Article
Engineering, Chemical
Qingjun Du, Peng Zhou, Yuping Pan, Xiao Qu, Lu Liu, Hui Yu, Jian Hou
Summary: Hydrophobicity and roughness of solid surfaces play crucial roles in determining wetting and flow behavior. Increasing roughness can enhance apparent hydrophilicity in some cases, while it may improve apparent hydrophobicity in others. Beyond the superhydrophobic boundary, the effect of roughness on apparent hydrophobicity weakens or disappears.
CHEMICAL ENGINEERING SCIENCE
(2022)
Article
Construction & Building Technology
Jiayun Xu, Biao Ma, Shulin Zhou, Weijie Mao, Xiaoqing Wang
Summary: Based on the Wenzel model and Cassie model, this paper established a new wetting model for irregular rough surfaces and calculated the wetting depth and apparent contact angle. The experimental results showed significant differences in the surface texture parameters of different aggregates. The relative error between the predicted and measured contact angles was less than 15%, indicating excellent prediction effect. The wetting model analysis revealed that the surface tension of the test liquid, lithology of the solid aggregate, surface roughness, and texture structure are important control parameters affecting wetting.
CONSTRUCTION AND BUILDING MATERIALS
(2023)
Article
Chemistry, Physical
P. Xu, J. R. Bai, P. Zhou, L. L. Wang, X. N. Sun, L. Wei, Q. F. Zhou
Summary: A physical model was proposed to investigate the wettability of various microtextured surfaces, particularly superhydrophobicity. It was found that the sidewall angle restricted the contact angle of the microstructures, and re-entrant structures played a crucial role in the transition from hydrophilicity to superhydrophobicity.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2022)
Article
Engineering, Chemical
Fanny Thomas, Didier Dalmazzone, Jeffrey F. Morris
Summary: The wetting characteristics of ice-like clathrate hydrates at atmospheric pressure were studied using a new experimental method to measure the contact angle of various liquids. The results showed that the hydrate surface is water-wetting.
CHEMICAL ENGINEERING SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Matti J. Hokkanen, Matilda Backholm, Maja Vuckovac, Quan Zhou, Robin H. A. Ras
Summary: Superhydrophobic coatings with unique properties such as self-cleaning and staying dry have recently emerged in industrial and consumer markets. The stochastic nature of coating components can affect the uniformity of water repellency, and traditional contact angle goniometry may not provide accurate quantification of wetting properties. The study demonstrates that highly sensitive force-based methods can offer advantages in quantifying microscale heterogeneity in superhydrophobic coatings.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Li Cheng, Bei Fan, Zichen Zhang, Aaron McLeod, Wade Shipley, Prabhakar Bandaru
Summary: A new plasma processing-based methodology has been proposed to enhance the streaming potential (Vs) in electrokinetic flows over a silicon surface-based microchannel. The relationship between Vs, surface zeta potential, and electrolyte slip length was carefully determined through experiments. The study found that while the zeta potential always increases, the slip length may decrease under certain conditions. A record value of 0.1 mV/Pa was achieved using CF4 plasma.
Review
Chemistry, Multidisciplinary
Yasmin A. Mehanna, Emma Sadler, Rebekah L. Upton, Andrew G. Kempchinsky, Yao Lu, Colin R. Crick
Summary: Although superhydrophobic materials have garnered significant attention in scientific literature, their commercial development has been limited due to various factors such as material compatibility, physical resilience, and the stability of air layers in contact with water. Research efforts are focused on monitoring and improving air layer stability in order to overcome challenges in real-world applications.
CHEMICAL SOCIETY REVIEWS
(2021)
Article
Chemistry, Physical
G. C. Savulescu, M. Rucker, A. Scanziani, R. Pini, A. Georgiadis, P. F. Luckham
Summary: This study investigates the potential of using atomic force microscopy to characterize wetting behavior at the nanoscale, successfully observing an attraction phenomenon on the water droplet surface in experiments and obtaining parameters such as contact angle and contact angle distribution.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2021)
Article
Metallurgy & Metallurgical Engineering
Ai Chun-ming, Sun Ping-ping, Wu Ai-xiang, Chen Xun, Liu Chao
Summary: This study investigates the potential effect of surfactant on improving the surface wettability of copper ore through experimental and numerical analysis. The results show that the concentration of surfactant and sulfuric acid solution play a significant role in enhancing the wettability of the ore. Liquid surface tension and ore surface roughness are identified as the key factors affecting the surface wettability.
