4.7 Article

Degradation of reactive brilliant red in aqueous solution by ultrasonic cavitation

期刊

ULTRASONICS SONOCHEMISTRY
卷 15, 期 1, 页码 43-48

出版社

ELSEVIER
DOI: 10.1016/j.ultsonch.2007.01.008

关键词

degradation; reactive brilliant red K-BP; cavitation; sonochemistry

向作者/读者索取更多资源

Degradation of reactive brilliant red K-BP in aqueous solution by means of ultrasonic cavitation was investigated for a variety of operating conditions. It is found that the degradation of reactive brilliant red K-BP in aqueous solution follows pseudo-first-order reaction kinetics and the degradation rate is dependent on the initial concentration of reactive brilliant red K-BP, the temperature and acidity of the aqueous medium. The effects of Fe2+, Fenton reagent and NaCl addition on the sonochemical degradation of reactive brilliant red K-BP were also investigated. The results obtained here indicate that the degradation rate of brilliant red K-BP in aqueous solution was substantially accelerated by Fe2+, NaCl or Fenton reagent addition. (c) 2007 Elsevier B.V. All rights reserved.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.7
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Materials Science, Multidisciplinary

Fabrication of porous cellulose microspheres with controllable structures by microfluidic and flash freezing method

Mengjie Zhang, Weilin Guo, Meng Ren, Xiaohua Ren

MATERIALS LETTERS (2020)

Article Environmental Sciences

Enhanced catalytic activity of MIL-101(Fe) with coordinatively unsaturated sites for activating persulfate to degrade organic pollutants

Huaisu Guo, Shengnan Su, Yang Liu, Xiaohua Ren, Weilin Guo

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2020)

Article Engineering, Chemical

Morphology and crystal facet-dependent activation mechanism of persulfate by V2O5 nanomaterials for organic pollutants degradation

Xiaohua Ren, Yang Liu, Weilin Guo

SEPARATION AND PURIFICATION TECHNOLOGY (2020)

Article Engineering, Chemical

Facet-controlled activation of persulfate by magnetite nanoparticles for the degradation of tetracycline

Leixin Hu, Xiaohua Ren, Min Yang, Weilin Guo

Summary: The study investigated the catalytic performance of three types of magnetite nanoparticles with different exposed crystal facets for tetracycline degradation. The results showed that MNPs with {111} facet exhibited superior catalytic activity compared to {1 1 0} and {1 0 0} facets. The catalytic performance was determined by hydroxide, physically adsorbed H2O, and transformations of Fe(II)/Fe(III) on the MNPs{111} surface, with XPS analysis supporting the findings.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

Article Engineering, Environmental

Facet-controlled activation of persulfate by goethite for tetracycline degradation in aqueous solution

Min Yang, Xiaohua Ren, Leixin Hu, Weilin Guo, Jinhua Zhan

Summary: This study utilized goethite with different exposed facets as catalysts for PS activation, finding that more {021} facet exposed goethite exhibited better catalytic performance due to its facilitation of generating active radicals to drive the degradation process. Advanced oxidation processes based on the activation of persulfate by facet-dependent goethite provide valuable insights for environmental catalysis.

CHEMICAL ENGINEERING JOURNAL (2021)

Article Environmental Sciences

Persulfate activation by ferrocene-based metal-organic framework microspheres for efficient oxidation of orange acid 7

Xiaoyu Lv, Yanqiu Leng, Rongyao Wang, Yan Wei, Xiaohua Ren, Weilin Guo

Summary: In this study, ferrocene-based metal-organic frameworks with different transition metals were synthesized and used as catalysts for persulfate activation. The effects of catalyst dosage, persulfate concentration, and pH on the degradation of acid orange 7 were investigated. The results showed that cobalt-based ferrocenyl metal-organic framework microspheres exhibited the best catalytic performance.

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2022)

Article Engineering, Chemical

Polyoxometalate intercalated La-doped NiFe-LDH for efficient removal of tetracycline via peroxymonosulfate activation

Rongyao Wang, Shengnan Su, Xiaohua Ren, Weilin Guo

Summary: A novel NiFeLa{HPW}-LDH catalyst was synthesized and exhibited superior catalytic performance for PMS activation compared with the precursor. The degradation process was mainly driven by SO4· and HO· as reactive radicals, with the formation of Ni(II)/Fe(II)/La(III) complexes and subsequent redox cycles of Ni/Fe/La playing vital roles in generating active radicals. The intercalated HPW also played a significant role in electron transfer during the process.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

Article Engineering, Environmental

Peroxydisulfate activation by LaNiO3 nanoparticles with different morphologies for the degradation of organic pollutants

Yan Wei, Yanqiu Leng, Rongyao Wang, Xiaohua Ren, Weilin Guo

Summary: A series of LaNiO3 perovskite nanoparticles with different morphologies were prepared and used as catalysts for peroxydisulfate activation. Spheres-like LaNiO3 exhibited the highest catalytic activity, likely due to its largest specific surface area, higher proportion of reductive Ni2+, and higher electron transfer ability. Radical scavenging experiments and EPR revealed the production of sulfate radicals and hydroxyl radicals during the oxidation process, and possible mechanisms of PDS activation and AO7 degradation were proposed. The prepared LaNiO3 perovskites also showed excellent reusability and stability.

