期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 140, 期 42, 页码 13580-13585出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.8b08781
关键词
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资金
- National Natural Science Foundation of China [21772121]
- Thousand Plan Youth program
- Shanghai Sailing Program [18YF1416900]
We describe a synergistic utilization of cerium photocatalysis and photoinduced electron transfer catalysis that enables an atom- and step-economical ring expansion of readily available cycloalkanols. This operationally simple protocol provides rapid access to privileged and synthetically challenging bridged lactones. The mild catalytic manifold has been adapted to continuous flow for scale-up applications and employed for the concise synthesis of polycyclic core of nepalactones.
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