期刊
ORGANIC LETTERS
卷 20, 期 23, 页码 7470-7473出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b03247
关键词
-
资金
- National Natural Science Foundation of China [21232006, 21642002]
- Chinese Academy of Sciences
A Pd(OAc)(2)-catalyzed asymmetric cyclization of 2-aminoaryl alkynones involving an intramolecular trans-aminopalladation of alkyne and 1,2-addition to the carbonyl group tandem processes was developed. This strategy represents the first example using palladium as the catalyst and 2-alkynylaniline derivatives as the starting material to allow facile access to chiral 1,2,3,4-tetrahydro-beta-carbolines in high yields and excellent enantioselectivities.
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