimensional honeycomb materials

期刊

OPTICS LETTERS
卷 44, 期 9, 页码 2141-2144

出版社

OPTICAL SOC AMER
DOI: 10.1364/OL.44.002141

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  1. National Natural Science Foundation of China (NSFC) [11622429]
  2. National Basic Research Program of China [2014CB921601]
  3. National Key Research and Development Program of China [2016YFA0300900, 2016YFA0301002]
  4. Shanghai Education Development Foundation [18SG02]
  5. National Program for Support of Top-Notch Young Professionals

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We examine the chirality-dependent optical selection rules in two-dimensional monolayer materials with honeycomb lattices, and, based on symmetry argument, we generalize these rules to multi-photon transitions of arbitrary orders. We also present the phase relations between incident and outgoing photons in such processes. The results agree nicely with our experimental observations of second-and third-harmonic generation. In particular, we demonstrate that the phase relation of chiral second-harmonic generation can serve as a handy tool for imaging domains and domain boundaries of these monolayers. Our results can benefit future studies on chirality-related optical phenomena and opto-electronic applications of such materials. (C) 2019 Optical Society of America

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