期刊
JOURNAL OF MATERIALS CHEMISTRY A
卷 2, 期 27, 页码 10404-10409出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ta01261e
关键词
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资金
- Japan Science and Technology Agency PRESTO Program
- Japan Society for the Promotion of Science (JSPS)
- World Premier International Research Center Initiative (WPI), MEXT, Japan
- Grants-in-Aid for Scientific Research [26708006, 25620043, 25810047] Funding Source: KAKEN
We present a strategy for creating coordination frameworks exhibiting proton conduction with thermal stability. The coordination framework, where template cations link 1-D chains via hydrogen bonds, has dynamic hydrogen bond networks where protons move without water support. Solid-state NMR and X-ray studies visualized the proton hopping mechanism, and revealed that the templates provide the bridging of the 1-D chains to attain proton conduction. The templates also enable the proton conductive networks to be maintained at 190 degrees C through multiple interactions between the templates and the 1-D chains.
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