4.8 Article

Hourglass Dispersion in Overdoped Single-Layered Manganites

期刊

PHYSICAL REVIEW LETTERS
卷 108, 期 24, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.108.247209

关键词

-

资金

  1. Deutsche Forschungsgemeinschaft [Sonderforschungsbereich 608]

向作者/读者索取更多资源

The incommensurate stripelike magnetic ordering in two single-layered manganites, Nd0.33Sr1.67MnO4 and Pr0.33Ca1.67MnO4, is found to exhibit an hourglasslike excitation spectrum very similar to that seen in various cuprates superconductors, but only for sufficiently short correlation lengths. Several characteristic features of an hourglass dispersion can be identified: enhancement of intensity at the merging of the incommensurate branches, rotation of the intensity maxima with higher energy transfer, and suppression of the outward-dispersing branches at low energy. The correlation length of the magnetic ordering and the large ratio of intra- to interstripe couplings are identified as the decisive parameters causing the hourglass

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.8
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

Article Materials Science, Multidisciplinary

Crystal structure and distortion of superconducting CuxBi2Se3

Tobias Froehlich, Zhiwei Wang, Mahasweta Bagchi, Anne Stunault, Yoichi Ando, Markus Braden

PHYSICAL REVIEW MATERIALS (2020)

Article Materials Science, Multidisciplinary

Evidence for current-induced phase coexistence in Ca2RuO4 and its influence on magnetic order

K. Jenni, F. Wirth, K. Dietrich, L. Berger, Y. Sidis, S. Kunkemoeller, C. P. Grams, D. Khomskii, J. Hemberger, M. Braden

PHYSICAL REVIEW MATERIALS (2020)

Article Materials Science, Multidisciplinary

X-ray absorption and x-ray magnetic circular dichroism in bulk and thin films of ferrimagnetic GdTiO3

R. Aeschlimann, M. N. Grisolia, G. Sanchez-Santolino, J. Varignon, F. Choueikani, R. Mattana, V Garcia, S. Fusil, T. Frohlich, M. Braden, B. Delley, M. Varela, P. Ohresser, J. Santamaria, A. Barthelemy, C. Piamonteze, M. Bibes

Summary: This study investigates the magnetic behavior of rare-earth titanates, revealing the ferrimagnetic nature of GdTiO3 and providing insights into its structural and electronic properties in bulk and thin film form. The research sheds light on the insufficiently explored magnetic states of these complex materials, particularly at oxide interfaces.

PHYSICAL REVIEW MATERIALS (2021)

Article Physics, Multidisciplinary

Measurement of Spin Dynamics in a Layered Nickelate Using X-Ray Photon Correlation Spectroscopy: Evidence for Intrinsic Destabilization of Incommensurate Stripes at Low Temperatures

Alessandro Ricci, Nicola Poccia, Gaetano Campi, Shrawan Mishra, Leonard Mueller, Boby Joseph, Bo Shi, Alexey Zozulya, Marcel Buchholz, Christoph Trabant, James C. T. Lee, Jens Viefhaus, Jeroen B. Goedkoop, Agustinus Agung Nugroho, Markus Braden, Sujoy Roy, Michael Sprung, Christian Schuessler-Langeheine

Summary: Using x-ray photon correlation spectroscopy, fluctuations in stripe-type spin order of a layered nickelate were observed on timescales of tens of minutes across a wide temperature range. These fluctuations exhibit anomalous temperature dependence, slowing down at intermediate temperatures and speeding up during heating and cooling, reflecting a direct connection with spatial correlations. The decay of nickelate stripe correlations at low temperatures, similar to the competition between stripes and superconductivity in cuprates, occurs through loss of both spatial and temporal correlations.

PHYSICAL REVIEW LETTERS (2021)

Article Physics, Multidisciplinary

Combined Arrhenius-Merz Law Describing Domain Relaxation in Type-II Multiferroics

J. Stein, S. Biesenkamp, T. Cronert, T. Froehlich, J. Leist, K. Schmalzl, A. C. Komarek, M. Braden

Summary: The domain relaxation process in multiferroic TbMnO3 single crystals under different electric fields and temperatures can be described by a combination of activation law and Merz law, with just two parameters to explain the relaxation times. The domain inversion process is mainly controlled by domain wall motion, with other mechanisms causing accelerated inversion near the multiferroic transition.

