Article
Chemistry, Physical
Xiaofeng Shen, Yan Zhang, Zhun Shi, Shengdao Shan, Jianshe Liu, Lisha Zhang
Summary: The study developed a CF cloth with C3N4/CdS nanostructures as a filter-membrane-shaped photocatalyst, showing superior photocatalytic activity, especially in terms of the removal rates of dyes and pollutants. Additionally, possible reaction pathways were proposed, providing new insights for research in wastewater purification.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Chemistry, Physical
Ting Liu, Yan Zhang, Zhun Shi, Wei Cao, Lisha Zhang, Jianshe Liu, Zhigang Chen
Summary: This study presents a recyclable and efficient photocatalyst with broad-spectral-response constructed on carbon fiber cloth for flowing wastewater treatment. The photocatalyst exhibited high removal efficiencies of rhodamine B, acid orange 7, and tetracycline under visible light irradiation, outperforming traditional photocatalysts.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2021)
Article
Biotechnology & Applied Microbiology
Neriamara Martins-West, Ana Martin-Ryals, Bryan Maxwell, Lance Schideman
Summary: Anaerobic membrane bioreactors (AnMBR) have limitations in membrane cleaning energy demand and membrane flux. This study presents a novel AnMBR configuration, cloth filter anaerobic membrane bioreactor (CFAnMBR), which uses a commercially available cloth filter technology to improve the membrane flux and reduce the cleaning energy demand. The CFAnMBR demonstrates significant improvement in membrane flux and cleaning energy demand compared to previously reported AnMBR configurations.
FRONTIERS IN BIOENGINEERING AND BIOTECHNOLOGY
(2023)
Article
Environmental Sciences
Yubing Sun, Jingting Xiao, Xinshui Huang, Peng Mei, Huihui Wang
Summary: This study investigated the factors affecting the photocatalytic reduction of U(VI) by MoS2/CdS composite and optimized the experimental conditions. The results showed that 2.5 wt% MoS2/CdS composite had high U(VI) removal efficiency and good stability, indicating its potential application in environmental remediation.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2022)
Article
Nanoscience & Nanotechnology
Lulu Zhang, Jingxuan He, Na Li, Jie Yuan, Wenjuan Li, Ping Liu, Tingjiang Yan
Summary: This study presents a new ternary CdS@MoS2-Co3O4 multiheterojunction photocatalyst, which improves the solar energy conversion efficiency and long-term stability by regulating the charge transfer mechanism.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Engineering, Environmental
Wenda Kang, Shuo Chen, Hongtao Yu, Tengyao Xu, Shuai Wu, Xiaoting Wang, Na Lu, Xie Quan, Heng Liang
Summary: The study improved the mass-transfer performance of the PCO/O-3 process by using a helical photocatalytic module (HPM) in an annular UVC reactor, resulting in significantly higher TOC removal efficiency. The flowing through reactor demonstrated good stability in a continuous test, and the energy efficiency of the PCO/O-3 process in this reactor was higher compared to other processes.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Chemistry, Physical
Kang Peng, Linjie Zuo, Yihan Wang, Jingying Ye, Hongjie Wang, Yanlin Jia, Min Niu, Lei Su, Lei Zhuang, Xiaoyu Li
Summary: Reduced graphene oxide coated montmorillonite (rGO/Mt) was used as a hydrophilic conductive catalyst carrier to assemble CdS and MoS2 heterostructures. The composites exhibited efficient photocatalytic H2 evolution rate due to the synergistic effect of the carrier material.
APPLIED CLAY SCIENCE
(2023)
Article
Chemistry, Multidisciplinary
Shuyan Qi, Ruiyan Zhang, Yiming Zhang, Kaiyao Zhang, Huanyan Xu
Summary: The photocatalyst WS2/MoS2/CdS (WMC) was synthesized using a coprecipitation hydrothermal method, with WS2/MoS2 loaded on the CdS surface. The addition of WS2/MoS2 reduced the bandwidth of CdS and improved the photocatalytic efficiency, resulting in a higher reaction rate constant and relatively stable catalytic activity. The active groups in the photocatalytic degradation process were identified as O-2(-) and h(+).
NEW JOURNAL OF CHEMISTRY
(2022)
Article
Chemistry, Multidisciplinary
Chuanbiao Bie, Bicheng Zhu, Linxi Wang, Huogen Yu, Chenhui Jiang, Tao Chen, Jiaguo Yu
Summary: A bifunctional dual-cocatalyst-modified photocatalyst is constructed for hydrogen evolution and selective pyruvic acid production. A two-step single-electron route for pyruvic acid production is proposed based on monitoring the intermediates.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Engineering, Chemical
Haitao Fu, Hongming Zhao, Xiaohong Yang, Shixian Xiong, Xizhong An
Summary: This study demonstrates high-performance visible-light-driven H-2-evolution photocatalysts based on novel CdS nanodiamonds decorated with MoS(2) nanosheets. The composites exhibited enhanced photocatalytic performances due to improved optical absorption range, low recombination rate of the photo-generated electrons and holes, extra generated charges, excellent charge transfer ability, and increased donor density.
