期刊
ULTRASONICS SONOCHEMISTRY
卷 21, 期 2, 页码 535-541出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.ultsonch.2013.09.002
关键词
Mass transfer coefficient; Numerical simulation; Ultrasonic enhancement; Liquid-solid reaction
资金
- Project developing key scientific instrument and equipment of China [2011YQ120023]
Mass transfer coefficient is an important parameter in the process of mass transfer. It can reflect the degree of enhancement of mass transfer process in liquid-solid reaction and in non-reactive systems like dissolution and leaching, and further verify the issues by experiments in the reaction process. In the present paper, a new computational model quantitatively solving ultrasonic enhancement on mass transfer coefficient in liquid-solid reaction is established, and the mass transfer coefficient on silicon surface with a transducer at frequencies of 40 kHz, 60 kHz, 80 kHz and 100 kHz has been numerically simulated. The simulation results indicate that mass transfer coefficient increases with the increasing of ultrasound power, and the maximum value of mass transfer coefficient is 1.467 x 10(-4) m/s at 60 kHz and the minimum is 1.310 x 10(-4) m/s at 80 kHz in the condition when ultrasound power is 50 W (the mass transfer coefficient is 2.384 x 10(-5) m/s without ultrasound). The extrinsic factors such as temperature and transducer diameter and distance between reactor and ultrasound source also influence the mass transfer coefficient on silicon surface. Mass transfer coefficient increases with the increasing temperature, with the decreasing distance between silicon and central position, with the decreasing of transducer diameter, and with the decreasing of distance between reactor and ultrasound source at the same ultrasonic power and frequency. The simulation results indicate that the computational model can quantitatively solve the ultrasonic enhancement on mass transfer coefficient. (C) 2013 Elsevier B.V. All rights reserved.
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