JOURNAL OF CENTRAL SOUTH UNIVERSITY
(2022)
Article
Chemistry, Physical
Yangyang Wu, Konstantinos Lazaridis, Mikhail D. Krivilyov, Sinisa Dj. Mesarovic, Dusan P. Sekulic
Summary: Understanding the effect of gravity on the capillary flow of molten metal is crucial for repair and construction in space through brazing. Our experiments demonstrate the formation of a secondary liquid flux meniscus in contact between liquid Al-Si and an alumina substrate. The equilibrium contact angle is close to 180 degrees, while the apparent contact angle depends on the brazing liquid mass. Additionally, the surface profile of the molten braze alloy on inclined AA3003 changes from a non-symmetric shape to a more symmetric shape as the inclination angle decreases.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2023)
Article
Mechanics
Hanyi Liu, Jun Zhang, Paolo Capobianchi, Matthew K. Borg, Yonghao Zhang, Dongsheng Wen
Summary: This study presents a multiscale simulation strategy that enhances VOF simulations by utilizing self-consistent boundary conditions derived from MD, enabling dynamic wetting simulations at both the nanoscale and macroscale. The new boundary conditions provide improved consistency in predicting dynamic wetting of nanodroplets and outperform other VOF models.
Article
Chemistry, Multidisciplinary
Daniel J. Braconnier, Terence Davidovits, Randall M. Erb
Summary: Superhydrophobic coatings are often fragile and easily lose their properties when subjected to droplet impact. This paper systematically studies ten different self-similar superhydrophobic coating approaches to understand why some coatings are more robust against hydrodynamic wear. The study finds that coatings with robust apolar chemistry, hierarchal topography, and slow loss of sacrificial material are more resilient against rapid droplet impacts. A quantitative approach to hydrodynamic wear of self-similar superhydrophobic coatings is proposed.
Article
Physics, Fluids & Plasmas
Yechan Noh, N. R. Aluru
Summary: This study reports the influence of atomic-scale vibrational coupling at the solid-fluid interface on interfacial properties such as wettability and fluid slip. Molecular dynamics simulation reveals that the contact angle increases and solid-fluid adsorption weakens when the oscillation frequency of the substrate matches the bending frequency of liquid water. The study also shows that vibrational matching at the interface reduces wall-fluid friction and enhances water transport through nanopores.
Article
Chemistry, Physical
L. Savio, K. B. Bhavitha, G. Bracco, G. Luciano, D. Cavallo, G. Paolini, S. Passaglia, G. Carraro, L. Vattuone, R. Masini, M. Smerieri
Summary: The study investigates highly hydrophobic aluminium surfaces fabricated by chemical etching using Contact Angle Goniometry, Scanning Electron Microscopy, and X-ray Photoelectron Spectroscopy to correlate wettability with morphology and chemical composition. The etched aluminium surfaces exhibit binary structures with nanoscale block-like convexities and hollows, providing more space for air trapping. Results demonstrate that both hierarchical micro/nanostructures and surface composition contribute to excellent hydrophobic properties.
APPLIED SURFACE SCIENCE
(2021)
Article
Materials Science, Coatings & Films
Shafarina Azlinda Ahmad Kamal, Richard Ritikos, Saadah Abdul Rahman
Summary: The study found that increasing the annealing temperature can enhance the water repellence of carbon nitride nanostructures, significantly increasing the contact angle from 102.8° to 158.1° and greatly reducing the contact angle hysteresis. The film annealed at 700°C showed excellent durability performance, maintaining its super-hydrophobic behavior even after being subjected to more than 10 water droplets.
SURFACE & COATINGS TECHNOLOGY
(2021)
Review
Biochemical Research Methods
Navid Kashaninejad, Nam-Trung Nguyen
Summary: On-skin wearable systems for biofluid sampling and biomarker sensing have the potential to revolutionize healthcare monitoring and personalized medicine. However, there are challenges that need to be overcome to achieve widespread adoption of this technology. Microfluidic science and technology offer solutions for bridging the gap between basic and clinical research. The emerging field of epidermal microfluidics and advances in flexible microfluidic systems have the potential to enable on-skin wearable biofluid handling.
