Article
Physics, Multidisciplinary
A. F. Fang, R. Zhou, H. Tukada, J. Yang, Z. Deng, X. C. Wang, C. Q. Jin, Guo-Qing Zheng
Summary: This study investigates the superconducting properties of LiFeP and LiFeAs through nuclear magnetic resonance (NMR) studies, revealing differences in their superconducting behaviors. The saturation of λ(L) in LiFeAs indicates nodeless superconducting gaps, while the absence of saturation in LiFeP suggests the presence of nodes in the superconducting gap function. Strong spin fluctuations with diffusive characteristics are also observed in LiFeP, similar to some cuprate high temperature superconductors.
Article
Multidisciplinary Sciences
Peng Fan, Fazhi Yang, Guojian Qian, Hui Chen, Yu-Yang Zhang, Geng Li, Zihao Huang, Yuqing Xing, Lingyuan Kong, Wenyao Liu, Kun Jiang, Chengmin Shen, Shixuan Du, John Schneeloch, Ruidan Zhong, Genda Gu, Ziqiang Wang, Hong Ding, Hong-Jun Gao
Summary: The authors report evidence of hybridization between field-induced and magnetic adatom-induced Majorana modes in an iron-based superconductor FeTe0.55Se0.45, providing a possible single-material platform for braiding Majorana modes.
NATURE COMMUNICATIONS
(2021)
Article
Chemistry, Physical
Chi Ho Wong, Rolf Lortz
Summary: In this study, we computed the superconducting transition temperature (Tc) of iron-based superconductors using two existing models and tested their validity for predicting the Tc of FeSe monolayers. Our results show that the model, which takes into account the amplifying effect of antiferromagnetism and electron-phonon coupling, agrees well with experimental data. Furthermore, we found that interfacial effects may contribute to the observed Tc enhancement in FeSe monolayers.
Article
Multidisciplinary Sciences
Lu Cao, Wenyao Liu, Geng Li, Guangyang Dai, Qi Zheng, Yuxin Wang, Kun Jiang, Shiyu Zhu, Li Huang, Lingyuan Kong, Fazhi Yang, Xiancheng Wang, Wu Zhou, Xiao Lin, Jiangping Hu, Changqing Jin, Hong Ding, Hong-Jun Gao
Summary: The evolution of superconductivity in LiFeAs with respect to pressure or strain is still unclear, but this study found that different orientations of local wrinkles on the surface have varying effects on the superconducting states, suggesting that directional pressure may play an important role in iron-based superconductivity.
NATURE COMMUNICATIONS
(2021)
Article
Nanoscience & Nanotechnology
Mantao Huang, Muhammad Usama Hasan, Konstantin Klyukin, Delin Zhang, Deyuan Lyu, Pierluigi Gargiani, Manuel Valvidares, Sara Sheffels, Alexandra Churikova, Felix Buettner, Jonas Zehner, Lucas Caretta, Ki-Young Lee, Joonyeon Chang, Jian-Ping Wang, Karin Leistner, Bilge Yildiz, Geoffrey S. D. Beach
Summary: Voltage control of magnetic order is essential for energy-efficient spintronic applications, and solid-state hydrogen gating allows for reversible ferrimagnetic order control, external-field-free 180 degrees magnetic switching, and ferrimagnetic spin texture manipulation. In this study, the use of electric field-induced hydrogen loading/unloading in GdCo shifts the magnetic compensation temperature and enables control of the dominant magnetic sublattice. Additionally, the weakening of antiferromagnetic exchange coupling results in reversible gate voltage-induced net magnetization switching and generation of ferrimagnetic spin textures.
NATURE NANOTECHNOLOGY
(2021)
Review
Physics, Condensed Matter
Ya-Bin Liu, Yi Liu, Guang-Han Cao
Summary: This paper discusses the coexistence and interaction between superconductivity and ferromagnetism in iron-based materials. Through the study of doped iron pnictides and iron-based superconductors, a new material basis has been discovered. These materials exhibit both superconductivity and ferromagnetism at specific temperatures, which is of great significance for understanding the correlation between superconductivity and ferromagnetism.
