期刊
ORGANIC LETTERS
卷 16, 期 24, 页码 6350-6353出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol503128j
关键词
-
资金
- Natural Science Foundation of China [21272165]
A new radical-polar crossover reaction has been developed involving the combination of a tandem radical reaction and KornblumDeLaMare rearrangement in a one-pot process. This simple methodology allows for the construction of polyfunctionalized carbonyl compounds via the oxidative coupling of 1,3-dioxolanes with electron-deficient alkenes and vinylarenes in the presence of Co(salen) and TBHP under mild conditions. This reaction also exhibited high functional group tolerance, wide substrate scope, and operational simplicity.
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