4.8 Article

Creation of a two-dimensional electron gas at an oxide interface on silicon

期刊

NATURE COMMUNICATIONS
卷 1, 期 -, 页码 -

出版社

NATURE PORTFOLIO
DOI: 10.1038/ncomms1096

关键词

-

资金

  1. National Science Foundation [DMR-0906443, DMR-0704022]
  2. DARPA Seedling
  3. Fine Foundation
  4. DoE/BES [DE-FG02-07ER46416]
  5. Nanochip and David and Lucile Packard Fellowship
  6. US Department of Energy [DE-AC02-05CH11231]
  7. [DMR-0907191]
  8. Direct For Mathematical & Physical Scien [907191] Funding Source: National Science Foundation
  9. Direct For Mathematical & Physical Scien
  10. Division Of Materials Research [0906443] Funding Source: National Science Foundation
  11. Division Of Materials Research [907191] Funding Source: National Science Foundation
  12. Division Of Materials Research
  13. Direct For Mathematical & Physical Scien [GRANTS:13765097] Funding Source: National Science Foundation

向作者/读者索取更多资源

In recent years, reversible control over metal-insulator transition has been shown, at the nanoscale, in a two-dimensional electron gas (2DEG) formed at the interface between two complex oxides. These materials have thus been suggested as possible platforms for developing ultrahigh-density oxide nanoelectronics. A prerequisite for the development of these new technologies is the integration with existing semiconductor electronics platforms. Here, we demonstrate room-temperature conductivity switching of 2DEG nanowires formed at atomically sharp LaAlO3/SrTiO3 (LAO/STO) heterointerfaces grown directly on (001) Silicon (Si) substrates. The room-temperature electrical transport properties of LAO/STO heterointerfaces on Si are comparable with those formed from a SrTiO3 bulk single crystal. The ability to form reversible conducting nanostructures directly on Si wafers opens new opportunities to incorporate ultrahigh-density oxide nanoelectronic memory and logic elements into well-established Si-based platforms.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.8
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Oncology

Standard versus longer interval of radical resection after neoadjuvant chemoradiotherapy in locally advanced rectal cancer: A 20-year single-center experience & propensity-score matching

Saule Khamzina, Jongoh Lee, Seung-Bum Ryoo, Min Jung Kim, Ji Won Park, Hyun-Cheol Kang, Eui Kyu Chie, Dae-Won Lee, Sae-Won Han, Tae-You Kim, Seung-Yong Jeong, Kyu Joo Park

Summary: The interval between neoadjuvant chemoradiotherapy (nCRT) and surgery has been debated for its impact on oncological outcomes and postoperative complications. This study found that performing surgery >8 weeks after nCRT can increase tumor regression, but it does not significantly affect oncological outcomes and postoperative complications compared to surgery conducted at 6-8 weeks after nCRT.

JOURNAL OF SURGICAL ONCOLOGY (2023)

Article Physics, Multidisciplinary

Quantum coherence tomography of light-controlled superconductivity

L. Luo, M. Mootz, J. H. Kang, C. Huang, K. Eom, J. W. Lee, C. Vaswani, Y. G. Collantes, E. E. Hellstrom, I. E. Perakis, C. B. Eom, J. Wang

Summary: The coupling between superconductors and oscillation cycles of light pulses, known as lightwave engineering, remains poorly understood due to the lack of measurements of high-order correlation functions. This study reports the discovery of parametrically driven superconductivity in iron-based superconductors induced by light-induced order-parameter collective oscillations. By separating the terahertz-frequency multidimensional coherent spectra, we measured non-perturbative, high-order correlations and found that the breakdown of susceptibility perturbative expansion occurs in this parametric quantum matter.

NATURE PHYSICS (2023)

Article Surgery

Safety of early surgery after self-expandable metallic stenting for obstructive left-sided colorectal cancer

Jung Wook Suh, Heung-Kwon Oh, Jeehye Lee, In Jun Yang, Hong-min Ahn, Duck-Woo Kim, Sung-Bum Kang, Rumi Shin, Seung Chul Heo, Dong Woon Lee, Sung-Chan Park, Dae Kyung Sohn, Jae Hwan Oh, Min Jung Kim, Ji Won Park, Seung-Bum Ryoo, Seung-Yong Jeong, Kyu Joo Park, Seoul Colorectal Res Grp SECOG

Summary: In obstructive left-sided colorectal cancer, the time interval between self-expanding metallic stenting (SEMS) and radical surgery does not significantly impact short- and long-term outcomes.

