期刊
ORGANIC LETTERS
卷 21, 期 1, 页码 70-74出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b03506
关键词
-
资金
- German Federal Environmental Foundation (DBU)
A general and selective metal-catalyzed conversion of biomass-derived primary diols and amines to the highly valuable 2,5-unsubstituted pyrroles has been developed. The reaction is catalyzed by a stable nonprecious manganese complex (1 mol %) in the absence of organic solvents whereby water and molecular hydrogen are the only side products. The manganese catalyst shows unprecedented selectivity, avoiding the formation of pyrrolidines, cyclic imides, and lactones.
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