PHYSICAL REVIEW LETTERS (2021)

Review Physics, Condensed Matter

High-Pressure Studies of Correlated Electron Systems

Pau Jorba, Alexander Regnat, Anh Tong, Marc Seifert, Andreas Bauer, Michael Schulz, Christian Franz, Astrid Schneidewind, Stefan Kunkemoeller, Kevin Jenni, Markus Braden, Andre Deyerling, Marc A. Wilde, James S. Schilling, Christian Pfleiderer

Summary: The study demonstrates that tuning the crystallographic lattice constants can alter the electronic properties of transition-metal and rare-earth compounds, providing access to new forms of order. Experimental setups including tungsten carbide and moissanite cells, as well as bespoke diamond anvil cells, have successfully allowed studies on resistivity and neutron depolarization under high pressure conditions.

PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS (2022)

Article Physics, Multidisciplinary

Gigantic Magnetochiral Anisotropy in the Topological Semimetal ZrTe5

Yongjian Wang, Henry F. Legg, Thomas Boemerich, Jinhong Park, Sebastian Biesenkamp, A. A. Taskin, Markus Braden, Achim Rosch, Yoichi Ando

Summary: Researchers have discovered that ZrTe5 crystals exhibit a gigantic magnetochiral anisotropy when they are in proximity to a topological quantum phase transition, which is the largest ever observed. The low carrier density, inhomogeneities, and torus-shaped Fermi surface induced by breaking of inversion symmetry in a Dirac material are argued to be central to explaining this extraordinary property.

PHYSICAL REVIEW LETTERS (2022)

Article Materials Science, Multidisciplinary

Magnon dispersion in ferromagnetic SrRuO3

K. Jenni, S. Kunkemoeller, A. Tewari, R. A. Ewings, Y. Sidis, A. Schneidewind, P. Steffens, A. A. Nugroho, M. Braden

Summary: The magnetic excitations in ferromagnetic SrRuO3 were investigated using inelastic neutron scattering experiments on triple-axis and time-of-flight spectrometers. The low-energy low-temperature response exhibited a quadratic spin-wave dispersion with an anisotropy gap. The magnon dispersion extended up to 35 meV, with no evidence of a continuum of Stoner excitations below this energy. However, the magnon response weakened at higher energies. In addition to the anomalous softening of the spin-wave stiffness and gap induced by the topology of the Bloch states, the magnon excitations also showed broadening in energy, which increased with temperature.

PHYSICAL REVIEW B (2023)

Article Materials Science, Multidisciplinary

Quasimolecular electronic structure of the spin-liquid candidate Ba3InIr2O9

A. Revelli, M. Moretti Sala, G. Monaco, M. Magnaterra, J. Attig, L. Peterlini, T. Dey, A. A. Tsirlin, P. Gegenwart, T. Froehlich, M. Braden, C. Grams, J. Hemberger, P. Becker, P. H. M. van Loosdrecht, D. I. Khomskii, J. van den Brink, M. Hermanns, M. Grueninger

Summary: Ba3InIr2O9 is a promising candidate for quantum spin-liquid behavior and exhibits magnetism from spin-orbit entangled quasimolecular moments. Our study reveals its unique electronic states and excitations through various experimental and computational methods.

PHYSICAL REVIEW B (2022)

Article Materials Science, Multidisciplinary

Spin-orbit coupling and crystal-field splitting in Ti-doped Ca2RuO4 studied by ellipsometry

I Vergara, M. Magnaterra, P. Warzanowski, J. Attig, S. Kunkemoeller, D. Khomskii, M. Braden, M. Hermanns, M. Grueninger

Summary: This article discusses the competition between spin-orbit coupling and crystal field splitting in Ca2RuO4, and explains the orbital occupation ratio using optical spectral weights. The study shows that Δ(CF)/ζ is between 2.4 and 4 at 15 K. The crystal field dominates the orbital order of the ground state, but spin-orbit coupling is necessary for a quantitative description of the properties. Furthermore, the crystal field splitting decreases with increasing temperature.

