期刊
CHEMICAL SCIENCE
卷 4, 期 6, 页码 2665-2669出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3sc50630d
关键词
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资金
- National Natural Science Foundation of China [20625205, 20772034, 20932002]
- National Basic Research Program of China (973 Program) [2011CB808600]
- Doctoral Fund of Ministry of Education of China [20090172110014]
- Guangdong Natural Science Foundation [10351064101000000]
Versatile directed aromatic C-H bond activation and oxidative coupling with allylic alcohols is reported using a cationic Rh(III) catalyst. This method provides efficient and robust synthesis of functional beta-aryl ketones and indolines in good yields with excellent regioselectivity, even the reaction runs at 3 g scale. The catalytic systems have good functional group tolerance, such as CONR2, NHAc, NO2, CF3, CN, Cl, Br and I.
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