期刊
RSC ADVANCES
卷 5, 期 58, 页码 46455-46463出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ra05804j
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资金
- National Natural Science Foundation of China (NSFC) [21173064, 51203037, 21472031]
- Fundamental Research Funds for the Central Universities [GK201501005]
- Zhejiang Provincial Natural Science Foundation of China [LR14B030001]
It was found for the first time that cinchonine-and BINOL-derived multifunctional ligands bearing a siliconbased bulky group exhibited promising enantioselective control in the ruthenium-catalysed carbenoid N-H insertion reaction, in which the Ru-L26 system with multiple stereogenic centers was proved to be an enzyme-like catalyst because it exhibited a narrow substrate scope and size-sensitive discrimination in this reaction.
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