4.6 Article

A simple carbazole-N-benzimidazole bipolar host material for highly efficient blue and single layer white phosphorescent organic light-emitting diodes

期刊

JOURNAL OF MATERIALS CHEMISTRY C
卷 2, 期 14, 页码 2466-2469

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/c3tc32388a

关键词

-

资金

  1. NSFC/China [21161160442, 51203056]
  2. National Basic Research Program of China (973 Program) [2013CB922104]
  3. Ministry of Education of China [20100142120049]

向作者/读者索取更多资源

A new simple carbazole-N-benzimidazole bipolar luminogen mNBICz was constructed and utilized as a host for an FIrpic-doped blue device, and exhibited high efficiencies with a eta(EQE,max) of 26.2%, a eta(C,max) of 54.5 cd A(-1) and a eta(P,max) of 52.2 lm W-1. Furthermore, a two-color, all-phosphor single layer white device displayed a eta(EQE,max) of 22.9%, a eta(C,max) of 62.5 cd A(-1) and a eta(P,max) of 60.4 lm W-1.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.6
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Chemistry, Multidisciplinary

Efficient and Spectrally Stable Blue Perovskite Light-Emitting Diodes Based on Potassium Passivated Nanocrystals

Fei Yang, Hongting Chen, Rui Zhang, Xiaoke Liu, Weizhuo Zhang, JiBin Zhang, Feng Gao, Lei Wang

ADVANCED FUNCTIONAL MATERIALS (2020)

Article Materials Science, Multidisciplinary

Modifying the AIE-TADF chromophore with host-substituents to achieve high efficiency and low roll-off non-doped OLEDs

Panpan Leng, Shuaiqiang Sun, Runda Guo, Qing Zhang, Wei Liu, Xialei Lv, Shaofeng Ye, Lei Wang

ORGANIC ELECTRONICS (2020)

Article Materials Science, Multidisciplinary

High-Efficiency Formamidinium Lead Bromide Perovskite Nanocrystal-Based Light-Emitting Diodes Fabricated via a Surface Defect Self-Passivation Strategy

Hongting Chen, Lianwei Fan, Rui Zhang, Chunxiong Bao, Haifeng Zhao, Wei Xiang, Wei Liu, Guangda Niu, Runda Guo, Louwen Zhang, Lei Wang

ADVANCED OPTICAL MATERIALS (2020)

Article Engineering, Environmental

Asymmetric anthracene derivatives as multifunctional electronic materials for constructing simplified and efficient non-doped homogeneous deep blue fluorescent OLEDs

Shaofeng Ye, Yaxiong Wang, Runda Guo, Qing Zhang, Xialei Lv, Yalei Duan, Panpan Leng, Shuaiqiang Sun, Lei Wang

CHEMICAL ENGINEERING JOURNAL (2020)

Article Chemistry, Applied

Efficient deep-blue thermally activated delayed fluorescence emitters based on diphenylsulfone-derivative acceptor

Shuaiqiang Sun, Runda Guo, Qing Zhang, Xialei Lv, Panpan Leng, Yaxiong Wang, Zhi Huang, Lei Wang

DYES AND PIGMENTS (2020)

Article Materials Science, Multidisciplinary

Efficient CsPbBr 3 nanocrystals light emitting diodes achieved with Na plus modifying

Rui Zhang, Hongting Chen, Fei Yang, Weizhuo Zhang, Wei Xiang, Runda Guo, Lei Wang

ORGANIC ELECTRONICS (2020)

Article Engineering, Environmental

Regulating the photophysical properties of highly twisted TADF emitters by concurrent through-space/-bond charge transfer

Xialei Lv, Yaxiong Wang, Nengquan Li, Xiaosong Cao, Guohua Xie, Hong Huang, Cheng Zhong, Lei Wang, Chuluo Yang

CHEMICAL ENGINEERING JOURNAL (2020)

Article Chemistry, Applied

Donor engineering for diphenylsulfone derivatives with both thermally activated delayed fluorescence and aggregation-induced emission properties

Runda Guo, Panpan Leng, Qing Zhang, Yaxiong Wang, Xialei Lv, Shuaiqiang Sun, Shaofeng Ye, Yalei Duan, Lei Wang

Summary: This study presents the design and synthesis of two new AIE-TADF luminogens based on diphenylsulfone derivatives, with a focus on their fluorescence properties, performance, and applications in organic light-emitting diodes.

DYES AND PIGMENTS (2021)

Article Chemistry, Applied

Exploiting novel electron-deficient moiety 2,5-diazarcarbazole to functionally construct DPA-containing electron transporting materials for highly efficient sky-blue fluorescent OLEDs

Shaofeng Ye, Runda Guo, Yaxiong Wang, Yalei Duan, Lei Wang

Summary: The newly developed electron-deficient moiety 25NCz shows great potential for designing high-performance OLEDs' ETMs, offering possibilities in constructing organic electronic materials in the field of optoelectronics.

