Review
Chemistry, Multidisciplinary
Luca Burratti, Erica Ciotta, Fabio De Matteis, Paolo Prosposito
Summary: Heavy metal ions and pesticides pose great dangers to human health and the environment, making accurate detection essential. Traditional methods are expensive and complex, but recent technological advancements have made optical techniques based on noble metal nanomaterials a viable alternative, offering many advantages.
Review
Nanoscience & Nanotechnology
Armin Salek Maghsoudi, Shokoufeh Hassani, Kayvan Mirnia, Mohammad Abdollahi
Summary: Heavy metals pose significant environmental pollution and health hazards. Novel biosensors utilizing nanotechnology have been designed to detect ultra-trace amounts of heavy metals effectively and efficiently. Aptamers and whole cells are important bio-functional nanomaterials utilized in the design of heavy metal biosensors.
INTERNATIONAL JOURNAL OF NANOMEDICINE
(2021)
Article
Environmental Sciences
Mohamed A. Saad, Mahmoud A. S. Sakr, Vasil A. Saroka, Hazem Abdelsalam
Summary: Using density functional theory, this study investigates the interaction between covalent organic frameworks and heavy metal pollutants, finding that specific functional groups can effectively form strong chemical bonds with harmful metals, thereby increasing the reactivity of covalent organic frameworks.
Review
Chemistry, Analytical
Yi-Kun Li, Ting Yang, Ming-Li Chen, Jian-Hua Wang
Summary: This review discusses the application of nanomaterials in heavy metal analysis and emphasizes the importance of functionalizing traditional materials and utilizing bio-functional materials to enhance specificity. The hybridization of multiple materials can improve material properties, enabling the development of novel sensor systems or achieving detection-removal integration. Despite progress, challenges remain in the specificity and anti-interference performance of new nanomaterials and nanotechnology.
CRITICAL REVIEWS IN ANALYTICAL CHEMISTRY
(2021)
Article
Engineering, Environmental
Kandasamy Saravanakumar, Sugavaneswaran SivaSantosh, Anbazhagan Sathiyaseelan, Kumar Vishven Naveen, Mohamed Ali AfaanAhamed, Xin Zhang, Veeraraghavan Vishnu Priya, Davoodbasha MubarakAli, Myeong-Hyeon Wang
Summary: Marine pollution is a highly overlooked form of pollution that seriously affects aquatic life and public health in coastal areas. Various hazardous pollutants in the marine ecosystem have been linked to genetic disorders and diseases such as cancer, diabetes, and neurological disorders. Recent studies have highlighted the presence of microplastics, even in the human placenta, raising concerns globally. Nanomaterials have shown promise in detecting and remediating these contaminants. This comprehensive review discusses the sources and distribution of diverse marine pollution, as well as its impact on aquatic animals and coastal public health. The applicability and advancement of nanomaterials and nano-based biosensors in detecting, preventing, and remediating marine pollution are also examined.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Review
Engineering, Environmental
Harpreet Singh, Amy Bamrah, Sanjeev K. Bhardwaj, Akash Deep, Madhu Khatri, Ki-Hyun Kim, Neha Bhardwaj
Summary: This review focuses on the recent developments in fluorescent nanosensing technology for the detection of lead ions (Pb2+), highlighting the classification and evaluation of different types of nanomaterials, especially in terms of sensitivity.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Environmental Sciences
Ahmad Shakeel, Komal Rizwan, Ujala Farooq, Shahid Iqbal, Tanveer Iqbal, Nasser S. Awwad, Hala A. Ibrahium
Summary: A large number of people suffer from waterborne diseases caused by contaminated drinking water. Polymeric nanocomposites have been developed as a solution for detecting heavy metals, pesticides, and antibiotics in the environment.
Review
Water Resources
Bharti, J. S. Jangwan, Smita S. Kumar, Vivek Kumar, Amrish Kumar, Dushyant Kumar
Summary: This paper discusses the issues of heavy metals and pesticides in water decontamination, and introduces the latest research results of adsorption and photocatalysis as two removal methods.
