期刊
SCIENTIFIC REPORTS
卷 5, 期 -, 页码 -出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/srep16947
关键词
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资金
- NSFC [21003021, 21373051, U1305242]
- program for New Century Excellent Talents in Fujian Province University [JA14029]
- program for Qishan Scholar of Fuzhou University
- Collaborative Innovation Center of Clean Coal Gasification Technology [XK1401]
- National Natural Fund of Science Department of Fujian Province [2015J01601]
Herein, we reported a octahedral Cd-3(C3N3S3)(2) coordination polymer as a new noble metal-free photocatalyst for robust photocatalytic H2O2 production from methanol/water solution. The coordination polymer can give an unprecedented H2O2 yield of ca. 110.0 mmol center dot L-1 center dot g(-1) at pH = 2.8 under visible light illumination. The characterization results clearly revealed that the photocatalytic H2O2 production proceeds by a pathway of two-electron reduction of O-2 on the catalyst surface. This work showed the potential perspective of M-x(C3N3S3)(y) (M =transitional metals) coordination polymers as a series of new materials for solar energy storage and conversion.
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