JOURNAL OF PHYSICS-CONDENSED MATTER
(2022)
Article
Chemistry, Physical
Yi-Na Huang, Xiang-Long Yu, Da-Yong Liu, Miao-Miao Han
Summary: The study shows that CaAFe(4)As(4) can achieve a superconducting transition temperature of 31-36 K without doping. The introduced alkali metals can induce hole doping and chemical pressure effects, which can affect the superconducting transition temperature by changing the number of electrons and the structure of the FeAs conductive layer.
Article
Physics, Applied
Hangwei Ding, Hang Zhao, Pengcheng Huang, Lei Yu, Jianyuan Xu, Zhen Fang, Zhiyou Chen, Dongliang Wang, Xianping Zhang, Wenge Chen, Yanwei Ma
Summary: For the first time, this study combines iron-based superconductors with high field insert coil technology to generate a higher magnetic field. Through the fabrication and evaluation of large-sized iron-based superconducting double pancake coils, a superior performing insert coil is formed and tested under different background fields. The test results show that the insert coil successfully generates high magnetic fields under different background fields, surpassing previous performance tests.
SUPERCONDUCTOR SCIENCE & TECHNOLOGY
(2023)
Article
Physics, Multidisciplinary
Dongfei Wang, Jens Wiebe, Ruidan Zhong, Genda Gu, Roland Wiesendanger
Summary: Spin-resolved spectroscopic studies revealed the Yu-Shiba-Rusinov (YSR) bound states on the surface of the topological superconductor FeTe0.55Se0.45 induced by Fe atoms. Zero-energy bound states were observed for some of the adsorbed Fe atoms, with the absence of spin signature indicating the lack of Majorana bound states associated with Fe adatoms on FeTe0.55Se0.45.
PHYSICAL REVIEW LETTERS
(2021)
Article
Materials Science, Multidisciplinary
Xiangwei Huang, Chunyu Guo, Carsten Putzke, Martin Gutierrez-Amigo, Yan Sun, Maia G. Vergniory, Ion Errea, Dong Chen, Claudia Felser, Philip J. W. Moll
Summary: The cascade of electronic phases in CsV3Sb5 provides an opportunity to study the mutual interactions in a clean, strongly interacting kagome lattice. CsV3Sb5 is a three-dimensional metal in the charge density wave state and exhibits anomalous magnetoresistance at low temperatures.
Article
Physics, Multidisciplinary
Peng-Tao Yang, Qing-Xin Dong, Peng-Fei Shan, Zi-Yi Liu, Jian-Ping Sun, Zhi-Ling Dun, Yoshiya Uwatoko, Gen-Fu Chen, Bo-Sen Wang, Jin-Guang Cheng
Summary: We report the discovery of superconductivity on the border of antiferromagnetic order in a quasi-one-dimensional material RbMn6Bi5 under high pressures. The phase diagram of the material shows similarities to many magnetism-mediated superconductors. The study found that with increasing pressure, the antiferromagnetic ordering transition is enhanced and then suppressed, leading to the emergence of superconductivity with a relatively high critical temperature.
CHINESE PHYSICS LETTERS
(2022)
Article
Physics, Multidisciplinary
Tao Xie, Chang Liu, Tom Fennell, Uwe Stuhr, Shi-Liang Li, Hui-Qian Luo
Summary: An investigation on the spin resonance mode in optimally hole-doped iron-based superconductor Ba0.67K0.33Fe2As2 revealed a unique energy dispersion phenomenon, suggesting that the spin resonance may not be restricted by the superconducting gaps in multi-band systems. This breaks through the conventional understanding and poses new challenges in the study of superconductivity in iron-based materials.
