4.6 Article

Enhanced thermoelectric figure of merit in p-type Bi0.48Sb1.52Te3 alloy with WSe2 addition

期刊

JOURNAL OF MATERIALS CHEMISTRY A
卷 2, 期 22, 页码 8512-8516

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ta01554a

关键词

-

资金

  1. NSFC [51201175]
  2. Zhejiang Provincial Public Welfare Technology Program [2012C21109]

向作者/读者索取更多资源

P-type Bi0.48Sb1.52Te3 alloys added with WSe2 were achieved via the zone melting method. The electrical performance was improved due to the increased carrier concentration, while the lattice thermal conductivity was simultaneously decreased, mainly due to the numerous types of nanoprecipitates produced, such as the second phase, antisite substitution and interfaces with different scales. As a result, a 23% improvement in the thermoelectric figure of merit zT was obtained with the addition of WSe2, making these composites more attractive for commercial applications.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.6
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Materials Science, Ceramics

A far-red-emitting (Gd,Y)3(Ga,Al)5O12:Mn2+ ceramic phosphor with enhanced thermal stability for plant cultivation

Xuting Qiu, Zhaohua Luo, Haochuan Jiang, Hui Ding, Zehua Liu, Xiaopu Chen, Jingtao Xu, Jun Jiang

JOURNAL OF THE AMERICAN CERAMIC SOCIETY (2020)

Article Engineering, Environmental

Effects of AgBiSe2 on thermoelectric properties of SnTe

Qiang Zhang, Zhe Guo, Xiaojian Tan, Lisha Mao, Yinong Yin, Yukun Xiao, Haoyang Hu, Chang Tan, Qingsong Wu, Guo-Qiang Liu, Jingtao Xu, Jun Jiang

CHEMICAL ENGINEERING JOURNAL (2020)

Article Chemistry, Physical

Improved thermoelectric performance in PbSe -AgSbSe2 by manipulating the spin-orbit coupling effects

Sichen Duan, Hongxiang Wang, Guo-Qiang Liu, Qingsong Wu, Na Man, Qiang Zhang, Xiaojian Tan, Yinong Yin, Yukun Xiao, Haoyang Hu, Jingtao Xu, Kai Guo, Xinxin Yang, Jun Jiang

NANO ENERGY (2020)

Article Chemistry, Physical

Synergistic optimization of electrical and thermal transport in n-type Bi-doped PbTe by introducing coherent nanophase Cu1.75Te

Chen Zhu, Jian Zhang, Hongwei Ming, Lulu Huang, Yuanyue Li, Tao Chen, Di Li, Baoli Zhang, Jingtao Xu, Xiaoying Qin

Summary: The study utilized Bi doping and Cu1.75Te nanophase to enhance the thermoelectric properties of PbTe materials, resulting in n-type PbTe materials with high ZT values at lower temperatures and maintaining high ZT values over a broad temperature range.

JOURNAL OF MATERIOMICS (2021)

Article Polymer Science

Borate functionalized caramel as effective intumescent flame retardant for wool fabric

Xian-Wei Cheng, Wen Zhang, Yan-Xiang Wu, Yi-Dan Ma, Jing-Tao Xu, Jin-Ping Guan

Summary: The study prepared borate functionalized caramel (BF-Car) product using glucose and synthesized ethanolamine borate ester, which was then applied as an effective intumescent flame retardant (FR) system for wool fabric. The treated wool fabric showed improved fire safety with reduced smoke and heat emission.

POLYMER DEGRADATION AND STABILITY (2021)

Article Thermodynamics

Improving cabin thermal environment of parked vehicles under direct sunlight using a daytime radiative cooling cover

Yinyan Lv, Anchong Huang, Jian Yang, Jingtao Xu, Ronggui Yang

Summary: This study introduces a new type of car cover named Cover R, which utilizes daytime radiative cooling effect to reduce interior temperature when parking outside, improving passenger comfort and saving energy consumption as well as reducing carbon dioxide emission.

APPLIED THERMAL ENGINEERING (2021)

Article Chemistry, Physical

Realizing high thermoelectric performance in n-type SnSe polycrystals via (Pb, Br) co-doping and multi-nanoprecipitates synergy

Wen-Hao Gu, Yi-Xin Zhang, Jun Guo, Jian-Feng Cai, Yu-Ke Zhu, Fengshan Zheng, Lei Jin, Jingtao Xu, Jing Feng, Zhen-Hua Ge

Summary: This study investigates the doping effect of PbBr2 on n-type polycrystalline SnSe, demonstrating that PbBr2 can significantly increase the carrier concentration and electrical conductivity, thereby improving the thermoelectric performance of polycrystalline SnSe.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

Article Nanoscience & Nanotechnology

Phase Tuning for Enhancing the Thermoelectric Performance of Solution-Synthesized Cu2-xS

Meiling Yang, Xiaofang Liu, Bin Zhang, Yao Chen, Hengyang Wang, Jian Yu, Guoyu Wang, Jingtao Xu, Xiaoyuan Zhou, Guang Han

Summary: A series of Cu2-xS materials were synthesized by changing the CuCl/Na2S molar ratio, leading to improvements in electrical properties with the 1.75:1 molar ratio sample achieving a good power factor at 815K.

