Article
Chemistry, Physical
Gaoshang Gong, Jin Zhou, Yaran Duan, Huiyun Hu, Yongqiang Wang, Xuerui Cheng, Yuling Su
Summary: The study reveals that one-dimensional frustrated material Ca3CoMnO6 exhibits weak relaxor ferroelectric behavior and the presence of polar nanoregions, which results in the suppressed macroscopic ferroelectric polarization.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Engineering, Electrical & Electronic
Rui Wu, Di Zhang, Tuhin Maity, Ping Lu, Jie Yang, Xingyao Gao, Shishun Zhao, Xiucheng Wei, Hao Zeng, Ahmed Kursumovic, Guang Tian, Weiwei Li, Chao Yun, Yongqiang Wang, Zengyao Ren, Ziyao Zhou, Ming Liu, Kelvin H. L. Zhang, Quanxi Jia, Jinbo Yang, Haiyan Wang, Judith L. MacManus-Driscoll
Summary: Adding antiferromagnet to a 3-1-type multiferroic nanocomposite can result in a large, self-biased magnetoelectric effect at room temperature.
NATURE ELECTRONICS
(2021)
Article
Chemistry, Physical
Y. M. Xie, C. C. Wang
Summary: The memory effect of magnetoelectric coupling is observed in Co4Ta2O9, and it can be manipulated by adjusting the applied magnetic field and polarization process.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Materials Science, Multidisciplinary
Vilmos Kocsis, Yusuke Tokunaga, Yoshinori Tokura, Yasujiro Taguchi
Summary: The study reveals that the linear magnetoelectric effect allows for selection or switching between antiferromagnetic states through the application of electric and magnetic fields, which are preserved by energy barriers. Experimental results show that the field and temperature variation of the coercive field for switching is similar to the theoretical model. Investigation into the dynamics of antiferromagnetic domain switching confirms a power-law frequency dependence, indicating one-dimensional domain wall propagation.
Article
Materials Science, Ceramics
Andre Maia, Christelle Kadlec, Maxim Savinov, Rui Vilarinho, Joaquim Agostinho Moreira, Viktor Bovtun, Martin Kempa, Martin Misek, Jiri Kastil, Andriy Prokhorov, Jan Manak, Alexei A. Belik, Stanislav Kamba
Summary: Type-II multiferroics show large magnetoelectric coupling and are promising for new device functionalities. We report a new multiferroic material, BiMn3Cr4O12, where an antiferromagnetic phase is induced by the structural change at the ferroelectric phase transition. Thermodynamic, dielectric, and pyroelectric studies reveal that the ferroelectric critical temperature corresponds to the Ne'el temperature of the Cr3+ spins, and an increase in ferroelectric polarization is observed below the Ne'el temperature of the Mn3+ spins.
JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
(2023)
Review
Chemistry, Physical
Ganesha Channagoudra, Vijaylakshmi Dayal
Summary: This paper emphasizes the progress on magnetoelectric coupling and the impact of charge and strain in composite heterostructures. The direct and converse magnetoelectric effect on improving the magnetoelectric coefficient is discussed. Furthermore, a brief overview of devices based on multiferroic magnetoelectric materials and their future perspectives is presented.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Chemistry, Physical
Gowher Hameed Rather, Mehraj ud Din Rather, Nazima Nazir, Afreen Ikram, Mohd Ikram, Basharat Want
Summary: The study fabricates multiferroic particulate composites from terbium doped BaTiO3 and manganese doped CoFe2O4, improving dielectric and magnetic properties for unifying multiple order parameters. Structural changes and enhanced physical properties in multiferroic composites can be utilized for magnetoelectric device applications.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Materials Science, Ceramics
Yunke Chen, Xiong Luo, Xiaoxuan Ma, Chao Xu, Baojuan Kang, Wenlai Lu, Jincang Zhang, Shixun Cao
Summary: High quality Fe4Nb2O9 single crystal was grown by optical floating zone method. Magnetization measurements showed consistent results with reported magnetic structure obtained by neutron diffraction. Pyroelectric current-temperature curves revealed ferroelectric polarization below 90 K, which has not been reported before in single crystal Fe4Nb2O9. The single crystal also exhibited magnetoelectric coupling effect, with polarization increasing under applied magnetic field.
