期刊
ORGANIC LETTERS
卷 17, 期 2, 页码 310-313出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol503404p
关键词
-
资金
- Chinese National Natural Science Foundation [81430080, 81125021, 81373277]
- Major State Basic Research Development Program [2015CB910603]
A new strategy is reported for the economical synthesis of indoles bearing an N-(3-aminobut-2-enoyl) substituent through RhIII-catalyzed redox-neutral C-H activation of pyrazolones and alkynes. This approach utilizes cheap substrates and mild reaction conditions to access a unique class of indoles via a N-N bond oxidative cleavage without loss of the N-terminus, therefore meeting all the atom/step/redox economy principles.
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