Search for low-energy induced depletion of 178Hfm2 at the SPring-8 synchrotron

Electromagnetic transitions within nuclei reflect specific aspects of nuclear structure. This is particularly true for metastable excited states, or isomers, like Hf-178(m2) (T-1/2 = 31 years, excitation energy 2446 keV). The interaction of external radiation with isomers can be used to study atomic and nuclear properties and. perhaps, to induce a release of the stored energy. Some experiments indicated that low-energy photons near the L-3 edge (9.561 keV) Of hafnium could cause this to occur for Hf-178(m2), but the lack of a viable physical model and null experiments by other groups have left these claims in doubt. The present work describes a new experiment to examine this process by closely duplicating the irradiation conditions in positive studies, but using a more advanced multi-detector gamma array. No support for ail induced depletion of Hf-178(m2) by low-energy photons was obtained, with an upper limit for the integral cross section that is eight orders-of-magnitude below the reported value. (C) 2009 Elsevier B.V. All rights reserved.