Review
Biochemical Research Methods
Samith Hettiarachchi, Haotian Cha, Lingxi Ouyang, Amith Mudugamuwa, Hongjie An, Gregor Kijanka, Navid Kashaninejad, Nam-Trung Nguyen, Jun Zhang
Summary: This paper comprehensively studies the latest progress in microfluidic technology for submicron and nanoparticle manipulation and separation. It summarizes the principles of traditional techniques and explores the physics, device design, working mechanism, and applications of different microfluidic approaches. The merits and demerits of microfluidic techniques are compared to conventional technologies. Seven standard post-separation detection techniques for nanoparticles are summarized, and current challenges and future perspectives on microfluidic technology for nanoparticle manipulation are discussed.
Review
Materials Science, Multidisciplinary
Hoang Huy Vu, Nam-Trung Nguyen, Navid Kashaninejad
Summary: Superhydrophobic surfaces with hierarchal micro/nanostructures have many interesting applications due to their self-cleaning, waterproof, anti-biofouling, anti-corrosion, and low-adhesion properties. However, they suffer from loss of superhydrophobicity over time and inability to repel all types of liquids. To overcome these issues, microstructures with re-entrant curvature have emerged, showing excellent liquid-repellent abilities and robustness. This review summarizes the design and fabrication strategies of these microstructures, emphasizing wettability studies and other surface properties, as well as potential applications and remaining technical challenges.
ADVANCED MATERIALS TECHNOLOGIES
(2023)
Review
Chemistry, Multidisciplinary
Du Tuan Tran, Ajeet Singh Yadav, Nhat-Khuong Nguyen, Pradip Singha, Chin Hong Ooi, Nam-Trung Nguyen
Summary: Micro elastofluidics, a new research field that combines characteristics of conventional microfluidics and fluid-structure interactions, holds promise for practical applications requiring direct contact between biological samples and fluid handling systems. Choosing the right material is crucial for the practical use of micro elastofluidics, especially in interaction with biological interfaces and long-term functionality. Biodegradable polymers have been extensively studied for this purpose, as they offer exceptional mechanical elasticity, excellent biocompatibility, and degradation into non-toxic products. This article provides an insightful and systematic review of the utilization of biodegradable polymers in digital and continuous-flow micro elastofluidics.
Review
Chemistry, Analytical
Ajeet Singh Yadav, Tran Du Tuan, Adrian J. T. Teo, Yuchen Dai, Fariba Malekpour Galogahi, Chin Hong Ooi, Nguyen Nam-Trung
Summary: Core-shell particles are micro- or nanoparticles with solid, liquid, or gas cores encapsulated by protective solid shells, which have attracted increasing attention as versatile carriers for pharmaceutical and biomedical applications. This review provides an overview of fabrication methods, and discusses their application and manipulation, including assembly, sorting, and triggered release. Approaches for diagnostics and drug delivery are also discussed in detail.
Review
Chemistry, Analytical
WaqarAhmed Afridi, Simon Strachan, Surasak Kasetsirikul, Amandeep Singh Pannu, Narshone Soda, Daniel Gough, Nam-Trung Nguyen, Muhammad J. A. Shiddiky
Summary: Lung cancer, especially small-cell lung cancer (SCLC), is a major cause of cancer-related deaths worldwide. Cancer cell-derived exosomes and exosomal miRNAs have been identified as promising biomarkers for diagnosing and prognosis of various diseases, including SCLC. However, there have been limited advances in analyzing SCLC-derived exosomes. This review discusses the epidemiology and prominent biomarkers of SCLC, effective strategies for isolating and detecting SCLC-derived exosomes and exosomal miRNA, and highlights the challenges and limitations of current methodologies, providing an overview of future perspectives for exosome-based SCLC research.
