Plasmonic crystals for ultrafast nanophotonics: Optical switching of surface plasmon polaritons

We demonstrate that the dispersion of surface plasmon polaritons in a periodically perforated gold film can be efficiently manipulated by femtosecond laser pulses in spectral regions far from the intrinsic gold resonances. Using a time- and frequency-resolved pump-probe technique we observe shifting of the plasmon polariton resonances with response times from 200 to 800 fs depending on the probe photon energy, by which we obtain comprehensive insight into the electron dynamics in gold. We show that Wood anomalies in the optical spectra provide pronounced resonances in differential transmission and reflection with magnitudes up to 3% for moderate pump fluences of 0.5 mJ/cm(2).