DYES AND PIGMENTS (2021)

Article Multidisciplinary Sciences

Exceptionally efficient deep blue anthracene-based luminogens: design, synthesis, photophysical, and electroluminescent mechanisms

Runda Guo, Wei Liu, Shian Ying, Yuwei Xu, Yating Wen, Yaxiong Wang, Dehua Hu, Xianfeng Qiao, Bing Yang, Dongge Ma, Lei Wang

Summary: This study reports the rational design and synthesis of two new deep blue luminogens, achieving high efficiency deep blue emissions in non-doped electroluminescent devices. The unprecedented electroluminescent efficiency is attributed to the combined effects of higher-order reversed intersystem crossing and triplet-triplet up-conversion. This research offers a new approach to resolve the shortage of high efficiency deep blue fluorescent emitters.

SCIENCE BULLETIN (2021)

Article Chemistry, Multidisciplinary

Synergistic Halide- and Ligand-Exchanges of All-Inorganic Perovskite Nanocrystals for Near-Unity and Spectrally Stable Red Emission

Kaiwang Chen, Dengliang Zhang, Qing Du, Wei Hong, Yue Liang, Xingxing Duan, Shangwei Feng, Linfeng Lan, Lei Wang, Jiangshan Chen, Dongge Ma

Summary: This study presents a method to prepare stable pure red emission and high-PLQY-mixed-halide perovskite nanocrystals through simultaneous halide-exchange and ligand-exchange. By introducing ZnI2 for anion exchange, CsPbBr3 nanocrystals can be transformed to CsPbBrxI3-x nanocrystals. The luminescence properties can be regulated by the ZnI2 exchange process, allowing the fabrication of red CsPbBrxI3-x nanocrystals with near-unity PLQY and a stable emission peak.

NANOMATERIALS (2023)

Review Chemistry, Multidisciplinary

High Triplet Energy Hosts for Blue Organic Light-Emitting Diodes

Yaxiong Wang, Ju Hui Yun, Lei Wang, Jun Yeob Lee

Summary: Improving the performance of blue OLEDs is a challenge in both scientific and industrial communities, with optimizing the fabrication process of devices, developing stable and efficient luminescence and transporting materials, and developing host materials with high triplet energy being key approaches. The bottleneck lies in improving operational lifetimes, decreasing efficiency roll-off, and maintaining high quantum efficiency, and more innovation is needed in this field.

ADVANCED FUNCTIONAL MATERIALS (2021)

Article Materials Science, Multidisciplinary

Molecular engineering of anthracene-based emitters for highly efficient nondoped deep-blue fluorescent OLEDs

Yaxiong Wang, Wei Liu, Shaofeng Ye, Qing Zhang, Yalei Duan, Runda Guo, Lei Wang

JOURNAL OF MATERIALS CHEMISTRY C (2020)

Article Chemistry, Inorganic & Nuclear

From a blue to white to yellow emitter: a hexanuclear copper iodide nanocluster

Ke Xu, Bu-Lin Chen, Rui Zhang, Li Liu, Xin-Xin Zhong, Lei Wang, Feng-Yan Li, Guang-Hua Li, Khalid A. Alamry, Fa-Bao Li, Wai-Yeung Wong, Hai-Mei Qin

DALTON TRANSACTIONS (2020)

Article Materials Science, Multidisciplinary

Phenothiazine dioxide-containing derivatives as efficient hosts for blue, green and yellow thermally activated delayed fluorescence OLEDs

Runda Guo, Yaxiong Wang, Zhi Huang, Qing Zhang, Songpo Xiang, Shaofeng Ye, Wei Liu, Lei Wang

JOURNAL OF MATERIALS CHEMISTRY C (2020)

Article Materials Science, Multidisciplinary

Translating efficient fluorescence into persistent room-temperature phosphorescence by doping bipolar fluorophores into polar polymer matrix

Mengjiao Dong, Liyun Liao, Chensheng Li, Yingxiao Mu, Yanping Huo, Zhong-Min Su, Fushun Liang

Summary: This study investigates the influence of the polarity of polymer matrices on persistent room-temperature phosphorescence (pRTP). It is discovered that intense phosphorescence emission can be achieved in highly polar matrices such as polyacrylic acid (PAA). The dipole-dipole interaction between the polar fluorophore and polar matrix is proposed to stabilize the excited state and facilitate the generation of efficient room-temperature phosphorescence emissions.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