ACS APPLIED MATERIALS & INTERFACES (2021)

Article Physics, Applied

Two conductive mechanisms in LaMnO3 thin film: Adiabatic and nonadiabatic small polaronic hopping

Weiyuan Wang, Jiyu Fan, Huan Zheng, Jing Wang, Hao Liu, Caixia Wang, Chunlan Ma, Langsheng Ling, Jingtao Xu, Hao Yang

Summary: The study focused on the structural, surface morphology, magnetic, and resistivity data of perovskite LaMnO3 epitaxial thin films. The films exhibited paramagnetic behavior and insulating electron transport in the studied temperature range, with charge carriers following different small polaronic hopping mechanisms in high and low temperature regions. These findings provide new insights for exploring abnormal ferromagnetism in LaMnO3 multilayer thin films.

MODERN PHYSICS LETTERS B (2021)

Article Thermodynamics

Energy saving potential of a fresh air pre-cooling system using radiative sky cooling

Dikai Xu, Sebastien Boncoeur, Gang Tan, Jingtao Xu, Hua Qian, Dongliang Zhao

Summary: A new fresh air pre-cooling system using radiative sky cooling technique is proposed to reduce the cooling load of fresh air. Simulation results show an annual cooling energy consumption reduction of around 10% in most cities, with even better performance in arid areas like Abu Dhabi with a 19.34% energy saving.

BUILDING SIMULATION (2022)

Article Multidisciplinary Sciences

Defect-induced ferromagnetism in a S=1/2 quasi-one-dimensional Heisenberg antiferromagnetic chain compound

Zhe Wang, Lin Hu, Langsheng Lin, Yuyan Han, Ning Hao, Jingtao Xu, Qianwang Chen, Zhe Qu

Summary: Research has shown that defects in the spin S=1/2 Heisenberg antiferromagnetic chain (HAFC) compound can lead to ferromagnetism, with the long-range ferromagnetic order in MACuF attributed to Cu2+ ions in 2D networks. This unusual ferromagnetism not only enriches magnetic features in low-dimensional systems, but also aids in understanding exotic magnetic phenomena in other quasi-1D magnetic materials.

SCIENTIFIC REPORTS (2021)

Article Materials Science, Multidisciplinary

Bilayer structured coating for radiative cooling applications

Rongbing Wan, Zhihao Ma, Weiping Xu, Wenbo Zhao, Jingtao Xu, Ronggui Yang

Summary: The technology utilizes high reflectance and high emissivity to achieve passive daytime sub-ambient radiative cooling with a bilayer coating, resulting in cooling objects without energy consumption. Experimental results show that the bilayer coating can lower temperatures to sub-ambient levels under solar irradiance, with a maintained lower temperature during the night.

JOURNAL OF PHOTONICS FOR ENERGY (2021)

Article Chemistry, Physical

Performance evaluation of radiative cooling for commercial-scale warehouse

Ningsheng Wang, Yinyan Lv, Dongliang Zhao, Wenbo Zhao, Jingtao Xu, Ronggui Yang

Summary: In this study, a scalable-manufactured radiative cooling metamaterial film was applied to the roof of a commercial warehouse, and its energy performance was evaluated using experimental measurements and a simulation model in different locations under hot climates. The results showed that the radiative cooling roof significantly reduced roof temperature, minimized thermal stratification and fluctuation, and greatly reduced air conditioning energy consumption.

MATERIALS TODAY ENERGY (2022)

Article Nanoscience & Nanotechnology

Colored radiative cooling coatings using phosphor dyes

J. Xu, R. Wan, W. Xu, Z. Ma, X. Cheng, R. Yang, X. Yin

Summary: This study demonstrates colored radiative cooling materials with highly selective dyes, which can cool objects under direct solar irradiance while maintaining high energy efficiency. The results show that these materials have both aesthetic appeal and efficient cooling performance.

