期刊
PHYSICAL REVIEW LETTERS
卷 113, 期 14, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.113.143002
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资金
- French Agence Nationale de la Recherche IDEO Project [ANR-09-BLAN-0022]
- French Agence Nationale de la Recherche of Tomsk State University Competitiveness Improvement Program
- French-Russian SAMIA network
- IDRIS/CINES/ROMEO computer centers
- OTKA [F72423]
- Agence Nationale de la Recherche (ANR) [ANR-09-BLAN-0022] Funding Source: Agence Nationale de la Recherche (ANR)
Since the discovery of anomalies in ozone isotope enrichment, several fundamental issues in the dynamics linked to the shape of the potential energy surface in the transition state region have been raised. The role of the reeflike structure on the minimum energy path is an intricate question previously discussed in the context of chemical experiments. In this Letter, we bring strong arguments in favor of the absence of a submerged barrier from ultrasensitive laser spectroscopy experiments combined with accurate predictions of highly excited vibrations up to nearly 95% of the dissociation threshold.
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