4.6 Article

5f delocalization-induced suppression of quadrupolar order in U(Pd1-xPtx)3

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PHYSICAL REVIEW B
卷 84, 期 23, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.84.235142

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  1. UK Engineering and Physical Sciences Research Council
  2. DFG [SU229/1-3]
  3. US Department of Energy, Division of Materials Science [DE-AC02-98CH10886]

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We present bulk magnetic and transport measurements and x-ray resonant scattering measurements on U(Pd1-xPtx)(3) for x = 0.005 and 0.01, which demonstrate the high sensitivity of the quadrupolar order in the canonical antiferroquadrupolar ordered system UPd3 to doping with platinum. Bulk measurements for x = 0.005 reveal behavior similar to that seen in UPd3, albeit at a lower temperature, and x-ray resonant scattering provides evidence of quadrupolar order described by the Q(xy) order parameter. In contrast, bulk measurements reveal only an indistinct transition in x = 0.01, consistent with the observation of short-range quadrupolar order in our x-ray resonant scattering results.

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