Article
Engineering, Electrical & Electronic
Nikolaos Karamoschos, Feidias Bairamis, Konstantinos S. Andrikopoulos, Ioannis Konstantinou, Dimitrios Tasis
Summary: This study describes the synthesis of metal-doped CdS/MoS2 heterojunctions using a two-step microwave-assisted solvothermal approach, and characterizes the samples using various analytical techniques. The photocatalytic activity is influenced by the number of heterojunctions and the ratio of molybdenum-based species within the materials.
MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING
(2022)
Article
Materials Science, Ceramics
Hui Qiao, Rong Hu, Zongyu Huang, Shengqian Liu, Xiang Qi
Summary: Cadmium sulfide (CdS) is an effective semiconductor catalyst utilized in split water hydrogen evolution, but rapid recombination of photogenerated electron-hole pairs hinders its application. The synthesis of a CdS/MoS2 mixed-dimensional heterojunction improves the photocatalytic performance by promoting separation of electron-hole pairs and leveraging MoS2 as a co-catalyst. Additional enhancement in photocatalytic activity with nearly four times improvement is achieved by applying a voltage, facilitating faster carrier mobility and better photocatalytic performance.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2021)
Article
Engineering, Environmental
Xinxin Lu, Weijian Chen, Yin Yao, Xiaoming Wen, Judy N. Hart, Constantine Tsounis, Cui Ying Toe, Jason Scott, Yun Hau Ng
Summary: A series of MoS2-loaded CdS nanorods have been fabricated, with MoS2 spatially distributed on the tips or both tips and walls of the CdS NRs. The presence of a spatial electric field between CdS NRs and MoS2 tips strongly induces photogenerated electron-hole separation and electron transfer. MoS2 located on the tips of CdS NRs can better separate electron-hole pairs and suppress charge recombination, leading to superior photoactivity.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Engineering, Chemical
Yun Jia, Yu Zhang, Xuan Zhang, Jiahao Cheng, Yujiao Xie, Yuan Zhang, Xiaoyan Yin, Feng Song, Hongyou Cui
Summary: Polyaniline (PANI) and multi-walled carbon nanotubes (MWCNTs) were incorporated into hollow CdS spheres to create CdS/PANI/MWCNTs nanocomposites. These nanocomposites were utilized as photo-catalysts for the degradation of sodium butyl xanthate (SBX) in wastewater. The optimized CdS/PANI/MWCNTs catalyst exhibited excellent ultraviolet-light-driven photocatalytic performance with a degradation rate of 99.2% in 70 minutes. The enhanced catalytic activity was attributed to the facilitated separation of photogenerated electrons and holes by PANI, as well as the promotion of SBX adsorption and electron migration by MWCNTs. The stability of CdS/PANI/MWCNTs was also demonstrated by the inhibited photocorrosion of CdS.
SEPARATION AND PURIFICATION TECHNOLOGY
(2023)
Article
Chemistry, Physical
Kaixuan Zhuge, Zhoujie Chen, Yuqi Yang, Jin Wang, Yangyi Shi, Zhengquan Li
Summary: The study introduced a simple method for in-situ growth of MoS2 onto CdS quantum dots, forming CdS/MoS2 composite photocatalysts. These photocatalysts exhibit excellent catalytic activity and superior photocatalytic durability, providing new opportunities for developing new types of photocatalysts based on quantum dots.
APPLIED SURFACE SCIENCE
(2021)
Article
Engineering, Environmental
Wei Cao, Yan Zhang, Zhun Shi, Ting Liu, Xinshan Song, Lisha Zhang, Po Keung Wong, Zhigang Chen
Summary: By decorating UiO-66-NH2 nanoparticles as a co-photocatalyst on carbon fibers, the MoS2-based nanocomposites show significantly improved adsorption and photocatalytic performance for eliminating pollutants. The material can efficiently adsorb and remove LVFX and Cr(VI) within 60 minutes, with a slight decline in performance after visible light irradiation for 4 cycles.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Chemistry, Physical
Xiaofeng Shen, Yan Zhang, Zhun Shi, Shengdao Shan, Jianshe Liu, Lisha Zhang
Summary: The study developed a CF cloth with C3N4/CdS nanostructures as a filter-membrane-shaped photocatalyst, showing superior photocatalytic activity, especially in terms of the removal rates of dyes and pollutants. Additionally, possible reaction pathways were proposed, providing new insights for research in wastewater purification.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Green & Sustainable Science & Technology
Yan Zhang, Meiyu Xiong, Anran Sun, Zhun Shi, Bo Zhu, Daniel K. Macharia, Fang Li, Zhigang Chen, Jianshe Liu, Lisha Zhang
Summary: The study introduced a novel porous co-photocatalyst to decorate carbon fibers, which can efficiently remove pharmaceutical pollutants and exhibit enhanced performance under visible light irradiation.
