期刊
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
卷 57, 期 48, 页码 16442-16450出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.iecr.8b03953
关键词
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资金
- National Natural Science Foundation of China [21676171, 51507107]
- Fork Ying Tong Education Foundation for Young Teachers in the Higher Education Institutions of China [61099]
- Science and Technology Fund for Distinguished Young Scholars of Sichuan Province [2016JQ0002]
- 1000 Talents Program of Sichuan Province
- Science Foundation for Distinguished Young Scholars of Sichuan University [2017SCU04A04]
Taking plant polyphenols as multifunctional platforms, we developed an environmentally friendly surface decoration strategy for preparing new types of three-dimensional (3D) superhydrophobic foams. The superhydrophobic foams were fabricated by in situ growth of beta-FeOOH nanoparticles on melamine foams that were pretreated by noncovalent surface decoration of plant polyphenol-glutaraldehyde cross-linkage, followed by the Michael addition of 1-dodecanethiol to plant polyphenols. The as-prepared superhydrophobic foams had water contact angles of 154.93 degrees and 153.12 degrees on the exterior and interior surfaces, respectively. The superhydrophobic foams featured a large absorption capacity, high mechanical robustness, structural stability, and flame resistance. During the 100 cycles of absorption and squeezing, the loss of absorption capacity was as low as 0.14% per cycle. In a continuous separation process, organic pollutants were successfully removed from water with a separation efficiency of 98.0%. Notably, the 3D superhydrophobic foams successfully separated six types of oil/water microemulsions, with a peak separation efficiency of 99.82%.
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