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卷 15, 期 8, 页码 1918-1921出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol400568u
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- JSPS
- ERATO from JST
Fe-catalyzed direct dehydrogenative C(3)-functionalization of tertiary arylamines was developed via activation of the sp(3) C(3)-H bond. The reaction is applicable to both cyclic and acyclic amines. The key process is the catalytic desaturative enamine formation from tertiary amines and position-selective C-C bond formation (addition to nitro olefins) at the beta-carbon. Products can be converted to versatile and unique nitrogen-containing molecules.
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