APPLIED WATER SCIENCE
(2022)
Review
Chemistry, Analytical
Salim Ullah, Qurat ul Ain Zahra, Mojtaba Mansoorianfar, Zahid Hussain, Ismat Ullah, Wenjing Li, Edward Kamya, Shah Mehmood, Renjun Pei, Jine Wang
Summary: Heavy metal ions as metallic pollutants pose a global issue due to their harmful effects on the aquatic ecosystem and human health. Conventional detection methods have limitations, making the development of an efficient method for on-site and real-time detection of heavy metal residues crucial. Aptamer-based sensors, with their high sensitivity, ease of production, simplicity, specificity, stability, low immunogenicity, and cost-effectiveness, offer advantages over antibodies. When combined with nanomaterials, nucleic acid aptamers can selectively bind to metal ions, enabling on-site monitoring of their residues.
CRITICAL REVIEWS IN ANALYTICAL CHEMISTRY
(2022)
Review
Chemistry, Multidisciplinary
Chinchu Gibi, Cheng-Hua Liu, Scott C. Barton, Jerry J. Wu
Summary: This review presents the application of well-tuned nanomaterials in heavy metal ion sensing. The sensing performance for heavy metal ions can be effectively influenced by the dimensional characteristics of nanomaterials.
Review
Environmental Sciences
Abdelmonaim Azzouz, Lamia Hejji, Vanish Kumar, Ki-Hyun Kim
Summary: Diverse aptasensors have been developed through the combination of aptamers with nanomaterials for the timely and efficient detection of metals in environmental and biological matrices. These sensors have multiple advantages such as heightened sensitivity, facile production, uncomplicated operation, exceptional specificity, enhanced stability, low immunogenicity, and cost-effectiveness.
ENVIRONMENTAL RESEARCH
(2023)
Review
Food Science & Technology
Ruonan Meng, Qiujin Zhu, Tingyu Long, Xuli He, Zewei Luo, Ronghui Gu, Wenzhong Wang, Ping Xiang
Summary: Food safety is a major global concern, especially in terms of heavy metal contamination in foods. Electrochemical sensors have emerged as a promising strategy for detecting heavy metals due to their flexibility, selectivity, and accuracy. This review highlights the advances in electrochemical sensors for heavy metal detection in foods, including the use of various modified electrodes. The review also discusses the challenges, applications, and prospects of electrochemical sensors in ensuring food safety.
Review
Environmental Sciences
B. Senthil Rathi, P. Senthil Kumar, Dai-Viet N. Vo
Summary: This article discusses the impact of water pollution on the environment and health, introduces the presence and treatment methods of hazardous pollutants in wastewater effluents, and emphasizes the importance of risk assessment for hazardous pollutants.
SCIENCE OF THE TOTAL ENVIRONMENT
(2021)
Review
Chemistry, Multidisciplinary
Vinay Sharma, Pranav Tiwari, Navpreet Kaur, Shaikh M. Mobin
Summary: The increasing contamination of environmental media poses a serious health issue that requires advanced methods for detecting pollutants. Carbon dot sensors show unique advantages in detecting contaminants in water samples, with high sensitivity and wide applicability.
ENVIRONMENTAL CHEMISTRY LETTERS
(2021)
Article
Polymer Science
Joseph Merillyn Vonnie, Bong Jing Ting, Kobun Rovina, Kana Husna Erna, Wen Xia Ling Felicia, Nasir Md Nur 'Aqilah, Roswanira Abdul Wahab
Summary: This study developed a bio-film composed of Aloe vera, green banana, and curcumin for the detection of Fe2+ ions. The cross-linking interaction between banana starch-aloe vera gel and banana starch-curcumin enhanced the sensing performance of the composite film. The incorporation of aloe vera gel and curcumin particles onto the banana starch film successfully improved the film properties.
