期刊
ACS APPLIED MATERIALS & INTERFACES
卷 10, 期 47, 页码 40702-40709出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.8b11836
关键词
tellurene; stability; Seebeck coefficient; strong anharmonicity; thermoelectric material
资金
- National Natural Science Foundation of China [11775159]
- Natural Science Foundation of Shanghai [18ZR1442800]
- National Youth 1000 Talents Program in China
- Opening Project of Shanghai Key Laboratory of Special Artificial Microstructure Materials and Technology
In 2016, bulk tellurium was experimentally observed as a remarkable thermoelectric material. Recently, two-dimensional (2D) tellurium, called tellurene, has been synthesized and has exhibited unexpected electronic properties compared with the 2D MoS2. They have also been fabricated into air-stable and highly efficient field-effect transistors. There are two stable 2D tellurene phases. One (beta-Te) has been confirmed with an ultralow lattice thermal conductivity (kappa(L)). However, the study of the transport properties of the other more stable phase, alpha-Te, is still lacking. Here, we report the thermoelectric performance and phonon properties of alpha-Te using Boltzmann transport theory and first-principles calculations. A maximum ZT value of 0.83 is achieved under a reasonable hole concentration, suggesting that the monolayer alpha-Te is a potential competitor in the thermoelectric field.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据