期刊
PHYSICAL REVIEW LETTERS
卷 101, 期 13, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.101.133003
关键词
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资金
- ALS
- NSF [PHY-05-55699]
- CNRS
- Institut du Developpement et des Ressources en Informatique Scientifique (IDRIS), France
Polarization-dependent resonant inelastic x-ray scattering (RIXS) is shown to be a new probe of molecular-field effects on the electronic structure of isolated molecules. A combined experimental and theoretical analysis explains the linear dichroism observed in Cl 2p RIXS following Cl 1s excitation in HCl and CF(3)Cl as due to molecular-field effects, including singlet-triplet exchange, indicating polarized-RIXS provides a direct probe of spin-orbit-state populations applicable to any molecule.
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