期刊
ORGANIC LETTERS
卷 16, 期 21, 页码 5556-5559出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol502553p
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资金
- Uppsala University
- Wenner-Gren foundation
- Swedish Institute
- Stiftelsen Olle Engkvist Byggmastare
- Vetenskapsradet
An atom-efficient synthesis of keto thioethers was devised via tandem gold/palladium catalysis. The reaction proceeds through a regioselective thiol attack at the beta-position of the alcohol, followed by an alkyl, aryl, or benzyl 1,2-shift. Both acyclic and cyclic systems were studied, in the latter case leading to the ring expansion of cyclic substrates.
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