Editorial Material
Chemistry, Multidisciplinary
Leanne M. Gilbertson, Peter J. Vikesland
ENVIRONMENTAL SCIENCE-NANO
(2022)
Article
Microbiology
Dongjuan Dai, Connor Brown, Helmut Burgmann, D. G. Joakim Larsson, Indumathi Nambi, Tong Zhang, Carl-Fredrik Flach, Amy Pruden, Peter J. Vikesland
Summary: By using long-read sequencing, this study reveals that the activated sludge treatment in wastewater treatment plants acts as a barrier against the proliferation of most antibiotic resistance genes (ARGs), although some genes still persist or increase and require further attention.
Article
Nanoscience & Nanotechnology
Asifur Rahman, Seju Kang, Wei Wang, Qishen Huang, Inyoung Kim, Peter J. Vikesland
Summary: In this study, bacterial cellulose nanocrystals (BCNCs) modified with concanavalin A (con A) lectin and combined with gold nanoparticles (AuNPs) were used for label-free surface-enhanced Raman spectroscopy (SERS) detection of bacterial species. The detection assay showed high accuracy in differentiating bacterial strains using a support vector machine (SVM) classifier. The study demonstrates the potential of combining low-cost nanocellulose-based SERS biosensors with machine-learning techniques for the analysis of large spectral datasets.
ACS APPLIED NANO MATERIALS
(2022)
Review
Environmental Sciences
Asifur Rahman, Wei Wang, Divyapriya Govindaraj, Seju Kang, Peter J. Vikesland
Summary: Cellulose nanomaterials are advantageous due to their low cost, biocompatibility, and high stability and specific surface area. They can be combined with metal nanoparticles, organic polymers, and metal-organic frameworks to produce nanocomposites with various applications in environmental science and engineering.
CRITICAL REVIEWS IN ENVIRONMENTAL SCIENCE AND TECHNOLOGY
(2023)
Correction
Green & Sustainable Science & Technology
Shantanu V. Bhide, Stanley B. Grant, Emily A. Parker, Megan A. Rippy, Adil N. Godrej, Sujay Kaushal, Greg Prelewicz, Niffy Saji, Shannon Curtis, Peter Vikesland, Ayella Maile-Moskowitz, Marc Edwards, Kathryn G. Lopez, Thomas A. Birkland, Todd Schenk
NATURE SUSTAINABILITY
(2023)
Review
Chemistry, Multidisciplinary
Wei Wang, Seju Kang, Wei Zhou, Peter J. Vikesland
Summary: Many emerging infectious diseases are caused by viruses, which can be transmitted through various environmental matrices. The development of nanosensors based on unique properties of nanomaterials offers great potential for rapid and sensitive virus detection in the environment. These nanosensors can generate detectable signals through interactions between viruses and nanomaterials, providing fast response times, high sensitivity, and specificity.
ENVIRONMENTAL SCIENCE-NANO
(2023)
Article
Chemistry, Analytical
Wei Wang, Asifur Rahman, Seju Kang, Peter J. Vikesland
Summary: Label-free surface-enhanced Raman spectroscopy (SERS) is a promising technique for bacterial detection. This study evaluated the impact of storage conditions on label-free SERS spectra of Pseudomonas syringae samples stored in phosphate buffered saline. The results showed that storage conditions can significantly affect bacterial SERS signals and should be considered when detecting bacteria or evaluating bacterial response to stress stimuli.
ANALYTICAL CHEMISTRY
(2023)
Article
Microbiology
Andrea J. J. French, Alexandra K. K. Longest, Jin Pan, Peter J. J. Vikesland, Nisha K. K. Duggal, Linsey C. C. Marr, Seema S. S. Lakdawala
Summary: Efficient spread of respiratory viruses requires the virus to maintain infectivity in the environment. Our study measured the impact of initial droplet volume and relative humidity on the stability of influenza A virus, bacteriophage Phi6, and SARS-CoV-2. Virus decay rates differed between the wet and dry phases, and there were differences in virus decay characteristics by droplet size and virus. This study suggests that virus decay in media is related to droplet evaporation, which is controlled by relative humidity.