ACS MEASUREMENT SCIENCE AU
(2023)
Article
Nanoscience & Nanotechnology
Trung-Hieu Vu, Sharda Yadav, Canh-Dung Tran, Hong-Quan Nguyen, Tuan-Hung Nguyen, Thanh Nguyen, Tuan-Khoa Nguyen, Jarred W. Fastier-Wooller, Toan Dinh, Hoang-Phuong Phan, Hang Thu Ta, Nam-Trung Nguyen, Dzung Viet Dao, Van Thanh Dau
Summary: Electrohydrodynamic atomization (EHDA) is a precise method for controlling particle size and production rate, but the highly charged particles generated by conventional methods are not suitable for inhalation drug delivery. Researchers have developed a self-propelled EHDA system that can generate and deliver charge-reduced particles in one step. This system uses a sharp electrode to create ion wind, reducing the cumulative charge in the particles and transporting them to a target position. The technique has shown effective control over the morphologies of polymer products and has been proven safe for bioapplications, making it a versatile tool for drug delivery.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Nanoscience & Nanotechnology
Hung Nguyen, Thanh Nguyen, Duy Van Nguyen, Hoang-Phuong Phan, Tuan Khoa Nguyen, Dzung Viet Dao, Nam-Trung Nguyen, John Bell, Toan Dinh
Summary: This paper reports a significant enhancement of the photovoltaic effect in a 3C-SiC/Si heterostructure under the impact of a temperature gradient. The enhanced photovoltage can improve the sensitivity and reduce the energy consumption of microsensors.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Review
Engineering, Biomedical
Cuong Hung Luu, Nam-Trung Nguyen, Hang Thu Ta
Summary: This review provides a comprehensive study and discussion of the thrombosis-related issues in blood-contacting medical devices and summarizes several novel methods to prevent blood-material interactions or regulate coagulation reactions. It is of great importance for the prevention of thrombosis.
ADVANCED HEALTHCARE MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Dechao Chen, Muhammad Usman Zia, Fan Yang, Yuting Wang, Frederic D. L. Leusch, Nam-Trung Nguyen, Wei Zhang, Yongsheng Gao, Dongyuan Zhao, Colin L. L. Raston, Qin Li
Summary: A ligand-mediated, spatially-confined synthesis method is developed to produce high-quality carbon dots from crude bioresources. The choice of solvent plays a critical role in the formation and properties of the carbon dots. The ligand-carbon interactions and electron transfer result in the formation of uniform colloidal carbon dots with multiple emissions. These carbon dots can be easily dispersed in various solvents and fabricated into thin-film devices, making them suitable for optoelectronic applications.
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2023)
Proceedings Paper
Engineering, Electrical & Electronic
Luan Ngoc Mai, Tuan-Khoa Nguyen, Trung Hieu Vu, Thien Xuan Dinh, Canh-Dung Tran, Hoang-Phuong Phan, Toan Dinh, Thanh Nguyen, Nam-Trung Nguyen, Dzung Viet Dao, Van Thanh Dau
Summary: This paper presents the development of an ion-wind powered boat (iBoat) with a propeller-less design, low noise, and energy-efficient features. The iBoat utilizes a conducting wire as the ion emitter and the water surface as the ground electrode, eliminating the need for a counter electrode. A miniature version of the iBoat and an electro-hydrodynamic propulsion system are also developed, achieving a high thrust-to-power ratio using a novel wire-dielectric-water configuration. Numerical simulations are performed to explain the underlying physical principles of this concept.
2023 IEEE 36TH INTERNATIONAL CONFERENCE ON MICRO ELECTRO MECHANICAL SYSTEMS, MEMS
(2023)
Article
Biochemical Research Methods
Yingdong Luo, Yuanyuan Huang, Yani Li, Xiudong Duan, Yongguang Jiang, Cong Wang, Jiakun Fang, Lei Xi, Nam-Trung Nguyen, Chaolong Song
Summary: Biomolecular imaging is used for imaging and screening of intracellular structures of a single cell in metabolic engineering. However, current methods are limited to population-scale identification of cell phenotyping. To address this challenge, we propose to use dispersive phase microscopy combined with a droplet-based microfluidic system to achieve high-throughput screening of cells with an identified phenotype. The system has been validated for single-cell imaging and droplet manipulation, showing great potential for various biofactory scenarios.
Review
Environmental Sciences
Shui Cheung Edgar Leung, Dushanthi Wanninayake, Dechao Chen, Nam-Trung Nguyen, Qin Li
Summary: This article summarises the unique physicochemical properties of PFAS and critically reviews the intermolecular and intramolecular physicochemical interactions. It explores how these interactions can be applied to the process of sensing, capturing, and recycling PFAS. The influential factors and properties of these interactions are compared and recommendations for future designs are provided.
SCIENCE OF THE TOTAL ENVIRONMENT
(2023)