期刊
ACS APPLIED MATERIALS & INTERFACES
卷 8, 期 23, 页码 14572-14577出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.6b03164
关键词
PEDOT:PSS; organic-silicon heterojunction solar cells; acid isotropic etching(AIE); PECVD; MoO3
资金
- National Natural Science Foundation of China [61504068]
- Science and Technology Program of Hebei Province [15214305D]
Poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) is widely applied in organic-photoelectronic devices due to its excellent transparency and conductivity. However, when it is used in the organic-silicon heterojunction solar cells with traditional pyramid texturing surface, the device performance is limited by the contact between the PEDOT:PSS and silicon wafer at the bottom of the pyramids. We optimized the structure of the bottom of the pyramids via acid isotropic etching (AIE) method with mixed acid solution to ensure that the silicon wafer is fully covered by the PEDOT:PSS. In addition, hydrogenated amorphous silicon thin films were deposited with PEVCD method as the passivation and back surface field (BSF) layer to decrease the rear surface recombination rate, thus increasing the long wavelength response. Finally, a power conversion efficiency of 13.78% was achieved after depositing MoO3 on the front of the device as the antireflection layer.
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