CERAMICS INTERNATIONAL
(2021)
Article
Materials Science, Ceramics
Jae-Hyeon Cho, Seongwoo Cho, Jun Han Lee, Haribabu Palneedi, Ju-Hyeon Lee, Hwang-Pill Kim, Nyun Jong Lee, Siriporn Tigunta, Soodkhet Pojprapai, Sanghoon Kim, Jungho Ryu, Yoon Seok Oh, Seungbum Hong, Wook Jo
Summary: Intentional subtraction of Fe ions in NiFe2O4 induces spin canting and enhances magnetoelectric coupling, while also generating ferroelectricity. The peak enhancement in magnetoelectric coupling strength is observed when about 30% of Fe ions are subtracted, after which further removal of Fe ions affects the material's structure.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2021)
Article
Quantum Science & Technology
Ye Shao, Fengzhen Huang, Junting Zhang, Shuo Yan, Shuyu Xiao, Xiaomei Lu, Jinsong Zhu
Summary: This research demonstrates the successful induction of conical magnetic structure in BaFe12O19 by introducing a nonzero DM interaction through partial substitution of Fe3+ sites, leading to direct ME and magnetodielectric coupling in In-doped BaFe12O19 ceramics. Additionally, BaZn0.9Zr0.9Fe10.2O19 ceramics exhibit noncollinear magnetic structure and direct ME coupling due to larger Zn2+ and Zr4+ ions preferring the spin-down sites. The results provide a feasible approach to develop multiferroic and magnetoelectric coupling in ubiquitous M-type hexaferrite.
ADVANCED QUANTUM TECHNOLOGIES
(2021)
Article
Engineering, Manufacturing
Steven Malley, Scott Newacheck, George Youssef
Summary: The research emphasizes the opportunities and challenges of additively manufacturing magnetoelectric composite materials using digital light projection, highlighting the tailorability of the mechano-electro-magnetic properties.
ADDITIVE MANUFACTURING
(2021)
Article
Materials Science, Multidisciplinary
Pedro Martins, Ana C. Lima, Victor A. L'vov, Nelson Pereira, Pimpet Sratong-on, Hideki Hosoda, Volodymyr Chernenko, Senentxu Lanceros-Mendez
Summary: This study demonstrates a significant resonance amplification of the ME effect by incorporating Ni-Mn-Ga particles into P(VDF-TrFE) piezopolymer, resulting in a giant ME coefficient of 6.05 V.cm(-1) under specific magnetic fields. The physical mechanism behind this enhancement involves the volume magnetostriction of the magnetostrictive particles and the resonant elastic oscillation of the piezoelectric polymer matrix.
APPLIED MATERIALS TODAY
(2022)
Article
Materials Science, Multidisciplinary
Amit Kumar, Piyush K. Patel, K. L. Yadav, Yogendra Singh, Naveen Kumar, Abdullah, G. Sharma, Satyendra Singh
Summary: The effect of grain boundary resistance (G(BR)) and grain resistance (G(R)) on the magnetoelectric coupling in multiferroic composite thick films of BiFeO3 (BFO) nanocrystalline powder and poly vinylidene-fluoride (PVDF) polymer is significant. The study shows that grain boundary resistance plays an important role in strengthening the magnetoelectric effect in the BFO-PVDF system, with the BFO50 sample demonstrating promising results for device and sensor applications.
MATERIALS RESEARCH BULLETIN
(2022)
Article
Materials Science, Multidisciplinary
Tomohiro Ichinose, Hiroshi Naganuma
Summary: Evaluation of the bidirectional magnetoelectric effect in a BiFeO3/NiFeCuMo bilayer demonstrates that the electronically controlled ME effect and magnetically controlled ME effect have separate origins. The magnetically controlled ME effect is attributed to the cycloidal magnetic structure of the bulk BFO, while the electronically controlled ME effect is achieved through electric-field-induced ferroelectric polarization switching. The bidirectional ME effect is a result of the combination of the cycloidal magnetic structure throughout the film and an uncompensated weak ferromagnetic interface near the BFO/NiFeCuMo interface.