JOURNAL OF CLEANER PRODUCTION
(2021)
Article
Chemistry, Physical
Ting Liu, Yan Zhang, Zhun Shi, Wei Cao, Lisha Zhang, Jianshe Liu, Zhigang Chen
Summary: This study presents a recyclable and efficient photocatalyst with broad-spectral-response constructed on carbon fiber cloth for flowing wastewater treatment. The photocatalyst exhibited high removal efficiencies of rhodamine B, acid orange 7, and tetracycline under visible light irradiation, outperforming traditional photocatalysts.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2021)
Article
Engineering, Environmental
Yan Zhang, Anran Sun, Meiyu Xiong, Daniel K. Macharia, Jianshe Liu, Zhigang Chen, Maoquang Li, Lisha Zhang
Summary: Fabrication of weavable CF/TiO2/BiOI bundles on carbon fiber allows for strong and broad-spectrum photoabsorption, leading to superior adsorption and photodegradation efficiency for various pollutants. The reusable macroscopic photocatalyst retains excellent photocatalytic activity even after multiple cycles, showing potential for environmental purification applications.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Engineering, Environmental
Daniel K. Macharia, Shamima Sarker, Bo Zhu, Yan Zhang, Zixiao Liu, Nuo Yu, Zhigang Chen
Summary: Photoreversible color switching fabrics with high photocatalytic and photothermal effects were achieved by tuning the plasmonic performance of ZnO nanocrystals through indium doping. The semiconductor-catalyzed systems, combined with redox dyes, can be utilized to design novel color switching systems and switchable fabrics/papers with mono/multi-color response features, showing potential for advanced sensors and rewritable media.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Chemistry, Physical
Jiafeng Cai, Yan Zhang, Tianwei Qian, Xiaolong Li, Zhigang Chen, Lisha Zhang
Summary: A recyclable photocatalyst, consisting of BiOBr/BiOI nanojunctions on a flexible carbon fiber cloth substrate, was developed for efficient degradation of pollutants in wastewater under visible-light illumination. The photocatalyst exhibited superior performance compared to BiOBr alone, with high degradation rates of various pollutants and a significant reduction in chemical oxygen demand (COD) concentration. This recyclable catalyst holds great potential for wastewater purification.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Physical
Tianwei Qian, Yan Zhang, Jiafeng Cai, Wei Cao, Ting Liu, Zhigang Chen, Jianshe Liu, Fang Li, Lisha Zhang
Summary: A recyclable photocatalyst with high adsorption and photocatalytic performance was developed by constructing a three-component photocatalyst on carbon fiber cloth, which effectively treated antibiotics in flowing sewage.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2021)
Article
Engineering, Environmental
Congcong Li, Bo Zhu, Zixiao Liu, Jiangtong Zhao, Ruru Meng, Lisha Zhang, Zhigang Chen
Summary: This study presents the development of an anionic polyelectrolyte-based hydrogel with both photothermal characteristics for evaporating seawater and electrostatic properties for preventing solid-salt crystallization. The hydrogel exhibited high solar absorption efficiency and excellent evaporation performance, making it a promising candidate for solar-driven seawater desalination.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Physical
Yan Zhang, Wei Cao, Bo Zhu, Jiafeng Cai, Xiaolong Li, Jianshe Liu, Zhigang Chen, Maoquan Li, Lisha Zhang
Summary: This study successfully prepared an efficient and reusable photocatalyst by synthesizing ultrasmall Ti MOF nanodots on carbon fiber based MoS2. The nanodots showed improved surface area and generated more reactive oxygen species, resulting in enhanced pollutant removal performance. The easy-recyclable nanodots-based heterojunctions exhibited high stability and showed great potential for wastewater purification.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Energy & Fuels
Bo Zhu, Jiangtong Zhao, Yangfan Meng, Zixiao Liu, Nuo Yu, Lisha Zhang, Zhigang Chen
Summary: Solar-enabled interfacial steam generation is hindered by high material cost and low evaporation rate. In this study, a 3D carbon aerogel (CA) with hierarchical pores was prepared and utilized as an efficient photothermal material for seawater desalination. The CA showed broad and strong light absorption, and when incorporated into a 3D evaporator, exhibited high evaporation rate and long-term stability under simulated sunlight.