期刊
PHYSICAL REVIEW B
卷 83, 期 12, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.83.125419
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资金
- Deutsche Forschungsgemeinschaft (DFG)
- German-Israeli Foundation for Scientific Development (GIF)
We analyze various limits of vibrationally coupled resonant electron transport in single-molecule junctions. Based on a master equation approach, we discuss analytic and numerical results for junctions under a high bias voltage or weak electronic-vibrational coupling. It is shown that in these limits, the vibrational excitation of the molecular bridge increases indefinitely, i.e., the junction exhibits a vibrational instability. Moreover, our analysis provides analytic results for the vibrational distribution function and reveals that these vibrational instabilities are related to electron-hole pair creation processes.
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