Article
Chemistry, Multidisciplinary
Giang D. Nguyen, Mingming Fu, Qiang Zou, Liurukara D. Sanjeewa, An-Ping Li, Athena S. Sefat, Zheng Gai
Summary: The study reveals localized superconducting states in a calcium-iron-based superconductor using low-temperature scanning tunneling microscopy and spectroscopy. The competition between local strain of praseodymium dopants and defect-induced local magnetic moments affects the superconductivity. These superconducting states exist at the nanoscale near the praseodymium dopants and are not influenced by surface reconstruction or defects.
Article
Multidisciplinary Sciences
Chuang Li, Xun-Jiang Luo, Li Chen, Dong E. Liu, Fu-Chun Zhang, Xin Liu
Summary: In this study, an iron-based superconducting nanowire system is proposed as a platform to manipulate Majorana zero modes (MZMs) and reveal their non-Abelian braiding statistics in a broad topological nontrivial parameter space.
NATIONAL SCIENCE REVIEW
(2022)
Article
Chemistry, Multidisciplinary
Jessie Manopo, Tio Prince Lubis, Muhammad Arief Mustajab Enha Maryono, Pepen Arifin, Toto Winata, Rena Widita, Yudi Darma
Summary: We studied the electronic, magnetic, and optical properties of (LaO1-xFx)MnAs systems with different doping levels of F. The properties of the system, such as bandgap and magnetism, were found to change significantly with F doping. This research highlights the potential of F doping for advanced device applications.
Article
Chemistry, Physical
D. Liang, Y. B. Yang, W. Y. Yang, C. Y. Zhu, J. L. Zhu, H. Xu, S. C. Vogel, O. Gourdon, R. Q. Zou, G. Tian, C. S. Wang, H. L. Du, J. B. Yang
Summary: This study investigated the structural and magnetic properties of MnxSb compounds, showing that magnetic properties can be tuned by controlling the concentration of Mn and doping at interstitial sites. By doping nonmagnetic elements into Mn1.12Zr0.1Sb compound, a significant room-temperature magnetocaloric effect without magnetic hysteresis was achieved, which is beneficial for practical magnetic refrigeration applications.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Chemistry, Multidisciplinary
Xin Huang, Jinlong Zhu, Binghui Ge, Frauke Gerdes, Christian Klinke, Zhongwu Wang
Summary: This study investigates the crystallization and growth of anisotropic nanocrystals into distinct superlattices in real time, providing kinetic details and designer parameters for the scale-up fabrication of functional materials. By studying the assembly of octahedral PbS NC blocks, the researchers found that NCs preferentially self-assembled into an orientation-disordered face-centered cubic superlattice, which later transformed into a body-centered cubic superlattice with single NC-orientational ordering across individual domains. Such insights and defined parameters allowed for the scalable fabrication of large/single bcc supercrystals with coherent ordering of NC translation and atomic plane orientation.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2021)
Article
Multidisciplinary Sciences
Jianfa Zhao, Jiacheng Gao, Wenmin Li, Yuting Qian, Xudong Shen, Xiao Wang, Xi Shen, Zhiwei Hu, Cheng Dong, Qingzhen Huang, Lipeng Cao, Zhi Li, Jun Zhang, Chongwen Ren, Lei Duan, Qingqing Liu, Richeng Yu, Yang Ren, Shih-Chang Weng, Hong-Ji Lin, Chien-Te Chen, Liu-Hao Tjeng, Youwen Long, Zheng Deng, Jinlong Zhu, Xiancheng Wang, Hongming Weng, Runze Yu, Martha Greenblatt, Changqing Jin
Summary: The A-site-ordered perovskite PbHg3Ti4O12 is the only known quadruple perovskite that undergoes a phase transition from a high-temperature centrosymmetric paraelectric phase to a low-temperature non-centrosymmetric ferroelectric phase under high pressure synthesis. It bridges the gap between simple ABO(3) perovskites and A-site-ordered AA'3Ti4O12 perovskites, exhibiting both displacive ferroelectricity and unique structural coordination.