WATER SCIENCE AND TECHNOLOGY (2022)

Article Environmental Sciences

Elucidating the origin mechanism of a morphology-dependent layered double hydroxide catalyst toward organic contaminant oxidation via persulfate activation

Rongyao Wang, Yanjun Yu, Ruijuan Zhang, Xiaohua Ren, Weilin Guo

Summary: Understanding the morphology-dependence of NiFe-LDH catalysts on their catalytic activity is important for the rational design of high-efficiency catalysts. In this study, three different NiFe-LDH catalysts with regulable oxygen vacancies were synthesized and their abilities to activate persulfate for the degradation of acid orange 7 were investigated. The results showed that the NiFe-LDH catalyst with a hollow structure exhibited the highest activity, attributed to the highly accessible surface areas, higher intrinsic activity of the exposed crystal planes, and abundant oxygen vacancies.

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2022)

Article Engineering, Environmental

Enhanced electro-Fenton degradation of tetracycline in aqueous solution using a self-supported BiOCl/CF cathode

Jiangshan Kuai, Xiusen Geng, Xiaohua Ren, Weilin Guo

Summary: In this study, a self-standing cathode material was prepared by in situ growing bismuth oxychloride on carbon felt, and it was used for the electro-Fenton degradation of tetracycline. The hybrid electrode exhibited excellent conductivity and abundant active sites, leading to the almost complete degradation of tetracycline within 90 minutes.

WATER SCIENCE AND TECHNOLOGY (2022)

Article Environmental Sciences

Controllable synthesis of FeMn bimetallic ferrocene-based metal-organic frameworks to boost the catalytic efficiency for removal of organic pollutants

Chengjie Qu, Xiaoyu Lv, Rongyao Wang, Ruijuan Zhang, Weilin Guo

Summary: A series of FeMn bimetallic ferrocene-based metal-organic frameworks were synthesized and Fe4Mn6-Fc-MOFs demonstrated superior catalytic activity and electron transfer capability, showing great potential for water decontamination.

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2023)

Article Engineering, Environmental

Synthesis of a layered double hydroxide-based hybrid electrode for efficient removal of phosphate ions in capacitive deionization

Xiusen Geng, Jiangshan Kuai, Xiaohua Ren, Weilin Guo

Summary: In this study, hybrid electrodes composed of nickel-iron layered double hydroxide anchored on activated carbon fiber were synthesized and applied in capacitive deionization for phosphate ions removal. The adsorption performance of the hybrid electrodes was compared, and it was found that increasing the loading capacity of nickel-iron layered double hydroxide enhanced the adsorption capacity. The adsorption kinetics and isotherms analysis showed that the adsorption capacity increased with applied voltage and followed pseudo-first-order kinetics and Langmuir isotherms. The pH during the adsorption process also affected the adsorption of phosphate ions.

WATER SCIENCE AND TECHNOLOGY (2022)

Article Engineering, Environmental

Characteristics, source apportionment and health risk assessment of perfluoroalkyl acids in typical drinking water sources of eastern China

Hong Liu, Ruibao Jia, Zhenqi Du, Xiaodong Xin, Mingquan Wang, Shaohua Sun, Weilin Guo, Xiang Li, Li Liu

Summary: This study provides detailed information on the characteristics, source apportionment, and health risk assessment of perfluoroalkyl acids (PFAAs) in surface drinking water in Shandong Province, eastern China. The study identifies PFOA as the dominant pollutant and determines different sources of contamination during wet and dry seasons. Although the health risks through drinking water exposure are negligible for different age groups, children aged 3-6 years are most vulnerable. The findings of this study are important for decision-makers to monitor and mitigate PFAA pollution.

ENVIRONMENTAL SCIENCE-WATER RESEARCH & TECHNOLOGY (2023)

Article Green & Sustainable Science & Technology

CeO2@LDH decorated 3D porous module with mortise-tenon structure: Activation of peroxymonosulfate for ultrafast removal of tetracycline

Rongyao Wang, Xiaohua Ren, Weilin Guo

Summary: This study presents a robust catalytic module for industrial water treatment, which features lower energy consumption, fast liquid transport, and simultaneous highly catalytic oxidizability. The module consists of cerium oxide loaded layered double hydroxide composites anchored on a three-dimensional porous polyvinylidene fluoride framework. It exhibits dual functions of filtration and oxidation, showing promising removal efficiency for tetracycline in conjunction with peroxymonosulfate. The module is highly efficient in removing various contaminants and has wide practical applicability in tap water and reservoir.

JOURNAL OF CLEANER PRODUCTION (2023)

Article Environmental Sciences

Insights into the facet-dependent adsorption of antibiotic ciprofloxacin on goethite

Min Yang, Xiaohua Ren, Leixin Hu, Haihong Zhou, Weilin Guo

Summary: Goethite is the most common iron oxide mineral in soils, and the adsorption of organic pollutants on goethite has a significant impact on their fate and transport in the environment. This study found that goethite samples with a higher proportion of {021}/{110} facets exhibited better adsorption capacity due to the presence of more reactive singly coordinated sites on the {021} facet. Additionally, the adsorption of CIP on {021} and {110} facets was shown to involve the formation of a tridentate complex through bridge coordination, H-bonding, and bidentate chelate complex formation.

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2021)

暂无数据