期刊
PHYSICAL REVIEW LETTERS
卷 104, 期 7, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.104.073002
关键词
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The benchmark system of molecular photoionization dynamics, the (1 + 1') two-photon ionization of NO via the A state, is investigated using the time-energy mapping of the photoelectron angular distribution in a laboratory frame. The molecular frame photoelectron angular distribution and partial wave composition are determined from time-energy maps and compared with those obtained by Schwinger variational calculation (SVC) and state-to-state photoelectron spectroscopy. Good agreement is found with SVC. By comparison of the phase shifts of the scattering waves and the quantum defects of the Rydberg states, the l hybridization of p waves is identified.
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