期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 15, 期 18, 页码 6849-6855出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3cp50992c
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资金
- Office of FreedomCAR and Vehicle Technologies of the U. S. Department of Energy [DE-AC02-05CH11231]
Rechargeable lithium or lithium-ion cells can be overcharge-protected by an electroactive polymer composite separator. The use of non-woven fibrous membranes instead of conventional microporous membranes as the composite substrates allowed better distribution of the electroactive polymer, which led to improved utilization and a 40-fold increase in sustainable current density. For the first time, stable overcharge protection for hundreds of cycles was demonstrated in several cell chemistries, including LiNi1/3Co1/3Mn1/3O2, LiFePO4, and spinel Li1.05Mn1.95O4 half-cells. Protection at a charging rate as high as 5 C was achieved at a steady state cell potential below 4.85 V.
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