High spatial resolution X-ray scintillators based on a 2D copper(i) iodide hybrid

Han-Jiang Yang, Weijia Xiang, Xiangzhou Zhang, Jin-Yun Wang, Liang-Jin Xu, Zhong-Ning Chen

Summary: This article reports a 2D copper(I)-based cluster material for X-ray imaging, which exhibits ultra-high spatial resolution, high photoluminescence efficiency, and low detection limit. The material shows excellent linear response to X-ray dose rates and light output, and has the best spatial resolution among reported lead-free metal halide hybrids.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Review Materials Science, Multidisciplinary

Interlayer and intermolecular excitons in various donor-acceptor heterostructures: applications to excitonic devices

Taek Joon Kim, Sang-hun Lee, Dayeong Kwon, Jinsoo Joo

Summary: Donor-acceptor heterostructures using organic-inorganic halide perovskites, two-dimensional transition metal dichalcogenides, pi-conjugated organic small/macro molecules, and quantum dots are promising platforms for exciton-based photonics and optoelectronics. Hetero-interlayer excitons and hetero-intermolecular excitons formed through optical and/or electrical charge transfer in various heterostructures are important quasi-particles for light emission, detection, and harvesting systems.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Designing CMOS compatible efficient ohmic contacts to WSi2N4 via surface-engineered Mo2B monolayer electrodes

Liemao Cao, Xiaohui Deng, Zhen-kun Tang, Rui Tan, Yee Sin Ang

Summary: We investigate the interface properties between WSi2N4 and Mo2B, O-modified Mo2B, and OH-modified Mo2B nanosheets. We find that WSi2N4 and Mo2B form n-type Schottky contacts, while functionalizing Mo2B with O and OH leads to the formation of both n-type and p-type ohmic contacts with WSi2N4. Additionally, we demonstrate the emergence of quasi-ohmic contact with ultralow lateral Schottky barrier and zero vertical interfacial tunneling barriers in Mo2B(OH)2-contacted WSi2N4.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Soft nanocomposites of lead bromide perovskite and polyurethane prepared via coordination chemistry for highly flexible, stable, and quaternary metal alloy-printed light emitting diodes

Ga Eun Kim, Hae-Jin Kim, Heesuk Jung, Minwoo Park

Summary: This study presents a solution to the commercialization challenges of flexible LEDs based on MAPbBr(3) by incorporating polyurethane and an In-Ga-Zn-Sn liquid alloy. The designed devices showed high flexibility, efficiency, and durability, with improved electron injection and reduced defects, making them promising for next-generation displays.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Elucidating the effects of the sidechain substitution direction on the optoelectronic properties of isomeric diketopyrrolopyrrole-based conjugated polymers for near-infrared organic phototransistors

Tao Shen, Zeng Wu, Zhen Jiang, Dongsheng Yan, Yan Zhao, Yang Wang, Yunqi Liu

Summary: Sidechain engineering is an important molecular design strategy for tuning the solid-state packing and structural ordering of conjugated polymers. The effects of sidechain direction on the optoelectronic properties of polymers and device performance were systematically investigated in this study. The results demonstrate that tuning the sidechain substitution direction can effectively improve the molecular structure and light absorption properties of polymers, providing new insights for the rational design of functional polymers.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Phase-engineering compact and flexible CsPbBr3 microcrystal films for robust X-ray detection

Lotte Clinckemalie, Bapi Pradhan, Roel Vanden Brande, Heng Zhang, Jonathan Vandenwijngaerden, Rafikul Ali Saha, Giacomo Romolini, Li Sun, Dirk Vandenbroucke, Mischa Bonn, Hai I. Wang, Elke Debroye

Summary: In this study, a facile strategy using a non-conductive polymer was proposed to fabricate stable, pinhole-free thick films. The effect of introducing a second phase into CsPbBr3 perovskite crystals on their photophysical properties and charge transport was investigated. The dual phase devices exhibited improved stability and more effective operation at higher voltages in X-ray detection.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Photoluminescence and structural phase transition relationship in Er-doped BaTiO3 model ferroelectric system

Jingye Zou, Shenglan Hao, Pascale Gemeiner, Nicolas Guiblin, Omar Ibder, Brahim Dkhil, Charles Paillard

Summary: When rare-earth ions are embedded in a ferroelectric material, their photoluminescence can serve as an all-optical probe for temperature, electric field, and mechanical stimulus. However, the impact of ferroelectric phase transitions on photoluminescence is not well understood. In this study, we demonstrate changes in the photoluminescence of green emission bands during critical ferroelectric transitions in an Er-doped BaTiO3 material. We also find that the intensity ratio and wavelength position difference of sub-peaks provide information on the phase transitions.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Resonant tunneling induced large magnetoresistance in vertical van der Waals magnetic tunneling junctions based on type-II spin-gapless semiconductor VSi2P4

