期刊
JOURNAL OF FLOW CHEMISTRY
卷 2, 期 1, 页码 24-27出版社
SPRINGER
DOI: 10.1556/jfchem.2012.00019
关键词
supercritical fluids; automation; self-optimising reactors; green chemistry; flow chemistry
资金
- European Community [NMP2-LA-2010-246461]
- National Research Foundation (NRF)
This paper describes the next stage in our development of self-optimising reactors. We demonstrate that the same reaction can be optimised for a series of different criteria including yield, space-time yield, E factor and a weighted yield function (the product of space-time yield and yield). In different experiments, we achieved 97.6% yield, space-time yield of 42.9 kg/L/h and E factors of 1.4 and 3.3 (including CO2) and the weighted yield, which gave a promising balance between yield, E factor and space-time yield.
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