PHYSICAL REVIEW MATERIALS
(2023)
Article
Chemistry, Physical
Anusree Das, Nilesh Khamaru, Sudipta Bandyopadhyay, Souvik Chatterjee, Dipankar Das
Summary: This study synthesized nanocomposites (NCs) containing SrFe12O19 and Bi0.9Dy0.1FeO3, where Dy-substitution increased the magnetization and dielectric constant of BiFeO3 (BFO), while increasing SFO content in the NCs led to higher magnetization but lower dielectric constant. The changes in capacitance of the NC samples in the presence of a magnetic field up to 150 kOe indicated a substantial enhancement of the magnetoelectric (ME) coupling coefficient of BFO in the nanocomposites, which tended to improve with higher SFO content in the NCs.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Chemistry, Multidisciplinary
Jonas Ruby Sandemann, Thomas Bjorn Egede Gronbech, Kristoffer Andreas Holm Stockler, Feng Ye, Bryan C. Chakoumakos, Bo Brummerstedt Iversen
Summary: ZnFe2O4 exhibits spin-glass transition and has dominant ferromagnetic and antiferromagnetic correlations. The 3D-m Delta PDF method is used to visualize the local magnetic ordering preferences.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Shitong Wang, Lijiang Zhao, Yanhao Dong, He Zhu, Yang Yang, Haowei Xu, Baoming Wang, Yakun Yuan, Yang Ren, Xiaojing Huang, Wei Quan, Yutong Li, Yimeng Huang, Charles M. Settens, Qi He, Yongwen Sun, Hua Wang, Zunqiu Xiao, Wenjun Liu, Xianghui Xiao, Riqiang Fu, Qiang Li, Yong S. Chu, Zhongtai Zhang, Qi Liu, Andrew M. Minor, Junying Zhang, Zilong Tang, Ju Li
Summary: Wadsley-Roth oxides (WROs) with pore diameters of 2.5 angstrom < d < 2.8 angstrom allow rapid diffusion of Li+ in single-crystal particles, enabling high-rate charge cycles similar to gasoline vehicles and improving the cycle life up to 10,000 cycles.
ENERGY & ENVIRONMENTAL SCIENCE
(2023)
Article
Materials Science, Ceramics
Abhijit Pramanick, Laurent Daniel, Sarangi Venkateshwarlu, Valentin Segouin, Yang Ren
Summary: Through experimental and modeling results, we have discovered a unique tetragonal-to-orthorhombic-to-tetragonal phase transformation induced under low electric fields (< 1 kV/mm) in grains with 002 crystallographic poles oriented either within 20 degrees or orthogonal to the applied electric-field direction in a polycrystalline Pb-free piezoceramic. In contrast, grains with their 002 poles oriented 30 degrees- 80 degrees to the electric-field direction undergo a continuous tetragonal-to-orthorhombic transformation for electric fields larger than 1 kV/mm. These findings highlight the critical role of a phase-transition-assisted domain switching mechanism in grains of specific orientations towards achieving a large electrostrain coefficient of d(33)* similar to 600 pm/V under low electric fields (< 1 kV/mm) in the Pb-free Sn-doped (Ba,Ca)(Zr,Ti)O-3 piezoceramic.
JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
(2023)
Article
Nanoscience & Nanotechnology
Yingchao Li, Junsong Zhang, Martin Saunders, Yang Ren, Hong Yang, Yinong Liu
Summary: By utilizing the principles of lattice strain matching and collective atomic load transfer, ultralarge elastic strains were induced in a brittle NiTi-Nb3Sn eutectic composite, where Nb3Sn lamellae achieved a remarkable elastic lattice strain of -2.4%. This study both tests the applicability of lattice strain matching in brittle materials and explores a novel fabrication approach for in-situ composites via eutectic solidification.
MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING
(2023)
Article
Environmental Sciences
Tingting Kang, Han Wang, Zhangyuan He, Zhengying Liu, Yang Ren, Pengjun Zhao
Summary: This paper explores the impact of land use change on energy-related CO2 emissions using multi-dimension metrics. The results indicate that the scale of land use types has a bidirectional effect on emissions; land use mixture in mature city agglomerations has a significant suppressive effect; land use intensity is associated with emissions in most cities, with adverse effects spreading from west to northeast. Therefore, it is suggested to regulate land transaction, promote mixed land use, and utilize renewable energy to reduce energy footprints and mitigate emissions.
SCIENCE OF THE TOTAL ENVIRONMENT
(2023)
Article
Chemistry, Multidisciplinary
Yadong Liu, Yikang Yu, Fan Yang, Guangqi Zhu, Kang Yu, Ronghui Kou, Chengjun Sun, Yuzi Liu, Jiayi Xu, Cong Liu, Chenzhao Li, Tianwei Liu, Yang Ren, Wenquan Lu, Rafael Ferreira, Paulo Ferreira, Zhengcheng Zhang, Jian Xie
Summary: A sustainable FeOF nanocomposite with extraordinary performance has been developed in this study. Compared to the current mono-valence intercalation LiCoO2, it exhibits a specific capacity and energy of 621 mAh g(-1) and 1124 Wh kg(-1), respectively, which is three times the specific capacity and double the specific energy. The (de)lithiation process is made reversible by combining nanostructured FeOF with graphene, providing interparticle electric conduction. This breakthrough represents a significant progress in developing sustainable conversion materials, eventually overcoming the driving range and cost barriers.
Article
Materials Science, Multidisciplinary
Taotao Wang, Xiangxiang Rao, Qiang Zhang, Daqiang Jiang, Yang Ren, Lishan Cui, Kaiyuan Yu
Summary: The temperature dependence of the critical stress of the R -> B19' transformation in NiTi shape memory alloys has been found to be negative in this study, in contrast to previous reports. This discovery calls for a reevaluation of this transformation.
MATERIALS RESEARCH LETTERS
(2023)
Article
Chemistry, Multidisciplinary
Pousali Ghosh, Jiasen Guo, Feng Ye, Thomas Heitmann, Steven Kelley, Arthur Ernst, Vitalii Dugaev, Deepak K. K. Singh
Summary: This study investigates the potential of NiSi metal in high-temperature antiferromagnetic spintronics. It reveals high-temperature antiferromagnetism in single-crystal NiSi with a Neel temperature above 700 K. The antiferromagnetic order in NiSi has non-centrosymmetric magnetic character and a small ferromagnetic component in the a-c plane. Furthermore, NiSi exhibits different magnetic and electronic hysteresis responses to field applications due to the disparity in two moment directions, and these switching behaviors persist to high temperature. These findings highlight the importance of NiSi in the pursuit of antiferromagnetic spintronics.
ADVANCED MATERIALS
(2023)
Article
Multidisciplinary Sciences
Bin Gao, Tong Chen, Xiao-Chuan Wu, Michael Flynn, Chunruo Duan, Lebing Chen, Chien-Lung Huang, Jesse Liebman, Shuyi Li, Feng Ye, Matthew B. Stone, Andrey Podlesnyak, Douglas L. Abernathy, Devashibhai T. Adroja, Manh Duc Le, Qingzhen Huang, Andriy H. Nevidomskyy, Emilia Morosan, Leon Balents, Pengcheng Dai
Summary: Magnetic order can still occur in materials with spin-singlet ground state due to exchange interactions mixing excited crystal electric field states. The study investigates Ni2Mo3O8 and finds that crystal electric field states in both the paramagnetic and antiferromagnetic states exhibit dispersive excitations.
