期刊
PHYSICAL REVIEW LETTERS
卷 121, 期 13, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.121.136402
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资金
- Danish Council for Independent Research
- Natural Sciences under the Sapere Aude program [DFF-4002-00029]
- VILLUM FONDEN via the Center of Excellence for Dirac Materials [11744]
The spin structure of the valence and conduction bands at the (K) over bar and (K) over bar' valleys of single-layer WS2 on Au(111) is determined by spin-and angle-resolved photoemission and inverse photoemission. The bands confining the direct band gap of 1.98 eV are out-of-plane spin polarized with spin-dependent energy splittings of 417 meV in the valence band and 16 meV in the conduction band. The sequence of the spin-split bands is the same in the valence and in the conduction bands and opposite at the (K) over bar and the (K) over bar' high-symmetry points. The first observation explains dark excitons discussed in optical experiments; the latter points to coupled spin and valley physics in electron transport. The experimentally observed band dispersions are discussed along with band structure calculations for a freestanding single layer and for a single layer on Au(111).
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