期刊
PHYSICAL REVIEW B
卷 84, 期 19, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.84.193101
关键词
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资金
- JSPS [21684019]
- MEXT, Japan
- Grants-in-Aid for Scientific Research [20540324, 20102003, 21684019, 11J05912] Funding Source: KAKEN
The Kondo resonance at the Fermi level is well established for the electronic structure of Ce (4f(1) electron) and Yb (4f(1) hole)-based systems. In this work, we report complementary experimental and theoretical studies on the Kondo resonance in the Pr-based 4f(2) system, PrTi2Al20. Using Pr 3d-4f resonant photoemission spectroscopy and single-impurity Anderson model (SIAM) calculations including the full multiplets of Pr ions, we show that a 4f(2) system can also give rise to a Kondo resonance at the Fermi level. The Kondo resonance peak is experimentally observed through a final-state multiplet-dependent resonance and is reproduced with properly tuned hybridization strength in SIAM calculations.
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