期刊
ACS CATALYSIS
卷 2, 期 11, 页码 2242-2246出版社
AMER CHEMICAL SOC
DOI: 10.1021/cs300445y
关键词
palladium; alcohol; selective oxidation; XAS; kinetics
资金
- EPSRC [EP/E046754/1, EP/G007594/2]
- EPSRC [EP/E046754/1, EP/G007594/2] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/G007594/2, EP/E046754/1] Funding Source: researchfish
In-situ, synchronous MS/XANES reveals the Pd catalyzed selective aerobic oxidation of crotyl alcohol is regulated by the balance between the oxidation state and reducibility. Dynamic XANES measurements provide a new, rapid method to determine redox kinetics of nanoparticles and identify important parameters to optimize catalyst design.
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