NATURE COMMUNICATIONS
(2021)
Article
Chemistry, Physical
Yun Li, Songbai Han, Baifa Zhang, Hui Tang, Jun Han, Hongwei Kang, Yusheng Zhao, Jinlong Zhu
Summary: The nucleation and dissociation of CO2 hydrate in the inter- and intra-particle pores of dioctahedral smectite particles are affected by the layer charge distribution and type of exchangeable cations in the smectite, altering the structural ordering of water molecules. CO2 diffusion into intra-particle pores enhances the formation of clathrate-like structures but does not increase the structural ordering of water molecules. Increasing temperature or adding electrolytes accelerates CO2 hydrate dissociation in smectite particles.
APPLIED CLAY SCIENCE
(2022)
Article
Chemistry, Physical
Chenkai Li, Yaoyao Liu, Qishuo Yang, Qunfei Zheng, Zhipeng Yan, Jun Han, Junhao Lin, Shanmin Wang, Jingbo Qi, Ying Liu, Jinlong Zhu
Summary: Researchers have shown great interest in two-dimensional crystals due to their thickness-dependent electronic and optical properties. By investigating the Raman and photoluminescence spectra of free-standing monolayer and bilayer MoS2, it was found that electronic and crystal phase transitions occur at around 6 GPa and 16 GPa in bilayer MoS2, but not in the monolayer. These pressure-induced features provide insights into the importance of interlayer interactions in modifying the optical properties of MoS2 and other 2D materials.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2022)
Article
Chemistry, Multidisciplinary
Xu Zheng, Dayu Yan, Changjiang Yi, Jinlong Zhu, Qinghua Zhang, Junyi Zhai, Teng Ma, Pinwen Zhu, Hui Li, Lin Gu, Yusheng Zhao, Yugui Yao, Youguo Shi, Xiaohui Yu, Changqing Jin
Summary: Al2.69B50 is a superhard p-type semiconductor with high hardness, optical transmittance, and photon emission intensity, as well as excellent thermal and chemical stability and ultra-low density, suitable for high power electronic design and applications.
MATERIALS HORIZONS
(2022)
Article
Chemistry, Multidisciplinary
Meiling Jin, Peng Yu, Changzeng Fan, Qiang Li, Panlong Kong, Zhiwei Shen, Xiaomei Qin, Zhenhua Chi, Changqing Jin, Guangtong Liu, Guyue Zhong, Gang Xu, Zheng Liu, Jinlong Zhu
Summary: The study reported a pressure-induced phase transition and a dome-shaped superconducting phase in van der Waals layered NbIrTe4, with the highest critical temperature observed at approximately 5.8 K under a pressure of about 16 GPa. Anisotropic transport near the superconducting state was also observed, possibly due to the spatial modulation of interlayer Josephson coupling.
Article
Chemistry, Multidisciplinary
Pengcheng Yu, Yu Ye, Jinlong Zhu, Wei Xia, Yusheng Zhao
Summary: Solid-state lithium metal batteries offer high energy density and enhanced safety, but face challenges with interfaces. An in situ welding strategy has been developed to address interface issues and improve battery performance and cycling endurance.
FRONTIERS IN CHEMISTRY
(2021)
Article
Chemistry, Physical
Pei Wang, Sheng-Cai Zhu, Yongtao Zou, Haiyan Chen, Ying Liu, Weiwei Li, Jian Chen, Jinlong Zhu, Liusuo Wu, Shanmin Wang, Wenge Yang, Yuming Xiao, Paul Chow, Liping Wang, Yusheng Zhao
Summary: Cooperative Jahn-Teller (JT) distortion, combined with electromagnetic lattice coupling, plays a crucial role in numerous phenomena in materials science. While JT distortion is common in high-spin 3d4 and 3d9 configurations in octahedral complexes, large distortions resulting from the degeneracy lifting of t2g orbitals have rarely been observed. In this study, we report the discovery of pressure-induced cooperative JT effect in MnTe, which is accompanied by a significant volume collapse and a collapse of magnetic moment. First-principles calculations suggest that the lifting of t2g orbital degeneracy in Mn2+(d5) due to weakened p-d hybridization and enhanced d state localization induces the cooperative JT effect and triggers electromagnetic lattice coupling. These findings present a new mechanism for cooperative JT distortion via pressure-induced ligand distortion in antiferromagnetic materials.
