期刊
PHYSICAL REVIEW B
卷 87, 期 16, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.87.161121
关键词
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资金
- National Basic Research Program of China [2011CBA00103, 2012CB927404, 2010CB923003]
- National Science Foundation of China
- Fundamental Research Funds for the Central Universities of China
Motivated by the rich interplay among electronic correlation, spin-orbit coupling (SOC), crystal-field splitting, and geometric frustrations in the honeycomblike lattice, we systematically investigated the electronic and magnetic properties of Li2RhO3. The material is semiconducting with a narrow band gap of Delta similar to 78 meV, and its temperature dependence of resistivity conforms to a three-dimensional variable range hopping mechanism. No long-range magnetic ordering was found down to 0.5 K, due to the geometric frustrations. Instead, single atomic spin-glass behavior below the spin-freezing temperature (similar to 6 K) was observed and its spin dynamics obeys the universal critical slowing down scaling law. A first-principles calculation suggested it to be a relativistic Mott insulator mediated by both electronic correlation and SOC. With moderate strength of electronic correlation and SOC, our results shed light on the research of the Heisenberg-Kitaev model in realistic materials.
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