期刊
PHYSICAL REVIEW B
卷 81, 期 24, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.81.245407
关键词
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资金
- Engineering and Physical Sciences Research Council (EPSRC)
- Engineering and Physical Sciences Research Council [EP/E062636/1] Funding Source: researchfish
- EPSRC [EP/E062636/1] Funding Source: UKRI
We present a general microscopic theory of intense optical pulse propagation in conjugated polymers. The multiscale theory is based on a combination of density-functional theory on the molecular level and many-particle vibronic density matrices which act as a source in Maxwell's equations. The resulting equations are solved nonperturbatively in the light field to study optical amplification and lasing. We illustrate our approach using a polyfluorene material of particular current interest containing a small component of planar (beta-phase) chromophores. Significant reshaping of amplified light pulses is found, stemming from the interplay between light propagation and the excitation of numerous vibrational modes. Furthermore a rich dynamic is observed in the amplified spontaneous emission regime with oscillatory structures rooted in the dynamical population and depopulation of lattice modes.
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