SURGICAL ENDOSCOPY AND OTHER INTERVENTIONAL TECHNIQUES (2023)

Article Materials Science, Multidisciplinary

Study on a Mixed-Cation Halide Perovskite-Based Deep-Ultraviolet Photodetector

Ga In Choi, Chung Wung Bark, Hyung Wook Choi

Summary: The study focuses on the development of a mixed-cation halide perovskite-based photodetector for deep-UV sensing. By mixing different ions, the prepared perovskite exhibits high stability, excellent light absorption, and increased bandgaps. The FAPbCl3-MAPbCl3 perovskite shows high responsivity, detectivity, and external quantum efficiency, making it a promising material for sensitive photodetection.

COATINGS (2023)

Article Chemistry, Multidisciplinary

Selective NOx- Electroreduction to Ammonia on Isolated Ru Sites

Zunjian Ke, Dong He, Xingxu Yan, Wenhui Hu, Nicholas Williams, Hongxing Kang, Xiaoqing Pan, Jier Huang, Jing Gu, Xiangheng Xiao

Summary: Nitrate and nitrite are common contaminants in industrial wastewater and groundwater. The electroreduction of NOx- to produce ammonia presents a sustainable alternative to the energy-intensive Haber-Bosch process. However, the development of selective catalysts that can regulate the reaction pathway and suppress competing reactions is still lacking.

ACS NANO (2023)

Article Chemistry, Multidisciplinary

Steering Bidirectional Sulfur Redox via Geometric/Electronic Mediator Comodulation for Li-S Batteries

Yifan Ding, Zixiong Shi, Yingjie Sun, Jianghua Wu, Xiaoqing Pan, Jingyu Sun

Summary: A generic and simple material strategy has been presented to fabricate advanced mediator for improved sulfur electrochemistry. The Li-S cells derived from this strategy exhibit impressive cyclic performances and durable areal capacity, indicating the potential for rationalizing the design and modulation of reliable polysulfide mediators in Li-S batteries.

ACS NANO (2023)

Article Chemistry, Analytical

Two-Dimensional Fe-N-C Single-Atomic-Site Catalysts with Boosted Peroxidase-Like Activity for a Sensitive Immunoassay

Zhaoyuan Lyu, Shichao Ding, Lingzhe Fang, Xin Li, Tao Li, Mingjie Xu, Xiaoqing Pan, Wenlei Zhu, Yang Zhou, Dan Du, Yuehe Lin

Summary: In this study, a two-dimensional Fe-N-C-based single-atomic-site catalyst (2D Fe-SASC) with excellent peroxidase-like activity was successfully synthesized and used to design ELISA for herbicide detection. The 2D structure of Fe-SASC exposes numerous single atomic active sites on the surface, enhancing the sensing performance. The assembled 2D Fe-SASC into a competitive ELISA kit achieved excellent detection performance for 2,4-dichlorophenoxyacetic acid (2,4-D). Fe-SASC shows great potential to replace expensive natural enzymes and work on various advanced sensing platforms for the detection of different target biomarkers.

ANALYTICAL CHEMISTRY (2023)

Article Chemistry, Multidisciplinary

Dislocation-Assisted Quasi-Two-Dimensional Semiconducting Nanochannels Embedded in Perovskite Thin Films

Huaixun Huyan, Zhe Wang, Linze Li, Xingxu Yan, Yi Zhang, Colin Heikes, Darrell G. Schlom, Ruqian Wu, Xiaoqing Pan

Summary: Defect engineering in perovskite thin films has received extensive attention due to their atomic-level modification and the design of novel nanostructures. However, three-dimensional defect-assisted nanostructures in thin film matrices usually have large misfit strains and unstable structures. In contrast, one- or two-dimensional defect-assisted nanostructures embedded in thin films can sustain large misfit strains without relaxation, making them suitable for defect engineering in perovskite thin films.

NANO LETTERS (2023)

Article Materials Science, Multidisciplinary

In-Situ Piezoelectric Effect for Augmenting Performance of Self-Powered ZnO-Based Photodetector

Thi My Huyen Nguyen, Chung Wung Bark

Summary: In this study, a self-powered ultraviolet photodetector based on a p-n junction of ZnO@Polyvinylidene fluoride (PVDF) and poly [9,9-dioctylfluorene-co-N-[4-(3-methylpropyl)]-diphenylamine] (TFB) was developed by integrating an in-situ piezoelectric effect into the photoactive region. The fabricated ZnO@fiPVDF nanocomposite with strong piezoelectricity exhibited improved on/off ratio, detectivity, and response speed under 365-nm UV illumination. The device also showed stable operation over 1000 continuous on/off cycles and long-lasting photostability when exposed to UV light.