CHEMISTRY OF MATERIALS
(2022)
Article
Chemistry, Physical
Lei Duan, XianCheng Wang, Jun Zhang, JianFa Zhao, Zhiwei Zhao, Changjiang Xiao, Chunlong Guan, Shun Wang, Liping Shi, Jinlong Zhu, ChangQing Jin
Summary: In this work, the critical properties of the ferromagnetic metal La3CrAs5 are reported. The isothermal magnetization curves are analyzed using various methods, and a set of precise and self-consistent critical exponents are obtained. The long-range magnetic coupling and the magnetic critical behavior in La3CrAs5 are discussed. The results provide insights into the magnetic properties and exchange mechanisms in this material.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Chemistry, Multidisciplinary
Yun Li, Meng Chen, Hui Tang, Songbai Han, Hongzhe Song, Pengfei Wang, Yusheng Zhao, Jinlong Zhu
Summary: CO2 hydrate nucleation on the surfaces of clay minerals is important for CO2 storage in marine sediments. This study used molecular dynamics simulations to investigate the heterogeneous nucleation of CO2 hydrates on different clay mineral surfaces. The results showed that the surface groups of clay minerals significantly affect CO2 hydrate nucleation and consequently CO2 storage in deposits.
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2022)
Article
Chemistry, Multidisciplinary
Qiang Li, Jian Zhang, Qunfei Zheng, Wenyu Guo, Jiangming Cao, Meiling Jin, Xingyu Zhang, Nana Li, Yanhui Wu, Xiang Ye, Pingping Chen, Jinlong Zhu, Tao Wang, Wangzhou Shi, Feifei Wang, Wenge Yang, Xiaomei Qin
Summary: This study reports the discovery of richer transport properties, including abnormal properties and superconductivity, in high-pressure HgTe crystals. By pressure-tuning, a series of high-pressure phases were observed in a 400 nm thick crystal, and superconductivity emerged after the semiconductor-to-metal transition. Density functional theory calculations confirmed the contribution of surface-dominated topological band structure to these properties.
Article
Materials Science, Multidisciplinary
Cheng Jin, Yonggang Wang, Meiling Jin, Zimin Jiang, Dequan Jiang, Junlong Li, Yuki Nakamoto, Katsuya Shimizu, Jinlong Zhu
Summary: In this study, the structural and electrical property changes of Cu2IrO3 under different pressures were investigated at low temperatures. It was found that Cu2IrO3 undergoes dimerization at a certain pressure and experiences an insulator-metal transition at -13.8 GPa. Additionally, a strange crossover in the magnetoresistance of Cu2IrO3 was observed within a specific pressure range.
Article
Chemistry, Multidisciplinary
Jun Han, Jieshun Cui, Qunfei Zheng, Zhipeng Yan, Yun Li, Jian Chen, Xiaodong Yao, Guangyang Dai, Shanmin Wang, Ying Liu, Hsing-Lin Wang, Yusheng Zhao, Jinlong Zhu
Summary: Organic solar cells are a promising development direction due to their low cost, light weight, and flexibility. However, their power conversion efficiency is limited by the difficulty in regulating the size of their bandgap. In this study, a new organic molecule TPEPA was synthesized and its luminescence performance and polymerization under high pressure were investigated. The results showed that the TPEPA molecule underwent amorphization and polymerization under high pressure, leading to a reduced bandgap within the optimal range for solar cell materials. These findings provide a potential method for large-scale synthesis of novel organic solar cell materials.
Article
Chemistry, Physical
Xiaohong Yuan, Yong Cheng, Hu Tang, Pei Wang, Fuyang Liu, Songbai Han, Jinlong Zhu, Ming-Sheng Wang, Liping Wang
Summary: The pressure-induced sp(2)-to-sp(3) transitions in graphite have been extensively studied, and it has been found that the use of a specific pressure-transmitting medium can lower the transition pressure and reveal unique structural features.
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
(2022)