期刊
INORGANIC CHEMISTRY FRONTIERS
卷 5, 期 11, 页码 2739-2745出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8qi00637g
关键词
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资金
- National Natural Science Foundation of China [21671075, 21621001]
- 111 Project [B17020]
A new hybrid material, CNDs@ZIF-8, has been synthesized by the calcination of ZIF-8 nanocrystals. Carbon nanodots (CNDs) are produced from the decomposition of organic ligands such as 2-methylimidazole, which are embedded in the interrupted cavities in the framework during calcination. The resultant CNDs@ZIF-8 composites not only possess the intact structure of ZIF-8, but also have slightly enhanced adsorption ability and higher BET surface area compared to ZIF-8. Moreover, hybrid material CNDs@ZIF-8 exhibit tunable luminescence resulting from the inherent blue emission of ZIF-8 and the yellow emission of CNDs with different intensities controlled by the calcination time. The CNDs@ZIF-8 composites can also be used as temperature sensors. This work paves a feasible way for the development of CNDs@MOF materials with both luminescence and adsorption properties.
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