COATINGS (2023)

Review Chemistry, Physical

Recent Advances of Doped SnO2 as Electron Transport Layer for High-Performance Perovskite Solar Cells

Vo Pham Hoang Huy, Thi My Huyen Nguyen, Chung Wung Bark

Summary: This review provides comprehensive insights into the factors that influence the performance of the electron transport layer (ETL) SnO2 in perovskite solar cells (PSCs). The potential for doping is evaluated, aiming to achieve better results in PSCs and promote further development of SnO2-based PSCs.

MATERIALS (2023)

Article Materials Science, Multidisciplinary

Optoelectronic Properties of Ferroelectric Composites of Bi3.25La0.75Ti3O12 (BLT) and Co-Doped BLT Thin Films Modified by FeCo-Doped BLT

Rui Tang, Rui He, Sangmo Kim, Chung Wung Bark

Summary: Driven by the demand for renewable and clean energy, this study investigated the photovoltaic effect of various solar cells and materials. By modifying the BLT and Co-BLT composites with FeCo-BLT films, the bandgap was narrowed and visible light absorption was increased, resulting in improved photovoltaic power generation performance. The modified double-ferroelectric, thin-film composites showed superior optoelectronic properties and enhanced current density, indicating improved efficiency of ferroelectric thin-film photovoltaic reactions.

COATINGS (2023)

Article Chemistry, Multidisciplinary

Toward Industrial Production of a High-Performance Self-Powered Ultraviolet Photodetector Using Nanoporous Al-Doped ZnO Thin Films

Manh Hoang Tran, Thi My Huyen Nguyen, Chung Wung Bark

Summary: Al-doped ZnO (AZO) thin films are effective n-type semiconductors for UV detection. However, finding a balance between performance and fabrication ease remains a challenge for practical AZO-based UV photodetectors. In this study, a strategy is proposed to achieve a large photoactive area for outstanding performance using a facile sol-gel method.

ACS OMEGA (2023)

Article Chemistry, Multidisciplinary

How Pt Influences H-2 Reactions on High Surface-Area Pt/CeO2 Powder Catalyst Surfaces

Jaeha Lee, Peter Tieu, Jordan Finzel, Wenjie Zang, Xingxu Yan, George Graham, Xiaoqing Pan, Phillip Christopher

Summary: The addition of platinum-group metals (PGMs, e.g., Pt) to CeO2 promotes the rate of redox surface reactions in heterogeneous catalysis. However, the mechanistic picture of PGM-promoted H-2 reactions on CeO2 surfaces in powder catalysts remains unclear. This study investigates the influence of Pt nanoclusters and single atoms on H-2 reactions on Pt/CeO2 powder catalysts using controlled catalyst synthesis and various experimental techniques. The results show that Pt can promote H-2 consumption rates even when existing on a small fraction of CeO2 particles, and Pt changes the activation mechanism and rate limiting step for H-2 on CeO2 surfaces.

JACS AU (2023)

Article Engineering, Electrical & Electronic

Growth of Low-defect Si-Doped Ga2O3 Film on Fluorine-doped Tin Oxide Substrate for Self-powered and High-performance Ultraviolet Photodetector

Thi My Huyen Nguyen, Manh Hoang Tran, Chung Wung Bark

Summary: In this study, an efficient ultraviolet photodetector (UV PD) is prepared based on a p-n junction that is metal-electrode-free and with a vertical configuration. The device exhibits high responsivity, a good on/off ratio, and fast response speed, with improved performance under reverse bias.

ACS APPLIED ELECTRONIC MATERIALS (2023)

Review Physics, Applied

Probing charge density in materials with atomic resolution in real space

Christopher Addiego, Wenpei Gao, Huaixun Huyan, Xiaoqing Pan

Summary: This article discusses the developments in high-resolution real-space charge distribution imaging using diffraction techniques and electron microscopy, focusing on the recent advancement of four-dimensional scanning transmission electron microscopy, electron holography, and applications to materials interfaces.

NATURE REVIEWS PHYSICS (2023)

暂无数据