PHYSICAL REVIEW B (2022)

Article Materials Science, Multidisciplinary

Chirality of magnetic excitations in ferromagnetic SrRuO3

K. Jenni, S. Kunkemoeller, W. Schmidt, P. Steffens, A. A. Nugroho, M. Braden

Summary: By conducting polarized inelastic neutron scattering experiments under magnetic fields, we have determined the chirality of ferromagnetic zone-center excitations as a function of temperature. The results show that the excitation is perfectly chiral in the ferromagnetic phase and when the spontaneous magnetization is almost completely suppressed, the chirality is reduced but does not change sign.

PHYSICAL REVIEW B (2022)

Article Materials Science, Multidisciplinary

Chiral order and multiferroic domain relaxation in NaFeGe2O6

S. Biesenkamp, D. Gorkov, W. Schmidt, K. Schmalzl, Y. Sidis, P. Becker, L. Bohaty, M. Braden

Summary: This study investigates the magnetic structure and multiferroic relaxation dynamics of NaFeGe2O6 using neutron scattering, revealing an additional component of magnetic moments at lower temperatures and demonstrating the reversibility of controlling spin-spiral handedness with external electric fields. The time-resolved measurements show a simple temperature and electric-field dependence of multiferroic relaxation, similar to what has been observed in TbMnO3, with the maximum speed of domain wall motion comparable to the spin-wave velocity.

PHYSICAL REVIEW B (2021)

Article Materials Science, Multidisciplinary

Multiple field-induced phases in the frustrated triangular magnet Cs3Fe2Br9

D. Breuning, T. Froehlich, D. Gorkov, I. Cisarova, Y. Skourski, L. Rossi, B. Bryant, S. Wiedmann, M. Meven, A. Ushakov, S. V. Streltsov, D. Khomskii, P. Becker, L. Bohaty, M. Braden, T. Lorenz

Summary: The Cs3Fe2Br9 material contains Fe2Br9 bi-octahedra with semiclassical S = 5/2 Fe3+ spins, leading to a rich magnetic phase diagram with different ordered phases. The high degree of magnetic frustration and strong magnetoelastic coupling result in a surprisingly complex magnetic behavior in this material.

PHYSICAL REVIEW B (2021)

Article Materials Science, Multidisciplinary

Neutron scattering studies on spin fluctuations in Sr2RuO4

K. Jenni, S. Kunkemoeller, P. Steffens, Y. Sidis, R. Bewley, Z. Q. Mao, Y. Maeno, M. Braden

Summary: The magnetic excitations in Sr2RuO4 were studied through polarized and unpolarized neutron scattering experiments, revealing that there is no evidence for resonance excitation in the superconducting phase at the scattering vector of the Fermi-surface nesting. Existing data suggests a weakening of scattered intensity in the nesting spectrum at very low energies, while a quasiferromagnetic contribution persists with a finite width in momentum space even at higher temperatures.

PHYSICAL REVIEW B (2021)

Article Materials Science, Multidisciplinary

Single-crystal investigations on the multiferroic material LiFe(WO4)2

S. Biesenkamp, D. Gorkov, D. Bruening, A. Bertin, T. Froehlich, X. Fabreges, A. Gukasov, M. Meven, P. Becker, L. Bohaty, T. Lorenz, M. Braden

Summary: The crystal and magnetic structures of multiferroic LiFe(WO4)(2) were studied through specific heat, susceptibility, and neutron diffraction experiments. Two different magnetic phases with incommensurate order were observed at different temperatures, demonstrating multiferroic behavior. LiFe(WO4)(2) exhibits a simple phase diagram with a sequence of transitions typical for a type-II multiferroic material.

PHYSICAL REVIEW B (2021)

暂无数据