期刊
SYNLETT
卷 -, 期 16, 页码 2565-2582出版社
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0029-1217747
关键词
alkenes; transition-metal catalysis; carbon-carbon bond formation; carbonyl-ene reactions; addition reactions
资金
- National Institute of General Medical Sciences [GM-063775, GM-072566]
- NSF [CHE-0134704, CHE-9809061, DBI-9729592]
- Amgen
- Boehringer Ingelheim
- Bristol Myers-Squibb
- Merck Research Laboratories
- GlaxoSmithKline
- Johnson Johnson
- Pfizer
- Sloan Foundation
- Wyeth
- Deshpande Center (MIT)
- The Chinese University of Hong Kong [2060323, 1902031]
- The Center of Novel Functional Molecules
- Croucher Foundation
- NIH [1S10RR13886-01]
Recent advances using nickel complexes in the activation of unactivated monosubstituted olefins for catalytic intermolecular carbon-carbon bond-forming reactions with carbonyl compounds, such as simple aldehydes, isocyanates, and conjugated aldehydes and ketones, are discussed. In these reactions, the olefins function as vinyl- and allylmetal equivalents, providing a new strategy for organic synthesis. Current limitations and the outlook for this new strategy are also discussed.
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