期刊
TETRAHEDRON LETTERS
卷 54, 期 22, 页码 2858-2860出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2013.03.097
关键词
Total synthesis; Lycopladine A; Lycopodium alkaloids
资金
- National Natural Science of China [20802084, 21072200]
- National Basic Research Program of China (973 Program) [2009Cb522300]
- Chinese Academy of Sciences
Asymmetric total synthesis of (+)-lycopladine A (1) has been achieved. Key elements of the synthesis include an efficient Helquist annulation to assemble the cis-fused 6/5 bicycle, Stille coupling reaction to elongate the allylic side chain, and Krohnke pyridine synthesis to set the pyridine core at the final stage. (C) 2013 Elsevier Ltd. All rights reserved.
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