Jiangchao Han, Daming Zhou, Wei Yang, Chen Lv, Xinhe Wang, Guodong Wei, Weisheng Zhao, Xiaoyang Lin, Shengbo Sang

Summary: Rare type-II spin-gapless semiconductors (SGSs) have attracted increasing attention due to their unique spin properties. In this study, the interface contacts and spin transport properties of different devices composed of VSi2P4 ferromagnetic layers were investigated. The results show that VSi2P4 is a promising material for designing vertical van der Waals heterostructures with a giant tunnel magnetoresistance (TMR) in spintronic applications.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Design of Cr-Ba-doped γ-Ga2O3 persistent luminescence nanoparticles for ratiometric temperature sensing and encryption information transfer

Tianqi Zhao, Renagul Abdurahman, Qianting Yang, Ruxiangul Aiwaili, Xue-Bo Yin

Summary: In this study, we designed and prepared Cr and Ba-doped gamma-Ga2O3 nanoparticles to achieve near-infrared emission and enhance the emission intensity. The emission mechanism was proposed based on the trap depth, band gap, and energy levels of Cr ions. The ratiometric temperature sensing and encryption information transfer demonstrated the potential applications of this technology.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Spin-gapless semiconducting characteristics and related band topology of quaternary Heusler alloy CoFeMnSn

Shuvankar Gupta, Jyotirmoy Sau, Manoranjan Kumar, Chandan Mazumdar

Summary: In this study, a new spin-gapless semiconductor material CoFeMnSn is reported, and its stable structure and spin-polarized band structure are determined through experimental realization and theoretical calculations. The compound exhibits a high ferromagnetic transition temperature, making it excellent for room temperature applications. The nearly temperature-independent resistivity, conductivity, and carrier concentration of the compound, adherence to the Slater-Pauling rule, and the high intrinsic anomalous Hall conductivity achieved through hole doping further confirm its spin-gapless semiconductor nature. Additionally, the compound's SGS and topological properties make it suitable for spintronics and magneto-electronics devices.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Two-dimensional metal-organic nanosheets composed of single-molecule magnets: structural modulation and enhanced magnetism utilizing the steric hindrance effect

Ikumi Aratani, Yoji Horii, Yoshinori Kotani, Hitoshi Osawa, Hajime Tanida, Toshiaki Ina, Takeshi Watanabe, Yohko F. Yano, Akane Mizoguchi, Daisuke Takajo, Takashi Kajiwara

Summary: In this study, two-dimensional arrays of single-molecule magnets (SMMs) based on metal-organic frameworks (MOFs) were systematically modified through Langmuir-Blodgett methods and chemical modifications. The introduction of bulky alkoxide groups induced structural changes and perpendicular magnetic anisotropy. This research provides a promising strategy for the construction of high-density magnetic memory devices using molecular spintronics.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Eulytite-type Ba3Yb(PO4)3:Tm/Er/Ho as a high sensitivity optical thermometer over a broad temperature range

Zonghao Lei, Houhe Dong, Lijie Sun, Bing Teng, Yanfei Zou, Degao Zhong

Summary: Researchers have successfully developed four different up-conversion phosphors based on the Eulytite-type host Ba3Yb(PO4)(3). The optical temperature sensing properties of these phosphors were thoroughly investigated, and it was found that Ba3Yb(PO4)(3):Tm/Er/Ho showed potential for optical temperature measurement applications.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Understanding trends in conductivity in four isostructural multifunctional crystals of Se substituted bis-dithiazolyl radicals

C. Roncero-Barrero, M. A. Carvajal, J. Ribas-Arino, I. de P. R. Moreira, M. Deumal

Summary: This study computationally investigates the conductivity of four isostructural compounds with different Se contents, and reveals the parameters that define their conductivity in stable organic radical materials. The results provide insights into the influence of Se content on the conductivity and highlight the importance of considering multiple parameters in understanding the trends in conductivity.

JOURNAL OF MATERIALS CHEMISTRY C (2024)

Article Materials Science, Multidisciplinary

Interplay between oxygen vacancies and cation ordering in the NiFe2O4 spinel ferrite

Remi Arras, Kedar Sharma, Lionel Calmels

Summary: In this study, we investigated the interplay between structural defects in NiFe2O4, showing that the complex formed by a Ni-Oh/Fe-Td-cation swap and a neutral oxygen vacancy is more stable than these two isolated defects, and significantly reduces the width of the minority-spin band gap.

JOURNAL OF MATERIALS CHEMISTRY C (2024)