MATERIALS TODAY NANO (2022)

Article Materials Science, Multidisciplinary

CaAlSiN3:Eu2+/Lu3Al5O12:Ce3+ phosphor-in-glass film with high luminous efficiency and CRI for laser diode lighting

Zehua Liu, Pan Hu, Hangjie Jiang, Peng Sun, Yongfu Liu, Zhaohua Luo, Jingtao Xu, Zhengren Huang, Jun Jiang

Summary: This study fabricated CASN phosphor-in-glass films using glass as an inorganic binder, achieving high efficiency and thermal stability. Introducing LuAG to offset the spectra of CASN PiFs, broad emission spectra and high efficiency were achieved. The high color quality LD white lighting produced by PiFs represents a significant advancement in the field.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

Article Chemistry, Physical

Enhanced moisture sorption through regulated MIL-101(Cr) synthesis and its integration onto heat exchangers

Mei Gui Vanessa Wee, Amutha Chinnappan, Runxin Shang, Poh Seng Lee, Seeram Ramakrishna

Summary: Cooling processes, from residences to industries, require a lot of energy and are essential. This study introduces MIL-101(Cr), a new desiccant, to heat exchangers for more efficient cooling. By improving the synthesis method and using a special binder, the MIL-101(Cr)-coated heat exchanger shows improved water uptake capacity and lower regeneration temperature.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Synthesis of completely solvent-free biomedical waterborne polyurethane with excellent mechanical property retention and satisfactory water absorption

Ao Zhen, Guanyu Zhang, Ao Wang, Feng Luo, Jiehua Li, Hong Tan, Zhen Li

Summary: In this study, a solvent-free microemulsion method was used to synthesize waterborne polyurethane (WPU) material with high retention of mechanical properties and satisfactory water absorption rates. The material showed excellent biocompatibility and has broad application potential in the field of biomedicine.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Review Chemistry, Physical

Recent progress in eutectic gallium indium (EGaIn): surface modification and applications

Wensong Ge, Rui Wang, Xiaoyang Zhu, Houchao Zhang, Luanfa Sun, Fei Wang, Hongke Li, Zhenghao Li, Xinyi Du, Huangyu Chen, Fan Zhang, Huifa Shi, Huiqiang Hu, Yongming Xi, Jiankang He, Liang Hu, Hongbo Lan

Summary: This paper reviews the research on the surface tension of eutectic gallium-indium alloys (EGaIn) in the field of stretchable electronics. It covers the principles of oxide layer formation, factors influencing surface tension, and methods for surface modification of liquid metals. The paper also discusses the applications of EGaIn surface modification in different fields and highlights the challenges still faced and the future outlook.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Review Chemistry, Physical

Nature-inspired sustainable solar evaporators for seawater desalination

Xiang Song, Lianghao Jia, Zhengen Wei, Tao Xiang, Shaobing Zhou

Summary: This paper provides an overview of the application, preparation, and role of biomimetic structures in solar evaporators with improved evaporation rate and lifetime.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Synergistic carrier and phonon transport advance Ag dynamically-doped n-type PbTe thermoelectrics via Mn alloying

Wei Yuan, Qian Deng, Dong Pan, Xiang An, Canyang Zhao, Wenjun Su, Zhengmin He, Qiang Sun, Ran Ang

Summary: Optimizing the performance of n-type PbTe thermoelectric materials is crucial for practical applications. Dynamic doping has emerged as an effective method to improve the performance of n-type PbTe by optimizing the carrier concentration. This study demonstrates the significance of Mn alloying in enhancing the performance of Ag-doped n-type PbTe by creating a hierarchical structure to suppress thermal transport and improving the Seebeck coefficient.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Review Chemistry, Physical

Recent advances of bifunctional electrocatalysts and electrolyzers for overall seawater splitting

Xiaoyan Wang, Meiqi Geng, Shengjun Sun, Qian Xiang, Shiyuan Dong, Kai Dong, Yongchao Yao, Yan Wang, Yingchun Yang, Yongsong Luo, Dongdong Zheng, Qian Liu, Jianming Hu, Qian Wu, Xuping Sun, Bo Tang

Summary: This review provides a comprehensive analysis of the progress and challenges in the field of bifunctional electrocatalysts and efficient electrolyzers for seawater splitting. It summarizes recent advancements and proposes future perspectives for highly efficient bifunctional electrocatalysts and electrolyzers.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Sequence-dependent self-assembly of supramolecular nanofibers in periodic dynamic block copolymers

Jason K. Phong, Christopher B. Cooper, Lukas Michalek, Yangju Lin, Yuya Nishio, Yuran Shi, Huaxin Gong, Julian A. Vigil, Jan Ilavsky, Ivan Kuzmenko, Zhenan Bao

Summary: Dynamic block copolymers (DBCPs) combine the phase separation of traditional block copolymers with the supramolecular self-assembly of periodic dynamic polymers, resulting in the spontaneous self-assembly of high aspect ratio nanofibers with well-ordered PEG and PDMS domains. DBCPs with a periodic block sequence exhibit superior properties compared to those with a random sequence, including delayed onset of terminal flow and higher ionic conductivity values.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Moisture-triggered proton conductivity switching in metal-organic frameworks: role of coordinating solvents

Hong Kyu Lee, Yasaswini Oruganti, Jonghyeon Lee, Seunghee Han, Jihan Kim, Dohyun Moon, Min Kim, Dae-Woon Lim, Hoi Ri Moon