Article
Chemistry, Multidisciplinary
Aditya Garg, Wonil Nam, Wei Wang, Peter Vikesland, Wei Zhou
Summary: This study demonstrates the in situ spatiotemporal characterization and multivariate analysis of Pseudomonas syringae biofilms using surface-enhanced Raman spectroscopy (SERS) and nanolaminate plasmonic crystal SERS devices. The results show the potential of this method for monitoring the dynamic evolution of biofilms and their response to viral infection, offering insights for anti-biofilm therapy and viral detection.
Article
Engineering, Environmental
Wei Wang, Peter J. Vikesland
Summary: In this study, surface-enhanced Raman spectroscopy (SERS) was used to monitor the bioactive metabolites produced by ampicillin-resistant Pseudomonas aeruginosa strains and investigate the mechanisms underlying antibiotic resistance. The results showed that the blue-green pigment pyocyanin (PYO) dominated the metabolite signals and was significantly enhanced in the presence of subminimal inhibitory concentrations of ampicillin. The SERS spectra also revealed minimal impact on the production of intermediate substances and consistent nutrient consumption. Furthermore, exogenously added PYO enhanced the tolerance of ampicillin-susceptible Escherichia coli to some extent, indicating that PYO mediates antibiotic resistance in both the parent species and cocultured bacterial strains. The metabolic SERS signal provides new insights into antibiotic resistance and has promising applications in environmental monitoring and rapid clinical detection.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2023)
Editorial Material
Engineering, Environmental
Peter Vikesland
ACS ENVIRONMENTAL AU
(2023)
Article
Chemistry, Analytical
Wei Wang, Peter J. Vikesland
Summary: This study incorporates gold nanoparticles into a hydrogel ink for 3D printing and culturing of cells, enabling the use of surface-enhanced Raman spectroscopy (SERS) for cell imaging. A random forest binary classifier is developed to accurately distinguish cell signals from the background. The results show that SERS signals provide information about cellular components.
ANALYTICAL CHEMISTRY
(2023)
Article
Engineering, Environmental
Wei Wang, Peter J. Vikesland
Summary: This study demonstrates the use of surface-enhanced Raman spectroscopy (SERS) to monitor the metabolites produced by ampicillin-resistant Pseudomonas aeruginosa strains and identify the mechanisms underlying antibiotic resistance. The results indicate that the blue-green pigment pyocyanin (PYO) dominates the metabolite signals and is significantly enhanced by exposure to subminimal inhibitory concentrations of ampicillin. These findings provide new insights into antibiotic resistance.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2023)
Article
Chemistry, Multidisciplinary
Seju Kang, Wei Wang, Asifur Rahman, Wonil Nam, Wei Zhou, Peter J. Vikesland
Summary: In this study, highly porous gold supraparticles were fabricated and evaluated as SERS substrates for the sensitive detection of environmental contaminants. The porous Au supraparticles successfully adsorbed six environmental contaminants and demonstrated quantitative SERS detection capability. They also enabled multiplex SERS detection and maintained sensitivity in wastewater influent, showing potential as practical and sensitive SERS devices for environmental analysis applications.
Article
Chemistry, Multidisciplinary
Govindaraj Divyapriya, Asifur Rahman, Weinan Leng, Wei Wang, Peter J. Vikesland
Summary: This study introduces a facile one-step biosynthesis method for a bilayer structured hydrogel composed of reduced-graphene oxide (rGO) and bacterial nanocellulose (BNC) for various photothermal water treatment applications. The bilayer hydrogel was synthesized by modifying the BNC growth medium with an optimized concentration of corn steep liquor, which acted as a growth enhancer. The resulting rGO-BNC bilayer membrane showed comparable performance with ultrafiltration in terms of particle rejection and water flux, and also demonstrated efficient filtration, photothermal disinfection, and solar water evaporation.
ENVIRONMENTAL SCIENCE-NANO
(2022)