4.6 Article

Local spin fluctuations in iron-based superconductors: 77Se and 87Rb NMR measurements of Tl0.47Rb0.34Fe1.63Se2

期刊

PHYSICAL REVIEW B
卷 84, 期 22, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.84.220505

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资金

  1. NSFC [10974254, 11074304, 10874244]
  2. National Basic Research Program of China [2010CB923000, 2011CBA00112]
  3. Chinese MoE

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We report nuclear magnetic resonance (NMR) studies of the intercalated iron selenide superconductor (Tl,Rb)(y)Fe2-xSe2 (T-c = 32 K). Single-crystal measurements up to 480 K on both Se-77 and Rb-87 nuclei show a superconducting phase with no magnetic order. The Knight shifts K and relaxation rates 1/T1T increase very strongly with temperature above T-c, before flattening at 400 K. The quadratic T-dependence and perfect proportionality of both K and 1/T1T data demonstrate their origin in paramagnetic moments. A minimal model for this pseudogap-type response is not a missing density of states, but rather two additive contributions from the itinerant electronic and local magnetic components, a framework unifying the K and 1/T1T data in many iron-based superconductors.

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