Summary: This study reports the moisture-triggered proton-conductivity switching behavior in Zn5FDC MOFs induced by the presence and absence of coordinating solvents, which illustrates the significant role of coordinating solvents in conductivity variation.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Spiro[fluorene-9,9′-xanthene]-based hole shuttle materials for effective defect passivation in perovskite solar cells

Bommaramoni Yadagiri, Sanjay Sandhu, Ashok Kumar Kaliamurthy, Francis Kwaku Asiam, Jongdeok Park, Appiagyei Ewusi Mensah, Jae-Joon Lee

Summary: The molecular engineering of the interface modulator between the perovskite and hole transporting material is crucial for achieving satisfactory performance and stability of perovskite solar cells. In this study, cruciform-shaped dual functional organic materials were employed as surface passivation and hole transporting interfacial layers in perovskite solar cells. The use of these materials significantly improved the power conversion efficiency of the solar cells.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Crystalline phase transition in as-synthesized pure silica zeolite RTH containing tetra-alkyl phosphonium as organic structure directing agent

Joaquin Martinez-Ortigosa, Reisel Millan, Jorge Simancas, Manuel Hernandez-Rodriguez, J. Alejandro Vidal-Moya, Jose L. Jorda, Charlotte Martineau-Corcos, Vincent Sarou-Kanian, Mercedes Boronat, Teresa Blasco, Fernando Rey

Summary: This study investigates the synthesis of all-silica RTH zeolites using triisopropyl(methyl)phosphonium as the organic SDA. The results show the formation of two distinct crystalline phases under different synthesis conditions, with fluoride bonding to different silicon sites. It demonstrates the possibility of controlling the placement of fluoride in RTH zeolites through synthesis conditions.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Heterostructured MoP/CoMoP2 embedded in an N, P-doped carbon matrix as a highly efficient cooperative catalyst for pH-universal overall water splitting

Luyao Zheng, Cong Liu, Wenbiao Zhang, Boxu Gao, Tianlan Yan, Yahong Zhang, Xiaoming Cao, Qingsheng Gao, Yi Tang

Summary: This study successfully improves the efficiency and stability of water splitting by constructing a heterostructured electrocatalyst. The catalyst shows extraordinary performance and could offer an effective approach for the sustainable production of hydrogen.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Lanthanide contraction effect on the alkaline hydrogen evolution and oxidation reactions activity in platinum-rare earth nanoalloys

Carlos A. Campos-Roldan, Raphael Chattot, Frederic Pailloux, Andrea Zitolo, Jacques Roziere, Deborah J. Jones, Sara Cavaliere

Summary: This study systematically evaluated the hydrogen evolution/oxidation reactions on a series of Pt-rare earth nanoalloys in alkaline media, and identified the effect of the lanthanide contraction. The experimental results revealed that the chemical nature of the rare earth modulates the adsorption and mobility of oxygenated-species, enhancing the kinetics of the reactions.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Correlating the structural transformation and properties of ZIF-67 during pyrolysis, towards electrocatalytic oxygen evolution

Sara Frank, Mads Folkjaer, Mads L. N. Nielsen, Melissa J. Marks, Henrik S. Jeppesen, Marcel Ceccato, Simon J. L. Billinge, Jacopo Catalano, Nina Lock

Summary: This study investigates the thermal decomposition of ZIF-67 and its correlation with structural evolution and electrocatalytic performance. The researchers used in situ X-ray absorption spectroscopy and total scattering techniques to analyze the process. They found that disorder emerges at lower temperatures and that extending the pyrolysis process can result in materials with superior electrochemical properties.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

SiO2 assisted Cu0-Cu+-NH2 composite interfaces for efficient CO2 electroreduction to C2+ products

Zi-Yang Zhang, Hao Tian, Han Jiao, Xin Wang, Lei Bian, Yuan Liu, Nithima Khaorapapong, Yusuke Yamauchi, Zhong-Li Wang

Summary: By constructing Cu-0-Cu+-NH2 composite interfaces with the assistance of SiO2, the electrochemical CO2 reduction reaction (CO2RR) achieves high Faraday efficiency and current density for C2+ production, improving the productivity of carbon cycle.

JOURNAL OF MATERIALS CHEMISTRY A (2024)

Article Chemistry, Physical

Electrochemically exfoliated covalent organic frameworks for improved photocatalytic hydrogen evolution

Ting Wang, Ruijuan Zhang, Pengda Zhai, Mingjie Li, Xinying Liu, Chaoxu Li

Summary: This study successfully exfoliated COFs using a simple electrochemical method, which resulted in improved photocatalytic performance for COFs and enriched the fabrication approach of COF exfoliation.

JOURNAL OF MATERIALS CHEMISTRY A (2024)