NATURE COMMUNICATIONS
(2023)
Article
Materials Science, Multidisciplinary
Jiacheng Ge, Peng Luo, Zhenduo Wu, Wentao Zhang, Sinan Liu, Si Lan, Jonathan D. Almer, Yang Ren, Xun-Li Wang, Weihua Wang
Summary: Studying the flow behavior of amorphous solids is crucial for understanding their deformation mechanism, but detecting basic flow events in these materials is challenging. Using simultaneous SAXS/WAXS experiments, researchers have identified elementary flow carriers in wound metallic glasses, with a radius of gyration ranging from 2.5 to 3.5 nm, based on flow-induced structural heterogeneities. The size of these carriers increases and their morphology changes from spherical to rod-like during flow. Additionally, the atomic structure undergoes an unusual change to a more disordered state during winding/annealing at a temperature around 0.8 Tg. This work provides an atomic-to-nanoscale description of flow carriers in amorphous solids during deformation.
MATERIALS RESEARCH LETTERS
(2023)
Article
Chemistry, Physical
Jincan Ren, Yu Tang, Weibao Li, Dong He, He Zhu, Xingyu Wang, Si Lan, Zijia Yin, Tingting Yang, Zhaowen Bai, Yang Ren, Xiangheng Xiao, Qi Liu
Summary: A synergetic strategy of La, Mg co-doping and LiAlO2@Al2O3 surface coating is designed to enhance the performance of LiCoO2 (CM-LCO) cathode material under extreme temperatures. CM-LCO exhibits excellent temperature adaptability and remarkable electrochemical performance, as well as excellent cycle stability and high-rate performance. The synergistic effects of this co-modification strategy are demonstrated by investigating the electrochemical reaction kinetics and structure evolution of CM-LCO, providing a promising strategy for the application of high-voltage LCO in a wide temperature range.
Article
Chemistry, Multidisciplinary
Jiantao Li, Guangwu Hu, Ruohan Yu, Xiaobin Liao, Kangning Zhao, Tianyi Li, Jiexin Zhu, Qiang Chen, Dong Su, Yang Ren, Khalil Amine, Liqiang Mai, Liang Zhou, Jun Lu
Summary: The integration of Si into TiO2 enhances charge transfer and increases lithium-ion storage capacity.
Article
Chemistry, Multidisciplinary
Fan Xue, Qiang Li, Mingxin Lv, Yuanfei Song, Tianxing Yang, Xiaoge Wang, Tianyi Li, Yang Ren, Koji Ohara, Yufei He, Dianqing Li, Qiheng Li, Xin Chen, Kun Lin, Xianran Xing
Summary: This study reports the local structure of Pd nanocatalysts, revealing the atomic surface distribution of unique compressed strain in Pd nanocatalysts. The surface strain, induced by the shape of the catalyst, significantly weakens the adsorption energy of ethylene and avoids the over-hydrogenation of acetylene, leading to higher selectivity for ethylene.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2023)
Article
Chemistry, Multidisciplinary
Jian Hui, Qingyun Hu, Hongjian Yuan, Ruiqian Shi, Xiang Huang, Yuanyuan Wu, Yang Ren, Zhan Zhang, Hong Wang
Summary: By using high-throughput experiments, the optical properties and structural evolution of Ge-Sb-Te alloy films were studied, and it was found that the modulation period and chemical composition have a significant impact on amorphous stability and optical properties.
Article
Materials Science, Multidisciplinary
Jiacheng Ge, Yao Gu, Zhongzheng Yao, Sinan Liu, Huiqiang Ying, Chenyu Lu, Zhenduo Wu, Yang Ren, Jun-ichi Suzuki, Zhenhua Xie, Yubin Ke, Jianrong Zeng, He Zhu, Song Tang, Xun-Li Wang, Si Lan
Summary: Fe-based metallic glasses are promising materials in the fields of advanced magnetism and sensors. This study proposes a novel approach to tailor the amorphous structure through liquid-liquid phase transition, and provides insights into the correlation between structural disorder and magnetic order. The results show that the liquid-liquid phase transition can induce more locally ordered nanodomains, leading to stronger exchange interactions and increased saturation magnetization. The increased local heterogeneity also enhances magnetic anisotropy, resulting in a better stress-impedance effect.
JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
(2024)